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We study numerically the crystallization of a hard-sphere mixture with 8\% polydispersity. Although often used as a model glass former, for small system sizes we observe crystallization in molecular dynamics simulations. This opens the…

Soft Condensed Matter · Physics 2016-09-05 Matteo Campo , Thomas Speck

This paper summarizes the properties of strongly correlating liquids, i.e., liquids with strong correlations between virial and potential energy equilibrium fluctuations at constant volume. We proceed to focus on the experimental…

Soft Condensed Matter · Physics 2015-03-14 Ulf R. Pedersen , Nicoletta Gnan , Nicholas P. Bailey , Thomas B. Schröder , Jeppe C. Dyre

We derive a general closed expression for the local pressure exerted onto the corrugated walls of a channel confining a fluid medium. When the fluid medium is at equilibrium the local pressure is a functional of the shape of the walls. It…

Soft Condensed Matter · Physics 2018-02-07 Paolo Malgaretti , Markus Bier

X-ray photon correlation is used to probe the slow dynamics of the glass-former B2O3 across the glass transition. In the undercooled liquid phase the decay times of the measured correlation functions are consistent with visible light…

Disordered Systems and Neural Networks · Physics 2019-07-03 Giovanna Pintori , Giacomo Baldi , Beatrice Ruta , Giulio Monaco

We examine the structural relaxation of glassy materials at finite temperatures, considering the effect of activated rearrangements and long-range elastic interactions. Our three-dimensional mesoscopic relaxation model shows how the…

Soft Condensed Matter · Physics 2023-12-20 Gieberth Rodriguez-Lopez , Kirsten Martens , Ezequiel E. Ferrero

The time evolution of the pore size distributions and mechanical properties of amorphous solids at constant pressure is studied using molecular dynamics simulations. The porous glasses were initially prepared at constant volume conditions…

Soft Condensed Matter · Physics 2018-10-22 Nikolai V. Priezjev , Maxim A. Makeev

We derive exact results for stress correlations in near-crystalline systems in two and three dimensions. We study energy minimized configurations of particles interacting through Harmonic as well as Lennard-Jones potentials, for varying…

Soft Condensed Matter · Physics 2023-12-18 Roshan Maharana , Kabir Ramola

The effects of randomly pinning particles in a model glass-forming fluid are studied, with a focus on the dynamically heterogeneous relaxation in the presence of pinning. We show how four-point dynamical correlations can be analysed in real…

Statistical Mechanics · Physics 2013-10-30 Robert L. Jack , Christopher J. Fullerton

The role that non-local short-range correlation plays at metal surfaces is investigated by analyzing the correlation surface energy into contributions from dynamical density fluctuations of various two-dimensional wave vectors. Although…

Materials Science · Physics 2009-11-07 J. M. Pitarke , J. P. Perdew

We show numeric evidence that, at low enough temperatures, the potential energy density of a glass-forming liquid fluctuates over length scales much larger than the interaction range. We focus on the behavior of translationally invariant…

Soft Condensed Matter · Physics 2009-04-21 L. A. Fernandez , V. Martin-Mayor , P. Verrocchio

Cooperative events requiring anomalously large fluctuations are a defining characteristic for the onset of glassy relaxation across many materials. The importance of such intermittent events has been noted in systems as diverse as…

Soft Condensed Matter · Physics 2021-12-10 Stefan Boettcher , Paula A. Gago , Paolo Sibani

We report experimental measurements of particle dynamics in a colloidal glass in order to understand the dynamical heterogeneities associated with the cooperative motion of the particles in the glassy regime. We study the local and global…

Soft Condensed Matter · Physics 2007-05-23 P. Wang , C. Song , H. A. Makse

Dynamic heterogeneity in glass-formers has been related to their static structure using the concept of dynamic propensity. We re-examine this relationship by analyzing dynamical fluctuations in two atomistic glass-formers and two…

Statistical Mechanics · Physics 2009-08-25 Ludovic Berthier , Robert L. Jack

We theoretically investigate the temperature dependence of the reversible structural relaxation time and diffusion constant of metallic glasses under pressure. The compression not only changes the glassy dynamics, but also generates a…

Materials Science · Physics 2021-05-28 Nguyen K. Ngan , Anh D. Phan , Alessio Zaccone

We study the response of a spin glass system with respect to the rescaling of its interaction random variables and investigate numerically the behaviour of the correlation functions with respect to the volume. While for a ferromagnet the…

Disordered Systems and Neural Networks · Physics 2009-11-13 Pierluigi Contucci , Francesco Unguendoli , Cecilia Vernia

Two atoms in an ultracold gas are correlated at short inter-atomic distances due to threshold effects where the potential energy of their interaction dominates the kinetic energy. The correlations manifest themselves in a distinct nodal…

Atomic Physics · Physics 2011-04-15 Christiane P. Koch , Ronnie Kosloff

The nature of defects in amorphous materials, analogous to vacancies and dislocations in crystals, remains elusive. Here we explore their nature in a three-dimensional microscopic model glass-former which describes granular, colloidal,…

Soft Condensed Matter · Physics 2019-11-13 Camille Scalliet , Ludovic Berthier , Francesco Zamponi

Simulations are used to examine the microscopic origins of strain hardening in polymer glasses. While stress-strain curves for a wide range of temperature can be fit to the functional form predicted by entropic network models, many other…

Soft Condensed Matter · Physics 2009-11-13 Robert S. Hoy , Mark O. Robbins

We discuss a novel approach, the point-to-set correlation functions, that allows to determine relevant static and dynamic length scales in glass-forming liquids. We find that static length scales increase monotonically when the temperature…

Disordered Systems and Neural Networks · Physics 2013-07-04 Walter Kob , Sandalo Roldan-Vargas , Ludovic Berthier

The competing effects of slow structural relaxations (aging) and deformation at constant strain rate on the shear yield stress $\tau^y$ of simple model glasses are examined using molecular simulations. At long times, aging leads to a…

Soft Condensed Matter · Physics 2009-11-11 Joerg Rottler , Mark O. Robbins
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