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The theory of the electron relaxation in metals excited by an ultrashort optical pump is developed on the basis of the solution of the linearized kinetic equation. The kinetic equation includes both the electron-electron and the…

Strongly Correlated Electrons · Physics 2014-03-06 V. V. Baranov , V. V. Kabanov

We compute the transient dynamics of phonons in contact with high energy "hot" charge carriers in 12 polar and non-polar semiconductors, using a first-principles Boltzmann transport framework. For most materials, we find that the decay in…

Mesoscale and Nanoscale Physics · Physics 2017-10-03 Sridhar Sadasivam , Maria K. Y. Chan , Pierre Darancet

We develop a theory to describe energy relaxation of photo-excited carriers in low-temperature ordered states with band gap opening and formulate carrier relaxation time $\tau$ near and below transition temperature $T_{\mathrm{c}}$ by…

Mesoscale and Nanoscale Physics · Physics 2012-02-14 Shota Ono , Hiroyuki Shima , Yasunori Toda

The femtosecond optical pump-probe technique was used to study dynamics of photoexcited electrons and coherent optical phonons in transition metals Zn and Cd as a function of temperature and excitation level. The optical response in time…

Strongly Correlated Electrons · Physics 2009-11-11 Muneaki Hase , Kunie Ishioka , Jure Demsar , Kiminori Ushida , Masahiro Kitajima

The transport relaxation rate 1/tau of a two-dimensional electron gas due to scattering by thermally excited surface acoustic phonons is calculated. The temperature dependence of 1/tau is found to be linear in T for high temperatures, but…

Mesoscale and Nanoscale Physics · Physics 2008-02-03 Andreas Knaebchen

Both theoretical and experimental results for the dynamics of photoexcited electrons at surfaces of Cu and the ferromagnetic transition metals Fe, Co, and Ni are presented. A model for the dynamics of excited electrons is developed, which…

Condensed Matter · Physics 2009-10-31 R. Knorren , K. H. Bennemann , R. Burgermeister , M. Aeschlimann

The ab-initio theory of charge transport in semiconductors typically employs the lowest-order perturbation theory in which electrons interact with one phonon (1ph). This theory is accepted to be adequate to explain the low-field mobility of…

Materials Science · Physics 2023-02-08 Benjamin Hatanpää , Alexander Y. Choi , Peishi S. Cheng , Austin J. Minnich

A semiempirical theory for the excitation and subsequent relaxation of nonthermal electrons is described. The theory, which is applicable to ultrafast-laser excited metals, is based on the Boltzmann transport equation for the carrier…

Materials Science · Physics 2023-07-12 D. M. Riffe , Richard B. Wilson

The first-principle theory of electron dephasing by disorder-induced two state fluctuators is developed. There exist two mechanisms of dephasing. First, dephasing occurs due to direct transitions between the defect levels caused by…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 V. V. Afonin , J. Bergli , Y. M. Galperin , V. L. Gurevich , V. I. Kozub

We analyze current-voltage characteristics taken on Au-doped indium-oxide films. By fitting a scaling function to the data, we extract the electron-phonon scattering rate as function of temperature, which yields a quadratic dependence of…

Disordered Systems and Neural Networks · Physics 2009-11-11 Roy Ceder , Oded Agam , Zvi Ovadyahu

The effect of the electron temperature on both the light absorption and the scattering by metal nanoparticles (MNs) with excitation of the surface plasmon electron vibrations is studied in the framework of the kinetic theory. The formulae…

Mesoscale and Nanoscale Physics · Physics 2013-11-25 N. I. Grigorchuk

We study the electron and phonon thermalization in simple metals excited by a laser pulse. The thermalization is investigated numerically by solving the Boltzmann transport equation taking into account all the relevant scattering mechanism:…

Materials Science · Physics 2018-02-28 Shota Ono

Photoexcited hot carriers in solids can drive processes, such as photocatalytic reactions on the surface, beyond those available in thermal equilibrium. Hot-electron-mediated reaction pathways are limited by the thermalization of the…

Materials Science · Physics 2026-04-13 Christopher Seibel , Tobias Held , Markus Uehlein , Baerbel Rethfeld

We report on a theoretical investigation concerning the polaronic effect on the transport properties of a charge carrier in the one-dimensional molecular chain. Our technique is based on the Feynman's path integral approach. Analytical…

Mesoscale and Nanoscale Physics · Physics 2015-12-10 Sikarin Yoo-Kong , Watchara Liewrian

Understanding the dynamics of photoexcited carriers is essential for advancing photoelectronic device design. Photon absorption generates electron-hole pairs, and subsequent scatterings can induce ultrafast thermalization within a…

Materials Science · Physics 2025-01-14 Zhuoqun Wen , Haiyu Zhu , Wenhao Liu , Zhi Wang , Wen Xiong , Xingzhan Wei

We theoretically study the relaxation of electron orbital states of a double quantum dot system due to two-phonon processes. In particular, we calculate how the relaxation rates depend on the separation distance between the quantum dots,…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 V. N. Stavrou , Xuedong Hu

Recent theoretical developments in the studies of two-photon exchange effects in elastic electron-proton scattering are reviewed. Two-photon exchange mechanism is considered a likely source of discrepancy between polarized and unpolarized…

High Energy Physics - Phenomenology · Physics 2017-08-23 Andrei V. Afanasev

The two-temperature model (2TM) introduced by Kaganov, Lifshitz, and Tanatarov is widely used to describe the energy relaxation in the electron-phonon system of a metallic film. At the same time, the accuracy of the description of the…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 A. I. Bezuglyj , V. A. Shklovskij

Using electrical transport experiments and shot noise thermometry, we find strong evidence that "supercollision" scattering processes by flexural modes are the dominant electron-phonon energy transfer mechanism in high-quality, suspended…

Mesoscale and Nanoscale Physics · Physics 2015-11-02 Antti Laitinen , Mika Oksanen , Aurélien Fay , Daniel Cox , Matti Tomi , Pauli Virtanen , Pertti Hakonen

We report the lattice dynamics of transition metal thin films by using the ultrafast electron diffraction. We observe a suppression of the diffraction intensity in a few picosecond after the photoexcitation, which is directly interpreted as…

Materials Science · Physics 2016-01-19 A. Nakamura , T. Shimojima , M. Nakano , Y. Iwasa , K. Ishizaka
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