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Accurate representation of the molecular electrostatic potential, which is often expanded in distributed multipole moments, is crucial for an efficient evaluation of intermolecular interactions. Here we introduce a machine learning model…

Chemical Physics · Physics 2017-10-09 Tristan Bereau , Denis Andrienko , O. Anatole von Lilienfeld

The simulation of strongly correlated electron systems remains a formidable challenge. Certain experimentally relevant dynamical response functions are especially difficult to calculate, due to issues of finite-size effects and the ill…

Strongly Correlated Electrons · Physics 2026-03-25 Petar Brinić , Hugo U. R. Strand , Jakša Vučičević

The fundamental non-Hermitian nature of the forms of coupled-cluster (CC) theory widely used in quantum chemistry has usually been viewed as a negative, but the present letter shows how this can be used to advantage. Specifically, the…

The $\Delta \text{NO}$ method for static correlation is combined with second-order M{\o}ller-Plesset perturbation theory (MP2) and coupled-cluster singles and doubles (CCSD) to account for dynamic correlation. The MP2 and CCSD expressions…

Chemical Physics · Physics 2020-06-05 Joshua W. Hollett , Pierre-François Loos

The curse of dimensionality (COD) limits the current state-of-the-art {\it ab initio} propagation methods for non-relativistic quantum mechanics to relatively few particles. For stationary structure calculations, the coupled-cluster (CC)…

Quantum Physics · Physics 2015-06-03 Simen Kvaal

Coupled cluster theory is the method of choice for weakly correlated systems. But in the strongly correlated regime, it faces a symmetry dilemma, where it either completely fails to describe the system, or has to artificially break certain…

Chemical Physics · Physics 2020-05-14 Yiheng Qiu , Thomas M. Henderson , Jinmo Zhao , Gustavo E. Scuseria

We present a deep machine learning (ML) approach to constraining cosmological parameters with multi-wavelength observations of galaxy clusters. The ML approach has two components: an encoder that builds a compressed representation of each…

Instrumentation and Methods for Astrophysics · Physics 2022-02-16 Michelle Ntampaka , Alexey Vikhlinin

The structure of single-$\Lambda$ hypernuclei is studied using the chiral hyperon-nucleon potentials derived at leading order (LO) and next-to-leading order (NLO) by the J\"{u}lich--Bonn--Munich group. Results for the separation energies of…

Nuclear Theory · Physics 2020-03-18 Johann Haidenbauer , Isaac Vidana

We develop a coupled-cluster theory for bosonic mixtures of binary species in external traps, providing a promising theoretical approach to demonstrate highly accurately the many-body physics of mixtures of Bose-Einstein condensates. The…

Quantum Gases · Physics 2024-02-01 Anal Bhowmik , Ofir E. Alon

The mass function of cluster-size halos and their redshift distribution are computed for 12 distinct accelerating cosmological scenarios and confronted to the predictions of the conventional flat $\Lambda$CDM model. The comparison with…

Cosmology and Nongalactic Astrophysics · Physics 2010-10-27 S. Basilakos , M. Plionis , J. A. S. Lima

Machine-learned potentials (MLPs) trained on ab initio data combine the computational efficiency of classical interatomic potentials with the accuracy and generality of the first-principles method used in the creation of the respective…

Chemical Physics · Physics 2024-08-07 Leonid Kahle , Benoit Minisini , Tai Bui , Jeremy T. First , Corneliu Buda , Thomas Goldman , Erich Wimmer

A new, three-dimensional, shock capturing, TVD hydrodynamic code is utilized to determine the distribution of hot gas in a CDM$+\Lambda$ model universe. This open model succeeds in matching local observations of clusters in contrast to the…

Astrophysics · Physics 2009-10-22 Renyue Cen , Jeremiah P. Ostriker

We introduce affordable computational strategies for calculating orbital and pair-orbital energies in atomic and molecular systems. Our methods are based on the pair Coupled Cluster Doubles (pCCD) ansatz and its orbital-optimized variant.…

Chemical Physics · Physics 2025-02-06 Seyedehdelaram Jahani , Somayeh Ahmadkhani , Katharina Boguslawski , Paweł Tecmer

The quark-meson coupling (QMC) model, which has been successfully used to describe the properties of both infinite nuclear matter and finite nuclei, is applied to a systematic study of $\Lambda, \Sigma$ and $\Xi$ hypernuclei. Assumptions…

Nuclear Theory · Physics 2010-02-17 K. Tsushima , K. Saito , J. Haidenbauer , A. W. Thomas

The orbital M1 collective mode predicted for deformed clusters in a schematic model is studied in a self-consistent random-phase-approximation approach which fully exploits the shell structure of the clusters. The microscopic mechanism of…

Atomic and Molecular Clusters · Physics 2009-10-31 V. O. Nesterenko , W. Kleinig , F. F. de Souza Cruz , N. Lo Iudice

An externally corrected coupled cluster (CC) method, where an adaptive configuration interaction (ACI) wave function provides the external cluster amplitudes, named ACI-CC, is presented. By exploiting the connection between configuration…

Chemical Physics · Physics 2023-09-27 Gustavo J. R. Aroeira , Madeline M. Davis , Justin M. Turney , Henry F. Schaefer

Condensed Matter Physics (CMP) seeks to understand the microscopic interactions of matter at the quantum and atomistic levels, and describes how these interactions result in both mesoscopic and macroscopic properties. CMP overlaps with many…

Computational Physics · Physics 2020-11-12 Edwin A. Bedolla-Montiel , Luis Carlos Padierna , Ramón Castañeda-Priego

We present our latest study of Lambda-Nucleon (LN) interaction by using lattice QCD, following up on our report at LATTICE 2008. We have calculated not only the scattering lengths but also the central and tensor potentials, which are…

High Energy Physics - Lattice · Physics 2010-11-05 H. Nemura , for HAL QCD , PACS-CS Collaboration

Coupled-cluster (CC) theory and Green's function many-body perturbation theory (MBPT) have long evolved as distinct yet complementary frameworks for describing electronic correlation. While CC methods employ exponential wavefunction…

Amorphous materials are coming within reach of realistic computer simulations, but new approaches are needed to fully understand their intricate atomic structures. Here, we show how machine-learning (ML)-based techniques can give new,…