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Ground State Energy Estimation (GSEE) is a central problem in quantum chemistry and condensed matter physics, demanding efficient algorithms to solve complex electronic structure calculations. This work introduces a structured benchmarking…

Multivariate quantum signal processing (M-QSP) has recently been shown to be applicable for non-Hermitian Hamiltonian simulation, opening several problems regarding the optimization landscape, angle-finding, and constant-factor analysis. We…

Quantum Physics · Physics 2026-05-14 Joshua M. Courtney

Surface energy is a fundamental property of materials and is particularly important in describing nanomaterials where atoms or molecules at the surface constitute a large fraction of the material. Traditionally, surface energy is considered…

Mesoscale and Nanoscale Physics · Physics 2024-04-24 Jason J. Calvin , Amanda S. Brewer , Michelle F. Crook , Tierni M. Kaufman , A. Paul Alivisatos

The Coupled Cluster (CC) method is used to compute the electronic correlation energy in atoms and molecules and often leads to highly accurate results. However, due to its single-reference nature, standard CC in its projected form fails to…

The practical application of quantum technologies to chemical problems faces significant challenges, particularly in the treatment of realistic basis sets and the accurate inclusion of electron correlation effects. A direct approach to…

Towards the scalable realization of a quantum computer, a quantum charge-coupled device (QCCD) based on ion shuttling has been considered a promising approach. However, the processes of detaching an ion from an array, reintegrating it, and…

Quantum Physics · Physics 2026-01-26 Ting Hsu , Wen-Han Png , Kuan-Ting Lin , Ming-Shien Chang , Guin-Dar Lin

Many organizations that vitally depend on computation for their competitive advantage are keen to exploit the expected performance of quantum computers (QCs) as soon as quantum advantage is achieved. The best approach to deliver hardware…

In this paper, a novel quantum classical hybrid framework is proposed that synergizes quantum with Classical Reinforcement Learning. By leveraging the inherent parallelism of quantum computing, the proposed approach generates robust Q…

Machine Learning · Computer Science 2025-05-21 Sahil Tomar , Shamshe Alam , Sandeep Kumar , Amit Mathur

The integration of high-penetration renewable energy introduces significant stochasticity and non-convexity into power system dispatching, challenging the computational limits of classical optimization. While Variational Quantum Algorithms…

Quantum Physics · Physics 2026-01-27 Fu Zhang , Yuming Zhao

We extend our recently-developed heat-bath configuration interaction (HCI) algorithm, and our semistochastic algorithm for performing multireference perturbation theory, to the calculation of excited-state wavefunctions and energies. We…

Strongly Correlated Electrons · Physics 2017-11-22 Adam A. Holmes , C. J. Umrigar , Sandeep Sharma

Quantum machine learning (QML) has great potential for the analysis of chemical datasets. However, conventional quantum data-encoding schemes, such as fingerprint encoding, are generally unfeasible for the accurate representation of…

Quantum Physics · Physics 2025-11-18 Choy Boy , Edoardo Altamura , Dilhan Manawadu , Ivano Tavernelli , Stefano Mensa , David J. Wales

The quantum-selected configuration interaction (QSCI) method is a promising approach for large-scale quantum chemical calculations on currently available quantum hardware. However, its naive implementation lacks size consistency, which is…

Quantum Physics · Physics 2026-01-06 Kenji Sugisaki

With the advent of exascale computing, effective load balancing in massively parallel software applications is critically important for leveraging the full potential of high performance computing systems. Load balancing is the distribution…

Quantum Physics · Physics 2025-01-30 Omer Rathore , Alastair Basden , Nicholas Chancellor , Halim Kusumaatmaja

With the birth of Noisy Intermediate Scale Quantum (NISQ) devices and the verification of "quantum supremacy" in random number sampling and boson sampling, more and more fields hope to use quantum computers to solve specific problems, such…

Programming Languages · Computer Science 2023-01-02 Menghan Dou , Tianrui Zou , Yuan Fang , Jing Wang , Dongyi Zhao , Lei Yu , Boying Chen , Wenbo Guo , Ye Li , Zhaoyun Chen , Guoping Guo

Signal processing stands as a pillar of classical computation and modern information technology, applicable to both analog and digital signals. Recently, advancements in quantum information science have suggested that quantum signal…

Signal Processing · Electrical Eng. & Systems 2025-10-27 Yuan Liu , John M. Martyn , Jasmine Sinanan-Singh , Kevin C. Smith , Steven M. Girvin , Isaac L. Chuang

Recent advancements in quantum algorithms have reached a state where we can consider how to capitalize on quantum and classical computational resources to accelerate molecular resonance state identification. Here we identify molecular…

Quantum Physics · Physics 2026-03-26 Jingcheng Dai , Atharva Vidwans , Eric H. Wan , Alexander X. Miller , Micheline B. Soley

Quantum chemistry is one of the most promising applications of quantum computers in the near future. For noisy intermediate-scale quantum devices, the quantum-classical hybrid framework based on the variational quantum eigensolver (VQE) has…

We explore the simulation of conical intersections (CIs) on quantum devices, setting the groundwork for potential applications in nonadiabatic quantum dynamics within molecular systems. The intersecting potential energy surfaces of…

Quantum Physics · Physics 2024-01-30 Yuchen Wang , David A. Mazziotti

The ability to perform ab initio molecular dynamics simulations using potential energies calculated on quantum computers would allow virtually exact dynamics for chemical and biochemical systems, with substantial impacts on the fields of…

A state-of-the-art method that combines a quantum computational algorithm and machine learning, so-called quantum machine learning, can be a powerful approach for solving quantum many-body problems. However, the research scope in the field…

Computational Physics · Physics 2023-04-04 Shu Kanno , Tomofumi Tada