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An algebraic model in terms of a local harmonic boson realization was recently proposed to study molecular vibrational spectra [Zhong-Qi Ma et al., Phys. Rev. A 53, 2173 (1996)]. Because of the local nature of the bosons the model has to…

Chemical Physics · Physics 2009-10-30 R. Lemus , F. Perez-Bernal , A. Frank , R. Bijker , J. M. Arias

The stretching and bending vibrational spectrum and the intensities of infrared transitions in a tetrahedral molecule are studied in two boson-realization models, where the interactions between stretching and bending vibrations are…

Chemical Physics · Physics 2009-10-31 Xi-Wen Hou , Mi Xie , Shi-Hai Dong , Zhong-Qi Ma

We discuss a symmetry-adapted algebraic (or vibron) model for molecular spectroscopy. The model is formulated in terms of tensor operators under the molecular point group. In this way, we have identified interactions that are absent in…

Chemical Physics · Physics 2017-11-02 R. Bijker , A. Frank , R. Lemus , J. M. Arias , F. Perez-Bernal

The stretching and bending vibrations of methane are studied in the framework of a symmetry-adapted algebraic model. The model is based on the realization of the one-dimensional Morse potential in terms of a $U(2)$ algebra. For the 44…

Chemical Physics · Physics 2017-11-03 R. Lemus , F. Perez-Bernal , A. Frank , R. Bijker , J. M. Arias

We apply the Anharmonic Oscillator Symmetry Model to the description of vibrational excitations in ${\cal D}_{3h}$ and ${\cal T}_d$ molecules. A systematic procedure can be used to establish the relation between the algebraic and…

chem-ph · Physics 2008-02-03 A. Frank , R. Lemus , R. Bijker , F. Perez-Bernal , J. M. Arias

The stretching and bending vibrations of methane are studied in a local anharmonic model of molecular vibrations. The use of symmetry-adapted operators reduces the eigenvalue problem to block diagonal form. For the 44 observed energies we…

chem-ph · Physics 2008-02-03 R. Lemus , F. Perez-Bernal , A. Frank , R. Bijker , J. M. Arias

Both the stretch and bend vibrational spectrum and the intensity of infrared transitions in a tetrahedral molecule are studied in a U(2) algebraic model, where the spurious states in the model Hamiltonian and the wavefunctions are exactly…

Chemical Physics · Physics 2009-10-31 Xi-Wen Hou , Shi-Hai Dong , Mi Xie , Zhong-Qi Ma

We introduce the Anharmonic Oscillator Symmetry Model to describe vibrational excitations in molecular systems exhibiting high degree of symmetry. A systematic procedure is proposed to establish the relation between the algebraic and…

chem-ph · Physics 2009-10-28 A. Frank , R. Lemus , R. Bijker , F. Perez-Bernal , J. M. Arias

We exploit the rich algebraic structure of the interacting boson model to explain the notion of partial dynamical symmetry (PDS), and present a procedure for constructing Hamiltonians with this property. We demonstrate the relevance of PDS…

Nuclear Theory · Physics 2013-04-16 A. Leviatan

Two identical non-interacting fermions in a three-dimensional harmonic oscillator well are bosonised exactly according to a recently developed general algebraic scheme. Rotational invariance is taken into account within the scheme for the…

Quantum Physics · Physics 2020-03-05 Katarina Rožman , D. K. Sunko

Interacting dipole ($p$) bosons along with scalar ($s$) bosons, based on the ideas drawn from the interacting boson model of atomic nuclei, led to the development of the vibron model based on $U(4)$ spectrum generating algebra for diatomic…

Chemical Physics · Physics 2021-07-15 V. K. B. Kota

Full-dimensional (12D) vibrational states of the methanol molecule (CH$_3$OH) have been computed using the GENIUSH-Smolyak approach and the potential energy surface from Qu and Bowman (2013). All vibrational energies are converged better…

Chemical Physics · Physics 2024-09-05 Ayaki Sunaga , Gustavo Avila , Edit Matyus

Methyl benzoate (MB) is studied as a model compound for the development of new IR pulse schemes with possible applicability to biomolecules. Anharmonic vibrational modes of MB are calculated on different level (MP2, SCS, CCSD(T) with…

Chemical Physics · Physics 2014-01-03 Kiran Sankar Maiti , Christoph Scheurer

We propose a novel formulation of the Interacting Boson Model (IBM) for rotational nuclei with axially-symmetric strong deformation. The intrinsic structure represented by the potential energy surface (PES) of a given multi-nucleon system…

Nuclear Theory · Physics 2011-07-19 Kosuke Nomura , Takaharu Otsuka , Noritaka Shimizu , Lu Guo

Accurately simulating molecular vibronic spectra remains computationally challenging due to the exponential scaling of required calculations. Here, we show that employing the linear coupling model within the gaussian boson sampling…

Quantum Physics · Physics 2025-08-07 I. Konyshev , R. Pradip , O. Page , C. Ünlüer , R. T. Nasibullin , V. V. Rybkin , W. Pernice , S. Ferrari

The vibrational excitations of ozone, including both bending and stretching vibrations, are studied in the framework of a symmetry-adapted algebraic approach. This method is based on the isomorphism between the U(2) algebra and the…

chem-ph · Physics 2015-06-24 F. Perez-Bernal , J. M. Arias , A. Frank , R. Lemus , R. Bijker

We apply a symmetry-adapted algebraic model to the vibrational excitations in D_3h and T_d molecules. A systematic procedure is used to establish the relation between the algebraic and configuration space formulations. In this way we have…

Chemical Physics · Physics 2017-11-02 A. Frank , R. Lemus , R. Bijker , F. Perez-Bernal , J. M. Arias

The present status of the mapped interacting boson model studies on nuclear structure is reviewed. With the assumption that the nuclear surface deformation induced by the multi-nucleon dynamics is simulated by bosonic degrees of freedom,…

Nuclear Theory · Physics 2025-06-19 Kosuke Nomura

The interacting boson model is extended to describe the spectroscopy of superdeformed bands. Microscopic structure of the model in the second minimum is discussed and superdeformed bosons are introduced as the new building blocks. Solutions…

Nuclear Theory · Physics 2009-09-25 S. Kuyucak , M. Honma , T. Otsuka

We give a new reduction of a general diatomic molecular Hamiltonian, without modifying it near the collision set of nuclei. The resulting effective Hamiltonian is the sum of a smooth semiclassical pseudodifferential operator (the…

Mathematical Physics · Physics 2015-06-26 André Martinez , Vania Sordoni
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