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The structure of the first sharp diffraction peak (FSDP) of amorphous silicon (${\it a}$-Si) near 2 Angstrom$^{-1}$ is addressed with particular emphasis on the position, intensity, and width of the diffraction curve. By studying a number…

Disordered Systems and Neural Networks · Physics 2021-10-04 Devilal Dahal , Hiroka Warren , Parthapratim Biswas

In hydrogenated amorphous silicon oxide (a-SiO:H) films, incorporation of oxygen enhances optical gap due to a large number of St-O-Si bond formation, which lies deep into valence band states. An induction effect of this Si-O on other bonds…

Condensed Matter · Physics 2007-11-17 S. M. Iftiquar

The recent synthesis of a four-fold silylated sila-adamantane molecule (C$_{24}$H$_{72}$Si$_{14}$, T$_d$), [J. Fischer, J. Baumgartner, and C. Marschner, {\it Science} {\bf 310,} (2005) 825] is the first attempt of making the silicon…

Chemical Physics · Physics 2010-05-31 Rajendra R. Zope , Tunna Baruah , Mark R. Pederson , Steven L. Richardson

We present Raman spectroscopy of the polycrystalline Si and Ge films deposited by molecular beam deposition on a dielectric substrate. The Raman study has been made using lasers with different wavelengths. Structural properties of the…

Glasses have a large excess of low-frequency vibrational modes in comparison with continuous elastic body, the so-called Boson Peak, which appears to correlate with several crucial properties of glasses, such as transport or fragility. I…

Materials Science · Physics 2014-11-19 Matthieu Wyart

Raman spectroscopic study of amorphous carbon layers for two different excitation wavelengths at room temperature. The amount of sp3 bondings is estimated to about 10% for both samples, evaluated from the ratio of the D- and G-Raman line…

Materials Science · Physics 2012-03-02 J. Debus

A theoretical study describing the coherence properties of near-field Raman scattering in two- and one-dimensional systems is presented. The model is applied to the Raman modes of pristine graphene and graphene edges. Our analysis is based…

Mesoscale and Nanoscale Physics · Physics 2014-03-31 Luiz Gustavo Cançado , Ryan Beams , Ado Jorio , Lukas Novotny

The complex interactions between orbital angular momentum (OAM) light and atoms are particularly intriguing in the areas of quantum optics and quantum information science. Building a versatile high-dimensional quantum network needs broad…

Quantum Physics · Physics 2019-02-15 Dong-Sheng Ding , Ming-Xin Dong , Wei Zhang , Shuai Shi , Yi-Chen Yu , Ying-Hao Ye , Guang-Can Guo , Bao-Sen Shi

Low-frequency Raman scattering spectra are presented for gold nanocrystals with diameters 3.5 and 13 nm. The frequencies of the Raman peaks but also their number are shown to vary with the nanocrystal size. These results are analyzed using…

Mesoscale and Nanoscale Physics · Physics 2012-02-09 Lucien Saviot , Nicolas Combe , Adnen Mlayah

We derive the frequency shifts and the broadening of $\Gamma$ point longitudinal optical (LO) and transverse optical (TO) phonon modes, due to electron-phonon interaction, in graphene under uniaxial strain as a function of the electron…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Mohamed Assili , Sonia Haddad

We study theoretically the Raman spectrum of the rotated double-layer graphene, consisting of two graphene layers rotated with respect to each other by an arbitrary angle \theta. We find a relatively simple dependence of the Raman G peak…

Mesoscale and Nanoscale Physics · Physics 2013-11-05 Sinisa Coh , Liang Z. Tan , Steven G. Louie , Marvin L. Cohen

Topological insulators are bulk semiconductors that manifest in-gap massless Dirac surface states due to the topological bulk-boundary correspondence principle [1-3]. These surface states have been a subject of tremendous ongoing interest,…

Raman spectroscopic investigations are carried out on one-dimensional nanostructures of InN,such as nanowires and nanobelts synthesized by chemical vapor deposition. In addition to the optical phonons allowed by symmetry; A1, E1 and…

Materials Science · Physics 2009-11-13 Satyaprakash Sahoo , M. S. Hu , C. W. Hsu , C. T. Wu , K. H. Chen , L. C. Chen , A. K. Arora , S. Dhara

We investigate the Raman spectra in the geometry where both incident and scattered photon polarizations are parallel to the $\hat{z}$-direction, for a plane-chain bilayer coupled via a single-particle tunneling $t_\perp$. The Raman vertex…

Condensed Matter · Physics 2016-08-31 W. C. Wu , J. P. Carbotte

For quantitative electron microscopy high precision position information is necessary so that besides an adequate resolution and sufficiently strong contrast of atoms, small width of peaks which represent atoms in structural images is…

Materials Science · Physics 2016-01-11 Binghui Ge , Yumei Wang , Yuan Yao , Fanghua Li

Amorphous silicon films prepared by electron beam evaporation have systematically and substantially greater atomic density for higher thickness, higher growth temperature, and slower deposition rate, reaching the density of crystalline Si…

Materials Science · Physics 2022-04-27 H. C. Jacks , M. Molina-Ruiz , M. H. Weber , J. J. Maldonis , P. M. Voyles , T. H. Metcalf , X. Liu , F. Hellman

For many materials, Raman spectra are intricately structured and provide valuable information about compositional stoichiometry and crystal quality. Here we use density-functional theory calculations, mass approximation, and the Raman…

Materials Science · Physics 2024-09-04 Nima Ghafari Cherati , I. Abdolhosseini Sarsari , Arsalan Hashemi , Tapio Ala-Nissila

This work presents how first-principles simulations validated through experimental measurements lead to a new accurate prediction of the expected Raman shift as a function of strain in silicon. Structural relaxation of a strained primitive…

Applied Physics · Physics 2023-01-31 Nicolas Roisin , Marie-Stéphane Colla , Jean-Pierre Raskin , Denis Flandre

We present a first-principles study of the structural, electronic, and optical properties of hydrogenated amorphous silicon (a-Si:H). To this end, atomic configurations of a-Si:H with 72 and 576 atoms respectively are generated using…

Materials Science · Physics 2017-03-31 Philippe Czaja , Urs Aeberhard , Massimo Celino , Simone Giusepponi , Michele Gusso

A comparison of experimentally observed Raman scattering data with Raman line-shapes, generated theoretically using phonon confinement model, has been carried out to understand the sensitivity of different Raman spectral parameters on…

Mesoscale and Nanoscale Physics · Physics 2020-03-20 Neeshu K. M. , Chanchal Rani , Ritika Kaushik , Manushree Tanwar , Ashisha Kumar , Rajesh Kumar