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We present a detailed comparison of the structural predictions of the effective many-body Brenner potential with those of ab-initio studies for known reconstructions of diamond (100) and (111) surfaces. These results suggest high…

Materials Science · Physics 2015-06-24 A. V. Petukhov , A. Fasolino

The evolution of the diamond (111) surface as it undergoes reconstruction and subsequent graphene formation is investigated with angle-resolved photoemission spectroscopy, low energy electron diffraction, and complementary density…

The optical properties of the 2$\times$1 reconstruction of the diamond (111) surface are investigated. The electronic structure and optical properties of the surface are studied using a microscopic tight-binding approach. We calculate the…

Condensed Matter · Physics 2009-10-28 Cecilia Noguez , Sergio E. Ulloa

We have carried out an ab-initio study of $\alpha$-Sn (111), with the aim of predicting and understanding its structure, reconstructions, and electronic states. We consider a variety of structural possibilities, and optimize them by moving…

Condensed Matter · Physics 2009-10-28 Zhong-Yi Lu , Guido L. Chiarotti , S. Scandolo , E. Tosatti

Boron-doped diamond (BDD) has attracted much attentions in semi-/super-conductor physics and electrochemistry, where the surface structures play crucial roles. Herein, we systematically re-examined the probable surface reconstructions of…

Materials Science · Physics 2020-10-30 Le The Anh , Shota Iizuka , Yasuaki Einaga , Celine Catalan , Yousoo Kim , Yoshitaka Tateyama

We have theoretically studied the stability and reconstruction of (111) surfaces of Au, Pt, and Cu. We have calculated the surface energy, surface stress, interatomic force constants, and other relevant quantities by ab initio electronic…

Condensed Matter · Physics 2009-11-10 Z. Crljen , P. Lazic , D. Sokcevic , R. Brako

An interatomic potential for the diamond and graphite phases of carbon has been created using a neural-network (NN) representation of the ab initio potential energy surface. The NN potential combines the accuracy of a first-principle…

Materials Science · Physics 2010-04-21 Rustam Z. Khaliullin , Hagai Eshet , Thomas D. Kühne , Jörg Behler , Michele Parrinello

The electronic structure and dielectric properties of the diamond, body centered cubic diamond (bc8), and hexagonal diamond (lonsdaleite) phases of carbon are computed using density functional theory and many-body perturbation theory with…

Materials Science · Physics 2022-03-14 Kushal Ramakrishna , Jan Vorberger

Unpaired electronic spins at diamond surfaces are ubiquitous and can lead to excess magnetic noise. They have been observed in several studies to date, but their exact chemical nature is still unknown. We propose a simple model to explain…

Quantum Physics · Physics 2023-06-26 Jyh-Pin Chou , Péter Udvarhelyi , Nathalie P. de Leon , Adam Gali

We computed the inter-layer bonding properties of graphite using an ab-initio many body theory. We carried out variational and diffusion quantum Monte Carlo calculations and found an equilibrium inter-layer binding energy in good agreement…

Materials Science · Physics 2015-05-14 Leonardo Spanu , Sandro Sorella , Giulia Galli

We use recent theoretical advances to develop a new functional form for interatomic forces in bulk silicon. The theoretical results underlying the model include a novel analysis of elastic properties for the diamond and graphitic structures…

Materials Science · Physics 2016-08-31 Martin Z. Bazant , Efthimios Kaxiras , J. F. Justo

We have studied the reconstruction of Pt(111) theoretically using a two-dimensional Frenkel-Kontorova model for which all parameters have been obtained from ab initio calculations. We find that the unreconstructed surface lies right at the…

Materials Science · Physics 2007-05-23 Shobhana Narasimhan , Raghani Pushpa

Monte Carlo simulations, supplemented by ab initio calculations, shed light into the energetics and thermodynamic stability of nanostructured amorphous carbon. The interaction of the embedded nanocrystals with the host amorphous matrix is…

Materials Science · Physics 2009-11-11 Maria G. Fyta , Pantelis C. Kelires

Graphite and diamond are two well-known allotropes of carbon with distinct physical properties due to different atomic connectivity. Graphite has a layered structure in which the honeycomb carbon sheets can easily glide, while atoms in…

Materials Science · Physics 2025-06-06 Sheng-cai Zhu , Xiao-zhi Yan , Jin Liu , Artem R. Oganov , Qiang Zhu

The interaction between graphene and copper (111) surface have been investigated using the molecular dynamics simulations. We have shown that it is possible to fit Lennard-Jones potential leading to the correct values of the binding energy…

Mesoscale and Nanoscale Physics · Physics 2016-11-03 A. V. Sidorenkov , S. V. Kolesnikov , A. M. Saletsky

Single-layer diamond or diamane is substituted by N atoms assisting the diamond-like structure to be stabilize without any passivation. One fourth of N substitution in diamane, vertically stacking as NCCC, is found to be stable by surface…

Materials Science · Physics 2020-08-19 T. Pakornchote , A. Ektarawong , W. Busayaporn , U. Pinsook , T. Bovornratanaraks

We propose a new structural model for the Si(111)-(5x2)-Au reconstruction. The model incorporates a new experimental value of 0.6 monolayer for the coverage of gold atoms, equivalent to six gold atoms per 5x2 cell. Five main theoretical…

Materials Science · Physics 2015-05-14 Steven C. Erwin , Ingo Barke , F. J. Himpsel

Mechanically induced degradation of diamond, as occurs during polishing, is studied using total--energy pseudopotential calculations. The strong asymmetry in the rate of polishing between different directions on the diamond (110) surface is…

Materials Science · Physics 2009-10-31 M. R. Jarvis , R. Perez , F. M. van Bouwelen , M. C. Payne

We use molecular simulation to construct equilibrium phase diagrams for two recently introduced model materials with isotropic, soft-repulsive pair interactions designed to favor diamond and simple cubic lattice ground states, respectively,…

Materials Science · Physics 2013-10-15 Avni Jain , Jeffrey R. Errington , Thomas M. Truskett

Graphyne (GY) and graphdiyne (GDY)-based materials represent an intriguing class of two-dimensional (2D) carbon-rich networks with tunable structures and properties surpassing those of graphene. However, the challenge of fabricating…

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