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We present a new method for modeling disordered solid solutions, based on the virtual crystal approximation (VCA). The VCA is a tractable way of studying configurationally disordered systems; traditionally, the potentials which represent…

Materials Science · Physics 2009-10-31 Nicholas J. Ramer , Andrew M. Rappe

We present an approach to the implementation of the virtual crystal approximation (VCA) for the study of properties of solid solutions in the context of density-functional methods. Our approach can easily be applied to any type of…

Materials Science · Physics 2009-10-31 L. Bellaiche , David Vanderbilt

The variational cluster approach (VCA) is applied to study spontaneous ferromagnetism in the Hubbard model at zero temperature. We discuss several technical improvements of the numerical implementation of the VCA which become necessary for…

Strongly Correlated Electrons · Physics 2010-12-03 Matthias Balzer , Michael Potthoff

The four-state model is proposed for description of phase transition in ferroelectric crystals of DMAGaS and DMAAlS type. Thermodynamical functions of the model are obtained in the mean field approximation. The phase transition between…

Materials Science · Physics 2007-05-23 I. V. Stasyuk , O. V. Velychko

Using the variational cluster approach (VCA), we study the transition from the antiferromagnetic to the superconducting phase of the two-dimensional Hubbard model at zero temperature. Our calculations are based on a new method to evaluate…

Strongly Correlated Electrons · Physics 2007-05-23 M. Aichhorn , E. Arrigoni , M. Potthoff , W. Hanke

A single crystal of lead-zirconate-titanate (PZT), composition Pb(Zr0.80Ti0.20)O3, was studied by polarized-Raman scattering as a function of temperature. Raman spectra reveal that the local structure deviates from the average structure in…

Materials Science · Physics 2015-06-23 J. Frantti , Y. Fujioka , A. Puretzky , Y. Xie , Z. -G. Ye , C. Parish , A. M. Glazer

A new approach in the investigation of the order parameter behaviour near ferroelectric phase transition point is suggested. The short range and dipole interactions between particles are taken into account. The logarithmic corrections and…

Statistical Mechanics · Physics 2013-07-16 M. A. Korynevskii , V. B. Solovyan

Molecular ferroelectrics have captured immense attention due to their superiority over inorganic oxide ferroelectrics, such as environmentally friendly, low-cost, flexible, foldable. However, the mechanisms of ferroelectric switching and…

Chemical Physics · Physics 2021-06-18 Xiaoqing Zhu , Wenbin Fan , Wei Ren , Yongle Li

A first-principles-derived approach is used to study structural, piezoelectric and dielectric properties of Pb(Zr_{1-x}Ti_{x})O_{3} (PZT) solid solutions near the morphotropic phase boundary at low temperature. Three ferroelectric phases…

Materials Science · Physics 2007-05-23 L. Bellaiche , A. Garcia , David Vanderbilt

We present a theoretical investigation of the anomalous ferroelectricity of mixed-stack charge transfer molecular crystals, based on the Peierls-Hubbard model, and first principles calculations for its parameterization. This approach is…

Materials Science · Physics 2014-09-30 Gabriele D'Avino , Matthieu J. Verstraete

A detailed investigation using variable temperature powder neutron diffraction demonstrates that BiFeO3 undergoes a phase transition from the ferroelectric alpha phase (rhombohedral, R3c) to a paraelectric beta phase (orthorhombic, Pbnm)…

Materials Science · Physics 2009-08-21 Donna C. Arnold , Kevin S. Knight , Finlay D. Morrison , Philip Lightfoot

Perturbed angular correlation spectroscopy combined with $ab-initio$ electronic structure calculations is used to unravel the structural phase transition path from the low-temperature polar structure to the high-temperature structural phase…

(1-x)Li0.12Na0.88NbO3-xBaTiO3 (0 to x to 0.40) ferroelectric ceramics were prepared using conventional ceramics route and their phase transitional behavior is investigated by using dielectric spectroscopy. The temperature-dependent…

Materials Science · Physics 2014-12-17 Supratim Mitra , Ajit R. Kulkarni

We have investigated the dielectric properties of Gd$_{1-x}$Tb$_{x}$MnO$_{3}$ crystals in magnetic fields to clarify the crossover between two distinct ferroelectric phases, GdMnO$_{3}$-type (first-order displacive) and TbMnO$_{3}$-type…

Strongly Correlated Electrons · Physics 2009-11-11 K. Noda , S. Nakamura , H. Kuwahara

We present a semi-empirical effective Hamiltonian to capture effects of disorder associated with Ba and Sr cations occupying $A$ sites in (Ba$_{x}$Sr$_{1-x}$)TiO$_3$ on its ferroelectric phase transition. Averaging between the parameters of…

Materials Science · Physics 2016-10-28 Takeshi Nishimatsu , Anna Gruenebohm , Umesh V. Waghmare , Momoji Kubo

We report the phase diagram of (Ba1-xCax)(Zr0.1Ti0.9)O3 solid solution. It is found that substitution of smaller Ca ions for Ba ions can slightly increase the cubic-tetragonal(T) para-ferroelectric phase transition temperature and strongly…

Materials Science · Physics 2013-10-08 Desheng Fu , Yuto Kamai , Naonori Sakamoto , Naoki Wakiya , Hisao Suzuki , Mitsuru Itoh

In a previous work a model was proposed for the phase transitions of crystals with localized magnetic moments which at low temperature have a "conical" arrangement that at higher T transforms into a more symmetrical structure (depending on…

Statistical Mechanics · Physics 2009-11-13 Vittorio Massidda

An atomistic approach is used to investigate finite-temperature properties of ferroelectric nanodots that are embedded in a polarizable medium. Different phases are predicted, depending on the ferroelectric strengths of the material…

Materials Science · Physics 2009-11-11 S. Prosandeev , L. Bellaiche

Ferroelectric solid solutions usually exhibit giant dielectric response and high piezoelectricity in the vicinity of the morphotropic phase boundary (MPB), where the structural phase transitions between the rhombohedral and the tetragonal…

Materials Science · Physics 2024-07-02 Yubai Shi , Yifan Shan , Hongyu Wu , Zhicheng Zhong , Ri He , Run-Wei Li

We analyze a system of polar molecules in a one-dimensional optical lattice. By controlling the internal structure of the polar molecules with static electric and microwave fields, we demonstrate the appearance of a quantum phase transition…

Quantum Gases · Physics 2015-09-02 Markus Klinsmann , David Peter , Hans Peter Büchler
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