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Motivated by recent neutron and x-ray observations in V$_2$O$_3$, we derive the effective Hamiltonian in the strong coupling limit of an Hubbard model with three degenerate t_{2g} states containing two electrons coupled to spin S = 1, and…

Strongly Correlated Electrons · Physics 2025-04-14 S. Di Matteo , N. B. Perkins , C. R. Natoli

We criticize the model proposed by Mila et al. (Phys.Rev.Lett. 85 (2000) 1714) for the description of the V3+ ion in V2O3 by pointing out that it is completely artificial because the condition about the degenerate (doublet) orbital ground…

Strongly Correlated Electrons · Physics 2007-05-23 R. J. Radwanski , Z. Ropka

Motivated by the recent neutron diffraction experiment on $YVO_3$, we consider a microscopic model where each $V^{3+}$ ion is occupied by two 3d electrons of parallel spins with two fold degenerate orbital configurations. The mean field…

Strongly Correlated Electrons · Physics 2007-05-23 Theja N. De Silva , Anuvrat Joshi , Michael Ma , Fu Chun Zhang

We have attributed magnetism and electronic structure of V2O3 to the V3+ ions. We claim that the V3+ ion in V2O3 should be considered as described by the quantum numbers S=1 and L=3. Such quantum numbers result from two Hund's rules. The…

Strongly Correlated Electrons · Physics 2007-05-23 R. J. Radwanski , Z. Ropka

The 3d electronic structure and phase transition in pure and Cr doped V2O3 are theoretically investigated in relation to the 3d spin-orbit interaction and lattice distortion. A model consisting of the nearest-neighbor V ion pair with full…

Strongly Correlated Electrons · Physics 2016-08-31 Arata Tanaka

The (SrTiO$_3$)$_m$/(SrVO$_3$)$_n$ $d^0-d^1$ multilayer system is studied with first principles methods through the observed insulator-to-metal transition with increasing thickness of the SrVO$_3$ layer. When correlation effects with…

Strongly Correlated Electrons · Physics 2015-05-19 Victor Pardo , Warren E. Pickett

Spin correlations in metallic and insulating phases of $V_2O_3$ and its derivatives are investigated using magnetic neutron scattering. Metallic samples have incommensurate spin correlations varying little with hole doping. Paramagnetic…

Strongly Correlated Electrons · Physics 2009-10-28 Wei Bao , C. Broholm , G. Aeppli , P. Dai , J. M. Honig , P. Metcalf

Neutron scattering was used to determine the spin structure and the magnon spectrum of the Mott--Hubbard insulator YTiO$_3$. The magnetic structure is complex, comprising substantial G-type and A-type antiferromagnetic components in…

Strongly Correlated Electrons · Physics 2009-11-07 C. Ulrich , G. Khaliullin , S. Okamoto , M. Reehuis , A. Ivanov , H. He , Y. Taguchi , Y. Tokura , B. Keimer

The local structure of (Al_0.06V_0.94)_2O_3 in the paramagnetic insulating (PI) and antiferromagnetically ordered insulating (AFI) phase has been investigated using hard and soft x-ray absorption techniques. It is shown that: 1) on a local…

Strongly Correlated Electrons · Physics 2009-11-07 P. Pfalzer , J. Will , A. Nateprov , M. Klemm , V. Eyert , S. Horn , A. I. Frenkel , S. Calvin , M. L. denBoer

We have carried out a comparative theoretical study of the electronic structure of the novel one-dimensional Ca$_3$CoRhO$_6$ and Ca$_3$FeRhO$_6$ systems. The insulating antiferromagnetic state for the Ca$_3$FeRhO$_6$ can be well explained…

Strongly Correlated Electrons · Physics 2007-06-21 Hua Wu , Z. Hu , D. I. Khomskii , L. H. Tjeng

The collective behavior of correlated electrons in the VO$_2-$interface layer of LaVO$_3$/SrTiO$_3$ heterostructure is studied within a quarter-filled $t_{2g}$-orbital Hubbard model on a square lattice. We argue that the ground state is…

Strongly Correlated Electrons · Physics 2008-11-21 G. Jackeli , G. Khaliullin

5$d$ transition metal oxides host a variety of exotic phases due to the comparable strength of Coulomb repulsion and spin-orbit coupling. Herein, by pursuing density-functional studies on a delta-doped quasi-two-dimensional iridate…

Materials Science · Physics 2023-11-16 Amit Chauhan , Arijit Mandal , B. R. K. Nanda

The odd-parity spin-triplet Cooper pairing states show a six-fold degeneracy for a quasi-two-dimensional electron system. In this article we show how spin-orbit coupling can lift this degeneracy for Sr_2RuO_4 taking the band structure based…

Superconductivity · Physics 2009-10-31 Kwai-Kong Ng , Manfred Sigrist

Static electrical and magnetic properties of single crystal BaVS_3 were measured over the structural (T_S=240K), metal-insulator (T_MI=69K), and suspected orbital ordering (T_X=30K) transitions. The resistivity is almost isotropic both in…

Strongly Correlated Electrons · Physics 2009-10-31 G. Mihaly , I. Kezsmarki , F. Zamborszky , M. Miljak , K. Penc , P. Fazekas , H. Berger , L. Forro

We discuss the ground state properties of a spin 1/2 magnetic ion with threefold $t_{2g}$ orbital degeneracy on a highly frustrated pyrochlore lattice, like Ti$^{3+}$ ion in B-spinel MgTi$_2$O$_4$. We formulate an effective spin-orbital…

Strongly Correlated Electrons · Physics 2007-05-23 S. Di Matteo , G. Jackeli , N. B. Perkins

We have calculated the electronic structure of V2O3 associated with the V3+ ions taking into account strong on-site electron correlations and the spin-orbit coupling. Closely lying 9 states of the subterm 3T1g are a physical reason for…

Strongly Correlated Electrons · Physics 2007-05-23 Z. Ropka R. J. Radwanski

Recent neutron scattering and nuclear magnetic resonance experiments have revealed that the low temperature phase of doped V_{2-y}O_3 is an itinerant antiferromagnet with a helical spin structure. We use a band structure calculation as the…

Strongly Correlated Electrons · Physics 2009-10-31 T. Wolenski , M. Grodzicki , J. Appel

We performed resonant x-ray diffraction experiments at the $L$ absorption edges for the post-perovskite-type compound CaIrO$_{3}$ with $(t_{2g})^5$ electronic configuration. By observing the magnetic signals, we could clearly see that the…

We present our theoretical results on the mechanism of two transitions in vanadium spinel oxides $A$V$_2$O$_4$ ($A$=Zn, Mg, or Cd) in which magnetic V cations constitute a geometrically-frustrated pyrochlore structure. We have derived an…

Strongly Correlated Electrons · Physics 2007-05-23 Yukitoshi Motome , Hirokazu Tsunetsugu

The semi-metallic behavior of the perovskite iridate SrIrO3 shifts the end-member of the strongly spin-orbit (SO) coupled Ruddlesden-Popper series Srn+1IrnO3n+1 away from the Mott insulating regime and the half-filled pseudospin Jeff=1/2…

Strongly Correlated Electrons · Physics 2025-02-06 Dirk Fuchs , Arun Kumar Jaiswal , Fabrice Wilhelm , Di Wang , Andre Rogalev , Matthieu Le Tacon
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