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We identify putative load-bearing structures (bridges) in experimental colloidal systems studied by confocal microscopy. Bridges are co-operative structures that have been used to explain stability and inhomogeneous force transmission in…

Soft Condensed Matter · Physics 2010-06-18 Matthew C. Jenkins , Mark D. Haw , Gary C. Barker , Wilson C. K. Poon , Stefan U. Egelhaaf

A model for the radial distribution function $g(r)$ of a square-well fluid of variable width previously proposed [S. B. Yuste and A. Santos, J. Chem. Phys. {\bf 101}, 2355 (1994)] is revisited and simplified. The model provides an explicit…

Statistical Mechanics · Physics 2007-05-23 L. Acedo , A. Santos

A theoretical description for the radial density profile of a finite number of identical charged particles confined in a harmonic trap is developed for application over a wide range of Coulomb coupling (or, equivalently, temperatures) and…

Statistical Mechanics · Physics 2015-05-14 J. Wrighton , J. W. Dufty , H. Kählert , M. Bonitz

In this paper, starting from the Born-Green-Yvon (BGY) equation, we derive a general expression for the contact value of the singlet distribution function near a hard wall for anisotropic fluids. This relation includes two separate…

Soft Condensed Matter · Physics 2022-11-16 M. Holovko , D. di Caprio

A variational formulation for the calculation of interacting fermion systems based on the density-matrix functional theory is presented. Our formalism provides for a natural integration of explicit many-particle effects into standard…

Strongly Correlated Electrons · Physics 2013-05-29 Peter E. Bloechl , Christian F. J. Walther , Thomas Pruschke

Liquid capillary-bridge formation between solid particles has a critical influence on the rheological properties of granular materials and, in particular, on the efficiency of fluidized bed reactors. The available analytical and…

Soft Condensed Matter · Physics 2021-08-12 Lei Yang , Marcello Sega , Jens Harting

We derive an exact equation for density changes induced by a general external field that corrects the hydrostatic approximation where the local value of the field is adsorbed into a modified chemical potential. Using linear response theory…

Statistical Mechanics · Physics 2009-10-31 Kirill Katsov , John D. Weeks

We discuss the effective donor/acceptor coupling for a bridged electron transfer system with a site-diagonal disorder of bridge energies. The average spectral properties of the system are discussed by using the Wegner model (Anderson's type…

Condensed Matter · Physics 2009-10-30 Ewa Gudowska-Nowak , Gabor Papp , Juergen Brickmann

The van der Waals density functional (vdW-DF) of Dion et al. [Phys. Rev. Lett. 92, 246401 (2004)] is a promising approach for including dispersion in approximate density functional theory exchange-correlation functionals. Indeed, an…

Materials Science · Physics 2013-01-30 Jiří Klimeš , David R. Bowler , Angelos Michaelides

A quantitative model of the mobility of functionalized particles at the interface is pivotal to understanding important systems in biology and nanotechnology. In this work, we investigate the emerging dynamics of particles anchored through…

Soft Condensed Matter · Physics 2024-06-19 Janna Lowensohn , Laurie Stevens , Daniel Goldstein , Bortolo Matteo Mognetti

The mode-coupling theory of the glass transition predicts the time evolution of the intermediate scattering functions in viscous liquids on the sole basis of the structural information encoded in two-point density correlations. We provide a…

Statistical Mechanics · Physics 2010-10-01 Ludovic Berthier , Gilles Tarjus

This paper describes a mixed direct-iterative method for boundary integral formulations of dielectric solvation models. We give an example for which a direct solution at thermal accuracy is nontrivial and for which Gauss-Seidel iteration…

chem-ph · Physics 2008-02-03 S. A. Corcelli , J. D. Kress , L. R. Pratt , G. J. Tawa

We performed a benchmark study on a series of dihydrogen bond complexes and constructed a set of reference bond distances and interaction energies. The test set was employed to assess the performance of several wave-function correlated and…

Chemical Physics · Physics 2015-01-22 E. Fabiano , L. A. Constantin , F. Della Sala

Different advanced bridge function closures are utilized to investigate the structural and thermodynamic properties of dense Yukawa one-component plasma liquids within the framework of integral equation theory. The isomorph-based…

Soft Condensed Matter · Physics 2021-01-21 F. Lucco Castello , P. Tolias

Radial-basis-function networks are traditionally defined for sets of vector-based observations. In this short paper, we reformulate such networks so that they can be applied to adjacency-matrix representations of weighted, directed graphs…

Machine Learning · Computer Science 2019-08-05 Isaac J. Sledge , Jose C. Principe

We use a recently derived diagrammatic formulation of the dynamics of interacting Brownian particles [G. Szamel, J. Chem. Phys. 127, 084515 (2007)] to study a four-point dynamic density correlation function. We re-sum a class of diagrams…

Statistical Mechanics · Physics 2009-11-13 Grzegorz Szamel

We consider binary mixtures of soft repulsive spherical particles and calculate the depletion interaction between two big spheres mediated by the fluid of small spheres, using different theoretical and simulation methods. The validity of…

Correlation functions provide information on the properties of mesons in vacuum and of hot nuclear matter. In this Letter, we present a new method to derive a well-defined spectral representation for correlation functions. Combining this…

Nuclear Theory · Physics 2013-07-19 Si-xue Qin

Determining the microstructure of colloidal suspensions under shear flows has been a challenge for theoretical and computational methods due to the singularly-perturbed boundary-layer nature of the problem. Previous approaches have been…

Soft Condensed Matter · Physics 2019-06-05 L. Banetta , A. Zaccone

An alternative type of approximation for the exchange and correlation functional in density functional theory is proposed. This approximation depends on a variable $u$ that is able to detect inhomogeneities in the electron density $\rho$…

Materials Science · Physics 2019-01-02 Fabien Tran , Peter Blaha