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The mid-infrared spectra of large PAHs ranging from C54H18 to C130H28 are determined computationally using Density Functional Theory. Trends in the band positions and intensities as a function of PAH size, charge and geometry are discussed.…

Astrophysics · Physics 2012-08-27 Charles W. Bauschlicher, , Els Peeters , Louis J. Allamandola

The search for large polycyclic aromatic hydrocarbons (PAHs) with over 100 carbon atoms is crucial to resolving the origin of unidentified infrared emission (UIE) bands. These bands are commonly observed in nebulae and the interstellar…

Astrophysics of Galaxies · Physics 2025-08-22 Yi Shao , Yong Zhang , Xu-Jia Ouyang , Chuan-Peng Zhang

The PAH family of organic compounds (polycyclic aromatic hydrocarbons), involved in several fields of chemistry, has received particular attention in astrochemistry, where their vibrational spectroscopy, thermodynamic, dynamic, and…

Chemical Physics · Physics 2017-06-13 Georges Trinquier , Aude Simon , Mathias Rapacioli , Florent Xavier Gadéa

Ultraviolet (UV) processing in the insterstellar medium (ISM) induces the dehydrogenation of hydrocarbons. Aliphatics, including alkanes, are present in different interstellar environments, being prevalently formed in evolved stars; thus,…

Polycyclic aromatic hydrocarbons (PAHs) are responsible for a variety of near- and mid-infrared spectral features in Galactic and extragalactic sources. A feature at 1.05 $\mu$m arising from electronic transitions in PAH cations is…

Astrophysics of Galaxies · Physics 2026-03-25 Dennis Lee , Brandon S. Hensley , Tzu-Ching Chang , Olivier Doré

We model the production of OH+, H2O+, and H3O+ in interstellar clouds, using a steady state photodissociation region code that treats the freeze-out of gas species, grain surface chemistry, and desorption of ices from grains. The code…

Astrophysics of Galaxies · Physics 2015-06-05 David Hollenbach , M. J. Kaufman , D. Neufeld , M. Wolfire , J. R. Goicoechea

The pre-transitional disk around the Herbig Ae star HD 169142 shows a complex structure of possible ongoing planet formation in dust thermal emission from the near infrared (IR) to millimeter wavelength range. Also, a distinct set of broad…

Solar and Stellar Astrophysics · Physics 2016-02-17 Ji Yeon Seok , Aigen Li

A novel theoretical method is developed to study the polycyclic aromatic hydrocarbon - diffuse interstellar band (PAH-DIB) hypothesis. In this method, a computer program is used to enumerate all PAH molecules with up to a specific number of…

Astrophysics · Physics 2007-05-23 Xiaofeng Tan

Hydrocarbons are ubiquitous in the interstellar medium, but their formation is still not well understood, depending on the physical environment they are found in. M8 is host to one of the brightest HII regions and PDRs in our galaxy. Using…

Astrophysics of Galaxies · Physics 2019-06-12 M. Tiwari , K. M. Menten , F. Wyrowski , J. P. Pérez-Beaupuits , M. -Y. Lee , W. -J. Kim

Deuterium (D) was exclusively generated in the Big Bang and the standard Big Bang Nucleosynthesis (BBN) model predicts a primordial abundance of D/H~26ppm. As the Galaxy evolves, D/H gradually decreases because of astration. The Galactic…

Astrophysics of Galaxies · Physics 2023-08-09 X. J. Yang , Aigen Li

The interstellar medium (ISM) consists of a diversity of structures across a range of spatial scales, intimately tied to galactic evolution. In this work, Fourier analysis is used to characterize the spatial structures of dust and…

Astrophysics of Galaxies · Physics 2025-04-04 Charlie Lind-Thomsen , Albert Sneppen , Charles L. Steinhardt

We extend the non-equilibrium model for the chemical and thermal evolution of diffuse interstellar gas presented in Richings et al. (2014) to account for shielding from the UV radiation field. We attenuate the photochemical rates by dust…

Astrophysics of Galaxies · Physics 2015-06-19 Alexander J. Richings , Joop Schaye , Benjamin D. Oppenheimer

Star formation depends critically on cooling mechanisms in the interstellar medium (ISM); however, thermal properties of gas in galaxies at the peak epoch of star formation (z ~ 2) remain poorly understood. A limiting factor in…

We present $Spitzer$/IRS mid-infrared spectral maps of the Galactic star-forming region M17 as well as IRSF/SIRIUS Br$\gamma$ and Nobeyama 45-m/FOREST $^{13}$CO ($J$=1--0) maps. The spectra show prominent features due to polycyclic aromatic…

Infrared (IR) emission spectra are calculated for dust composed of mixtures of amorphous silicate and graphitic grains, including varying amounts of polycyclic aromatic hydrocarbon (PAH) particles. The models are constrained to reproduce…

Astrophysics · Physics 2008-11-26 B. T. Draine , Aigen Li

Polycyclic Aromatic Hydrocarbons (PAHs) are believed to be the small-size tail of the interstellar carbonaceous dust grain population. Their vibrational emission is the most widely accepted source of the aromatic near-infrared features, and…

Astrophysics of Galaxies · Physics 2015-08-21 Yacine Ali-Haïmoud , Laura Pérez , Ronald Maddalena , Anish Roshi

Only 8% of the protoplanetary discs orbiting a T Tauri star show emission features of polycyclic aromatic hydrocarbons (PAHs). As PAHs are strong absorbers of UV radiation, they contribute to the heating of the discs photosphere, shielding…

Earth and Planetary Astrophysics · Physics 2025-10-01 K. Lange , C. Dominik , A. G. G. M. Tielens

Polycyclic Aromatic Hydrocarbon (PAH) molecules have been long proposed to be a major carrier of 'Unidentified Infrared' (UIR) emission bands that have been observed ubiquitously in various astrophysical environments. These molecules can…

Astrophysics of Galaxies · Physics 2017-11-28 Mridusmita Buragohain , Amit Pathak , Peter Sarre , Takashi Onaka , Itsuki Sakon