Related papers: First-principles calculations of hot-electron life…
We report a first-principles description of inelastic lifetimes of excited electrons in real Cu and Al, which we compute, within the GW approximation of many-body theory, from the knowledge of the self-energy of the excited quasiparticle.…
Electron dynamics in the bulk and at the surface of solid materials are well known to play a key role in a variety of physical and chemical phenomena. In this article we describe the main aspects of the interaction of low-energy electrons…
We report extensive first-principles calculations of the inelastic lifetime of low-energy electrons in the noble metals Cu, Ag, and Au. The quasiparticle self-energy is computed with full inclusion of exchange and correlation (xc) effects,…
During the last decade, significant progress has been achieved in the rapidly growing field of the dynamics of {\it hot} carriers in metals. Here we present an overview of the recent achievements in the theoretical understanding of electron…
The inelastic quasiparticle lifetime due to the electron-electron interaction (out-scattering time in the kinetic equation formalism) is calculated for finite metallic diffusive systems (quantum dots) in the whole range of parameters. Both…
We have investigated the hole dynamics at copper surfaces by high-resolution angle-resolved photoemission experiments and many-body quasiparticle GW calculations. Large deviations from a free-electron-like picture are observed both in the…
We calculate the inelastic lifetime of an electron quasiparticle due to Coulomb interactions in an electron liquid at low (or zero) temperature in two and three spatial dimensions. The contribution of "exchange" processes is calculated…
First principles calculations of the damping rates (inverse inelastic lifetimes) of low energy quasiparticles in bulk Pb are presented. Damping rates are obtained both for excited electrons and holes with energies up to 8 eV on a set of k…
We calculate the lifetime of low-energy electronic excitations in a two-dimensional quantum dot near a metallic gate. We find different behaviors depending on the relative values of the dot size, the dot-gate distance and the Thomas-Fermi…
The quasiparticle decays due to electron-electron interaction in silicon are studied by means of first-principles all-electron GW approximation. The spectral function as well as the dominant relaxation mechanisms giving rise to the finite…
Inelastic lifetime of an electron quasiparticle in an electron liquid due to electron-electron interaction evaluated in previous work is calculated in an alternative way. Both the contributions of the "direct" and "exchange" processes are…
A theoretical many-body analysis is presented of the electron-electron inelastic lifetimes of Shockley electrons and holes at the (111) surface of Cu. For a description of the decay of Shockley states both below and above the Fermi level,…
We present first-principles calculations of electron-electron scattering rates of low-energy electrons in Au. Our full band-structure calculations indicate that a major contribution from occupied d states participating in the screening of…
We present a detailed analysis of hole dynamics in noble metals (Cu and Au), by means of first-principles many-body calculations. While holes in a free-electron gas are known to live shorter than electrons with the same excitation energy,…
We report ab initio calculation of quasiparticle lifetimes in graphite, as determined from the imaginary part of the self-energy operator within the GW aproximation. The inverse lifetime in the energy range from 0.5 to 3.5 eV above the…
We calculate Coulomb scattering lifetimes of electrons in two-subband quantum wires and in double-layer quantum wells by obtaining the quasiparticle self-energy within the framework of the random-phase approximation for the dynamical…
In this work, the Coulomb scattering lifetimes of electrons in two coupled quantum wires have been studied by calculating the quasiparticle self-energy within a multisubband model of quasi-one-dimensional (Q1D) electron system. We consider…
We investigate the decoherence of the electron wavepacket in purely ballistic one-dimensional systems described through the Luttinger liquid (LL). At a finite temperature $T$ and long times $t$, we show that the electron Green's function…
We analytically study the inelastic lifetime of quasiparticles due to particle-particle interactions in a three-dimensional Fermi liquid approaching a density-wave instability. Using the G$_0$W approximation, we find that the softening of…
We use time-resolved thermometry to monitor the decay of nonequilibrium quasiparticles in superconducting Al in the temperature range from $0.3\,$K to $1.2\,$K. The quasiparticle lifetime at higher temperatures ($T>0.7\,$K) agrees well with…