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Using empirical scheme, atomic structure of a new exotic class of silicon nanoclusters was elaborated upon the central icosahedral core (Si-IC) and pentagonal petals (Si-PP) growing from Si-IC vertexes. It was shown that Si-IC/Si-PP…

Materials Science · Physics 2007-09-17 Pavel V. Avramov , Leonid A. Chernozatonskii , Pavel B. Sorokin , Mark S. Gordon

Si(331)-(12x1) is the only confirmed planar silicon surface with a stable reconstruction located between (111) and (110). We have optimized the annealing sequence and are able to obtain almost defect free, atomically precise surface areas…

We study the optimal packing of short, hard spherocylinders confined to lie tangential to a spherical surface, using simulated annealing and molecular dynamics simulations. For clusters of up to twelve particles, we map out the changes in…

Soft Condensed Matter · Physics 2016-05-25 Frank Smallenburg , Hartmut Löwen

We present a density-functional (DF) study of structures of Si cage clusters that encapsulate metal atoms. As a prototypical example, the case of WSi$_{n}$ clusters is shown. To obtain the low-energy clusters in efficient and unbiased ways,…

Materials Science · Physics 2007-05-23 Takehide Miyazaki , Hidefumi Hiura , Toshihiko Kanayama

We have located the global minimum for all lead clusters with up to 160 atoms using a glue potential to model the interatomic interactions. The lowest-energy structures are not face-centred cubic as suggested previously. Rather, for N<40…

Condensed Matter · Physics 2007-05-23 Jonathan P. K. Doye , Shaun C. Hendy

The fully halogenated or hydrogenated B12X12 (X = H, F, Cl, Br and I) clusters are confirmed to be icosahedral. On the other hand, the bare B12 cluster is shown to have a planar structure. A previous study showed that a transformation from…

Chemical Physics · Physics 2017-10-12 Liang-Fa Gong , Wei Li , Edison Osorio , Xin-Min Wu , Thomas Heine , Lei Liu

According to microscopic calculations with antisymmetrized molecular dynamics, we studied cluster features in stable and unstable nuclei. A variety of structure was found in stable and unstable nuclei in the $p$-shell and $sd$-shell…

Nuclear Theory · Physics 2015-06-26 Y. Kanada-En'yo , M. Kimura , H. Horiuchi

On basis of the first principle calculation we show that a crystalline structure of silicon, as a novel allotrope with nanotubular holes along two perpendicular directions, is stable. The calculations on geometrical and electronic…

Materials Science · Physics 2011-06-16 Chi-Pui Tang , Jie Cao , Shi-Jie Xiong

A new approach to solve quasicrystalline atomic structures in 3-dimensional (3D) real space is presented: The atomic pair distribution function (PDF) of face centred icosahedral Ho9Mg26Zn65 [a(6D) = 2x5.18(3)A was obtained from in-house…

Materials Science · Physics 2007-05-23 S. Bruehne , R. Sterzel , E. Uhrig , C. Gross , W. Assmus

Density-functional theory is used to study the geometric and electronic structure of cationic Si16^+ clusters with a Ti, V or Cr dopant atom. Through unbiased global geometry optimization based on the basin-hopping approach we confirm that…

Materials Science · Physics 2015-05-27 Dennis Palagin , Matthias Gramzow , Karsten Reuter

We have carried out extensive density functional calculations for series of sodium clusters $Na$$_{N}$ ranging from $N$=10 to 147 and have obtained $\approx$ 13000 distinct isomers. We unravel a number of striking features of the growth…

Materials Science · Physics 2016-09-28 Seyed Mohammad Ghazi , Shahab Zorriasatein , D. G. Kanhere

The nanostructure of hydrogenated amorphous silicon (a Si:H) is studied by a combination of small-angle X-ray (SAXS) and neutron scattering (SANS) with a spatial resolution of 0.8 nm. The a-Si:H materials were deposited using a range of…

Materials Science · Physics 2020-11-04 Eike Gericke , Jimmy Melskens , Robert Wendt , Markus Wollgarten , Armin Hoell , Klaus Lips

We show that new silicon crystalline phases, observed in the experiment with the laser-induced microexplosions inside silicon crystals (Rapp et al. // Nat. Commun. 6, 7555 (2015)), are all superstructures of a disordered high-symmetry phase…

Soft Condensed Matter · Physics 2020-06-15 Vladimir E. Dmitrienko , Viacheslav A. Chizhikov

Packing transitions in the lowest energy structures of Li clusters as a function of size have been identified via simulated annealing. For N>21, the large $p$ character of Li leads to unexpected ionic structures. At N~25, a packing pattern…

chem-ph · Physics 2009-10-22 Ming Wen Sung , Ryoichi Kawai , John H. Weare

We have used molecular dynamics simulations to construct a microcanonical caloric curve for a 1415-atom Ni icosahedron. Prior to melting the Ni cluster exhibits static solid-liquid phase coexistence. Initially a partial icosahedral…

Materials Science · Physics 2007-05-23 D. Schebarchov , S. C. Hendy

Silicon self-assembly at step edges in the initial stage of homoepitaxial growth on a vicinal Si(111) surface is studied by scanning tunneling microscopy (STM). The resulting atomic structures change dramatically from a parallel array of…

Materials Science · Physics 2007-05-23 T. Sekiguchi , S. Yoshida , K. M. Itoh

A family of unusually stable boron cages was identified and examined using first-principles local density functional method. The structure of the fullerenes is similar to that of the B12 icosahedron and consists of six crossing…

Materials Science · Physics 2021-09-21 Nevill Gonzalez Szwacki

We show that the optimal packing of hard spheres in an infinitely long cylinder yields structures characterised by a screw symmetry. Each packing can be assembled by stacking a basic unit cell ad infinitum along the length of the cylinder…

Soft Condensed Matter · Physics 2014-03-05 A. Mughal

We have examined the hypothesis by Bijker and Iachello who asserted that 12C has an internal structure with three alpha particles arranged in a triangular shape, leading to the formation of the ground rotational band consisting of 0+, 2+,…

Nuclear Theory · Physics 2024-04-02 Masaaki Kimura , Yasutaka Taniguchi

The theoretical formalism of the local density approximation (LDA) to density functional theory (DFT) has been used to study the electronic and geometric structures of SimCn (1<=m, n<=4;n<=m) clusters. An all electron 6-311++G** basis set…

Atomic and Molecular Clusters · Physics 2007-05-23 Prachi Pradhan , Asok K. Ray