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We report neutron scattering studies of the spin correlations of the geometrically frustrated pyrochlore Tb2Mo2O7 using single crystal samples. This material undergoes a spin-freezing transition below Tg~24 K, similar to Y2Mo2O7, and has…

Strongly Correlated Electrons · Physics 2009-11-13 D. K. Singh , J. S. Helton , S. Chu , T. H. Han , C. J. Bonnoit , S. Chang , H. J. Kang , J. W. Lynn , Y. S. Lee

We investigated the nature of the spin glass-like phase transition in the geometrically frustrated pyrochlore lattices Y$_{2}$Mo$_{2}$O$_{7}$ using the local probes nuclear and muon magnetic resonances, and the field-dependent long range…

Strongly Correlated Electrons · Physics 2010-09-24 Oren Ofer , Amit Keren , Jason S. Gardner , Yang Ren , W. A. MacFarlane

The glassy behavior observed in the pyrochlore magnet Y2Mo2O7, where the magnetic Mo^{4+} ions interact predominantly via isotropic nearest neighbor antiferromagnetic exchange, possibly with additional weak disorder, is a distinct class of…

Statistical Mechanics · Physics 2010-09-08 Ka-Ming Tam , Adam J. Hitchcock , Michel J. P. Gingras

The formation of a spin glass usually requires both structural disorder and frustrated magnetic interactions. Consequently, the origin of spin-glass behaviour in Y$_2$Mo$_2$O$_7$ $-$ in which magnetic Mo$^{4+}$ ions occupy a frustrated…

Some frustrated pyrochlore antiferromagnets, such as Y2Mo2O7, show a spin-freezing transition and magnetic irreversibilities below a temperature Tf similar to what is observed nonlinear magnetization measurements on Y2Mo2O7 that provide…

Disordered Systems and Neural Networks · Physics 2009-10-28 M. J. P. Gingras , C. V. Stager , N. P. Raju , B. D. Gaulin , J. E. Greedan

We show theoretically that spin and orbital degrees of freedom in the pyrochlore oxide Y2Mo2O7, which is free of quenched disorder, can exhibit a simultaneous glass transition, working as dynamical randomness to each other. The interplay of…

Disordered Systems and Neural Networks · Physics 2020-03-04 Kota Mitsumoto , Chisa Hotta , Hajime Yoshino

Geometric frustration inhibits magnetic systems from ordering, opening a window to unconventional phases of matter. The paradigmatic frustrated lattice in three dimensions to host a spin liquid is the pyrochlore, although there remain few…

The spin glass behavior of Y2Mo2O7 has puzzled physicists for nearly three decades. Free of bulk disorder within the resolution of powder diffraction methods, it is thought that this material is a rare realization of a spin glass resulting…

We report on the study of unusual spin glass properties in the geometrically frustrated pyrochlore Tb$_{2}$Mo$_{2}$O$_{7}$, $T$$_{g}$$\simeq$24 K. The analysis of the nonlinear part of dc and complex susceptibilities, near the glass…

Strongly Correlated Electrons · Physics 2013-09-17 D. K. Singh , Y. S. Lee

We have investigated the 89Y NMR spectrum and spin lattice relaxation, T1, in the magnetically frustrated pyrochlore Y2Mo2O7. We find that upon cooling the spectrum shifts, and broadens asymmetrically. A detailed examination of the low T…

Strongly Correlated Electrons · Physics 2009-11-07 Amit Keren , Jason S. Gardner

We investigated the nature of the freezing in the geometrically frustrated Heisenberg spin-glass Y2Mo2O7 by measuring the temperature dependence of the static internal magnetic field distribution above the spin-glass temperature, Tg, using…

Strongly Correlated Electrons · Physics 2009-11-11 Eva Sagi , Oren Ofer , Amit Keren , Jason S. Gardner

We propose the idea of a spin-lattice liquid, in which spin and lattice degrees of freedom are strongly coupled and remain disordered and fluctuating down to low temperatures. We show that such a state arises naturally from a microscopic…

Strongly Correlated Electrons · Physics 2019-06-12 Andrew Smerald , George Jackeli

We present an extensive numerical study of a new type of frustrated itinerant magnetism on the pyrochlore lattice. In this theory, the pyrochlore magnet can be viewed as a cross-linking network of Kondo or double-exchange chains. Contrary…

Strongly Correlated Electrons · Physics 2018-12-17 Jing Luo , Gia-Wei Chern

To search for novel spin-charge coupled phenomena in the strongly correlated electron system on a frustration lattice, charge transport and dynamics have been investigated for the hole-doped spin-glass (Mott) insulator…

Strongly Correlated Electrons · Physics 2011-09-20 S. Iguchi , Y. Kumano , K. Ueda , S. Kumakura , Y. Tokura

Although materials that exhibit nearest-neighbor-only antiferromagnetic interactions and geometrical frustration theoretically should not magnetically order in the absence of disorder, few such systems have been observed experimentally. One…

Strongly Correlated Electrons · Physics 2016-08-31 S. -W. Han , J. S. Gardner , C. H. Booth

Geometrical frustration, as in pyrochlore lattices made of corner-sharing tetrahedra, precludes the onset of conventional magnetic ordering, enabling the stabilization of fluctuating spin states at low temperature. Disorder is a subtle…

The recent discovery of Spin-ice is a spectacular example of non-coplanar spin arrangements that can arise in the pyrochlore A2B2O7 structure. We present magnetic and thermodynamic studies on the metallic-ferromagnet pyrochlore Sm2Mo2O7.…

Strongly Correlated Electrons · Physics 2009-11-13 Surjeet Singh , R. Suryanarayanan , R. Tackett , G. Lawes , A. K. Sood , P. Berthet , A. Revcolevschi

Three-dimensionally (3D) frustrated magnets generally exist in the magnetic diamond and pyrochlore lattices, in which quantum fluctuations suppress magnetic orders and generate highly entangled ground states (GS). LiYbSe2 in a previously…

Strongly Correlated Electrons · Physics 2022-06-15 Ranuri S. Dissanayaka Mudiyanselage , Haozhe Wang , Olivia Vilella , Martin Mourigal , Gabriel Kotliar , Weiwei Xie

Neutron scattering measurements show the ferromagnetic XY pyrochlore Yb2Ti2O7 to display strong quasi-two dimensional (2D) spin correlations at low temperature, which give way to long range order (LRO) under the application of modest…

Strongly Correlated Electrons · Physics 2010-02-08 K. A. Ross , J. P. C. Ruff , C. P. Adams , J. S. Gardner , H. A. Dabkowska , Y. Qiu , J. R. D. Copley , B. D. Gaulin

In frustrated magnetic systems, geometric constraints or the competition amongst interactions introduce extremely high degeneracy and prevent the system from readily selecting a low-temperature ground state. The most frustrated known spin…

Strongly Correlated Electrons · Physics 2016-11-23 Darren C. Peets , Hasung Sim , Maxim Avdeev , Je-Geun Park
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