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Monte Carlo methods were used to calculate heat capacities as functions of temperature for classical atomic clusters of aggregate sizes $25 \leq N \leq 60$ that were bound by pairwise Lennard-Jones potentials. The parallel tempering method…

Chemical Physics · Physics 2009-11-07 D. D. Frantz

Heat capacity curves as functions of temperature were calculated using Monte Carlo methods for the series of Ar_{13-n}Kr_n clusters (0 <= n <= 13). The clusters were modeled classically using pairwise additive Lennard-Jones potentials.…

chem-ph · Physics 2009-10-28 Don D. Frantz

Heat capacity curves as functions of temperature were calculated using Monte Carlo methods for the series of Ne_(13-n)Ar_n clusters (0 <= n <= 13). The clusters were modeled classically using pairwise additive Lennard-Jones potentials. The…

Chemical Physics · Physics 2009-10-30 Don D. Frantz

Detailed studies of the thermodynamic properties of selected binary Lennard-Jones clusters of the type X_{13-n}Y_n (where n=1,2,3) are presented. The total energy, heat capacity and first derivative of the heat capacity as a function of…

Statistical Mechanics · Physics 2009-11-10 Dubravko Sabo , Cristian Predescu , J. D. Doll , David L. Freeman

The thermal behaviour of the 309-atom Lennard-Jones cluster, whose structure is a complete Mackay icosahedron, has been studied by parallel tempering Monte Carlo simulations. Surprisingly for a magic number cluster, the heat capacity shows…

Other Condensed Matter · Physics 2007-05-23 Eva G. Noya , Jonathan P. K. Doye

The thermodynamic and structural properties of (NH$_4$Cl)$_n$ clusters, n=3-10 are studied. Using the method of simulated annealing, the geometries of several isomers for each cluster size are examined. Jump-walking Monte Carlo simulations…

chem-ph · Physics 2009-10-28 Alexander Matro , David L. Freeman , Robert Q. Topper

Single impurity effect on the melting process of magic number Lennard-Jones, rare gas, clusters of up to 309 atoms is studied on the basis of Parallel Tempering Monte Carlo simulations in the canonical ensemble. A decrease on the melting…

Atomic and Molecular Clusters · Physics 2015-05-19 Nicolás Quesada , Gloria E. Moyano

The heat capacity and isomer distributions of the 38 atom Lennard-Jones cluster have been calculated in the canonical ensemble using parallel tempering Monte Carlo methods. A distinct region of temperature is identified that corresponds to…

Chemical Physics · Physics 2009-11-06 J. P. Neirotti , F. Calvo , David L. Freeman , J. D. Doll

We present a new theoretical framework for modelling the cluster growing process. Starting from the initial tetrahedral cluster configuration, adding new atoms to the system and absorbing its energy at each step, we find cluster growing…

Atomic and Molecular Clusters · Physics 2007-05-23 A. Koshelev , A. Shutovich , Il. A. Solov'yov , A. V. Solov'yov , W. Greiner

The interplay between magic number stabilities and superfluidity of small para-hydrogen clusters with sizes $N = 5$ to 40 and temperatures $0.5 K \leq T \leq 4.5 $K is explored with classical and quantum Path Integral Monte Carlo…

Computational Physics · Physics 2010-09-14 S. A. Khairallah , M. B. Sevryuk , D. M. Ceperley , J. P. Toennies

We present a new theoretical framework for modelling the fusion process of Lennard-Jones (LJ) clusters. Starting from the initial tetrahedral cluster configuration, adding new atoms to the system and absorbing its energy at each step, we…

Atomic and Molecular Clusters · Physics 2009-09-29 Ilia A. Solovyov , Andrey V. Solovyov , Walter Greiner

Heat capacities of Na_N, N = 13, 20, 55, 135, 142, and 147, clusters have been investigated using a many-body Gupta potential and microcanonical molecular dynamics simulations. Negative heat capacities around the cluster melting-like…

Atomic and Molecular Clusters · Physics 2016-09-08 Juan A. Reyes-Nava , Ignacio L. Garzon , Karo Michaelian

We study phase transitions of small two dimensional Lennard Jones drops via microcanonical molecular dynamics in a broad energy range. We found that the caloric curve can be extended to high energies to comprehend high evaporation rates and…

Nuclear Theory · Physics 2008-11-26 A. Strachan , C. O. Dorso

The thermodynamic properties of 59 TeF6 clusters that undergo temperature-driven phase transitions have been calculated with a canonical J-walking Monte Carlo technique. A parallel code for simulations has been developed and optimized on…

Computational Physics · Physics 2009-11-07 R. Radev , A. Proykova

The melting of Al clusters in the size range 49 <= N <= 62 has been studied using two model interatomic potentials. The results for the two models are significantly different. The glue potential exhibits a smooth relatively featureless heat…

Other Condensed Matter · Physics 2007-05-23 Eva G. Noya , Jonathan P. K. Doye , Florent Calvo

A few experiments have already detected the presence of icosahedral superclusters in undercooled liquids, confirming a possible homogeneous nucleation of such entities as suggested by Franck. These superclusters survive in melts above the…

Materials Science · Physics 2014-07-29 Robert Felix Tournier

Simulations based on experimental data obtained from multifragmenting quasi-fused nuclei produced in central $^{129}$Xe + $^{nat}$Sn collisions have been used to deduce event by event freeze-out properties in the thermal excitation energy…

The equilibrium properties of classical LJ_38 versus quantum Ne_38 Lennard-Jones clusters are investigated. The quantum simulations use both the Path-Integral Monte-Carlo (PIMC) and the recently developed Variational-Gaussian-Wavepacket…

Chemical Physics · Physics 2009-11-11 Cristian Predescu , Pavel A. Frantsuzov , Vladimir A. Mandelshtam

The heat capacity of iron isotopes is calculated within the interacting shell model using the complete $(pf+0g_{9/2})$-shell. We identify a signature of the pairing transition in the heat capacity that is correlated with the suppression of…

Nuclear Theory · Physics 2009-11-06 S. Liu , Y. Alhassid

The excitation energies of parahydrogen clusters have been systematically calculated by the diffusion Monte Carlo technique in steps of one molecule from 3 to 40 molecules. These clusters possess a very rich spectra, with angular momentum…

Atomic and Molecular Clusters · Physics 2009-11-13 R. Guardiola , J. Navarro
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