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Slow relaxation and heterogeneous dynamics are characteristic features of glasses. The presence of glassy dynamics in nonequilibrium systems, such as active matter, is of significant interest due to its implications for living systems and…

Soft Condensed Matter · Physics 2024-06-27 Antina Ghosh , Sayan Maity , Vijayakumar Chikkadi

The relationship between spatially heterogeneous dynamics (SHD) and jamming is studied in a glass-forming binary Lennard-Jones system via molecular dynamics simulations. It has been suggested that the probability distribution of…

Disordered Systems and Neural Networks · Physics 2007-05-23 Naida Lacevic , Sharon C. Glotzer

We report results from the molecular dynamics simulations of a binary colloidal mixture subjected to an external potential barrier along one of the spatial directions at low volume fraction, {\phi} = 0.2. The variations in the asymmetry of…

Soft Condensed Matter · Physics 2021-01-26 Jalim Singh , Mahammad Mustakim , A. V. Anil Kumar

We study the nature of the glass transition by cooling model atomistic glass formers at constant rate from a temperature above the onset of glassy dynamics to $T=0$. Motivated by the East model, a kinetically constrained lattice model with…

Statistical Mechanics · Physics 2018-04-16 Alexander Hudson , Kranthi K. Mandadapu

Which phenomenon slows down the dynamics in super-cooled liquids and turns them into glasses is a long-standing question of condensed-matter. Most popular theories posit that as the temperature decreases, many events must occur in a…

Soft Condensed Matter · Physics 2024-03-22 Massimo Pica Ciamarra , Wencheng Ji , Matthieu Wyart

The effect of temperature on friction and slip at the liquid-solid interface has attracted attention over the last twenty years, both numerically and experimentally. However, the role of temperature on slip close to the glass transition has…

Soft Condensed Matter · Physics 2023-02-22 Suzanne Lafon , Alexis Chennevière , Frédéric Restagno , Samy Merabia , Laurent Joly

While deeply supercooled liquids exhibit divergent viscosity and increasingly heterogeneous dynamics as the temperature drops, their structure shows only seemingly marginal changes. Understanding the nature of relaxation processes in this…

Materials Science · Physics 2022-11-03 Matthias Lerbinger , Armand Barbot , Damien Vandembroucq , Sylvain Patinet

We investigate a binary Lennard-Jones mixture with molecular dynamics simulations. We consider first a system cooled linearly in time with the cooling rate gamma. By varying gamma over almost four decades we study the influence of the…

Statistical Mechanics · Physics 2015-06-25 K. Vollmayr-Lee , W. Kob , K. Binder , A. Zippelius

The dynamics of supercooled liquids slow down and become increasingly heterogeneous as they are cooled. Recently, local structural variables identified using machine learning, such as "softness", have emerged as predictors of local…

Soft Condensed Matter · Physics 2024-06-11 Sean A. Ridout , Andrea J. Liu

We use computer simulations to study the microscopic dynamics of an athermal assembly of soft particles near the fluid-to-solid, jamming transition. Borrowing tools developed to study dynamic heterogeneity near glass transitions, we…

Materials Science · Physics 2010-06-24 Claus Heussinger , Ludovic Berthier , Jean-Louis Barrat

We present simulation results for the dynamics of a schematic model based on the frustration-limited domain picture of glass-forming liquids. These results are compared with approximate theoretical predictions analogous to those commonly…

Statistical Mechanics · Physics 2009-11-10 Phillip L. Geissler , David R. Reichman

We present computer simulation results on the dynamic propensity [as defined by Widmer- Cooper, Harrowell, and Fynewever, Phys. Rev. Lett. 93, 135701 (2004)] in a Kob-Andersen binary Lennard-Jones liquid system consisting of 8788 particles.…

Materials Science · Physics 2011-05-26 M. Shajahan G. Razul , Gurpreet S. Matharoo , Peter H. Poole

The physical behavior of glass-forming liquids presents complex features of both dynamic and thermodynamic nature. Some studies indicate the presence of thermodynamic anomalies and of crossovers in the dynamic properties, but their origin…

Statistical Mechanics · Physics 2018-06-08 Daniele Coslovich , Misaki Ozawa , Walter Kob

Analysis of temperature dependence of structural relaxation time in supercooled liquids revealed a qualitatively distinct feature - a sharp, cusp-like maxumum in the second derivative of its logarithm. It suggests that the super-Arrhenius…

Soft Condensed Matter · Physics 2016-01-20 V. N. Novikov , A. P. Sokolov

Using molecular dynamics simulation, we calculate the distribution of atomic jum ps in Cu$_{33}$Zr$_{67}$ in the liquid and glassy states. In both states the distribution of jump lengths can be described by a temperature independent…

Disordered Systems and Neural Networks · Physics 2009-11-11 M. Kluge , H. R. Schober

We report a molecular dynamics simulation of a supercooled simple monatomic glass-forming liquid. It is found that the onset of the supercooled regime results in formation of distinct domains of slow diffusion which are confined to the…

Disordered Systems and Neural Networks · Physics 2009-11-07 Mikhail Dzugutov , Sergei I. Simdyankin , Fredrik H. M. Zetterling

In this work we investigate the transient solidification of a Lennard-Jones liquid using non-equilibrium molecular dynamics simulations and continuum heat transfer theory. The simulations are performed in slab-shaped boxes, where a cold…

Mesoscale and Nanoscale Physics · Physics 2020-10-26 Francesc Font , William Micou , Fernando Bresme

We propose a dynamic structure of coupled dynamic molecular strings for supercooled small polar molecule liquids and accordingly we obtain the Hamiltonian of the rotational degrees of freedom of the system. From the Hamiltonian, the…

Disordered Systems and Neural Networks · Physics 2009-11-10 Y. N. Huang , C. J. Wang , E. Riande

Using molecular dynamics simulations, we study a spherically-symmetric ``two-scale'' Jagla potential with both repulsive and attractive ramps. This potential displays a liquid-liquid phase transition with a positively sloped coexistence…

Soft Condensed Matter · Physics 2009-11-11 Limei Xu , Isaac Ehrenberg , Sergey V. Buldyrev , H. Eugene Stanley

We analyze dynamics of quantum supercooled liquids in terms of tagged particle dynamics. Unlike the classical case, uncertainty in the position of a particle in quantum liquid leads to qualitative changes. We demonstrate these effects in…

Statistical Mechanics · Physics 2025-01-14 Ankita Das , Gopika Krishnan , Eran Rabani , Upendra Harbola