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Halide perovskites constitute a chemically-diverse class of crystals with great promise as photovoltaic absorber materials, featuring band gaps between about 1 and 3.5 eV depending on composition. Their diversity calls for a general…

Materials Science · Physics 2019-10-23 Linn Leppert , Tonatiuh Rangel , Jeffrey B. Neaton

Surface states are ubiquitous to semiconductors and significantly impact the physical properties and consequently the performance of optoelectronic devices. Moreover, surface effects are strongly amplified in lower dimensional systems such…

Optical cavities provide a powerful means to engineer light-matter hybrid states by coupling confined electromagnetic fields with matter excitations. Achieving in situ control of the coupling strength is essential for investigating how such…

Modern communication and sensing technologies rely on connecting the optical domain with the microwave domain. Terahertz technologies, spanning increased frequencies from 100 GHz to 10 THz, are critical for providing larger bandwidths and…

Semiconductor heterostructures that combine components with different dimensionality provide an interesting way to manipulate the physical properties of the resulting material. Two-dimensional lead halide perovskites crystallize as flat…

Generating photon pairs via spontaneous parametric down-conversion (SPDC) in nonlinear crystals is important for a wide range of quantum optics experiments with spectral properties such as their bandwidths often being a crucial concern.…

Quantum Physics · Physics 2020-06-18 Aron Vanselow , Paul Kaufmann , Helen M. Chrzanowski , Sven Ramelow

Lead halide perovskites have emerged as platforms for exciton-polaritonic studies at room temperature thanks to their excellent photoluminescence efficiency and synthetic versatility. In this work we find proof of strong exciton-photon…

Materials Science · Physics 2024-05-07 Maximilian Black , Mehdi Asadi , Parsa Darman , Finja Schillmöller , Sara Darbari , Nahid Talebi

Photoinduced non-thermal phase transitions are new paradigms of exotic non-equilibrium physics of strongly correlated materials. An ultrashort optical pulse can drive the system to a new order through complex microscopic interactions that…

The amplified spontaneous emission from a superluminescent diode was frequency doubled in a periodically poled lithium niobate waveguide crystal. The temporally incoherent radiation of such a superluminescent diode is characterized by a…

Optics · Physics 2017-04-05 Henning Kurzke , Jan Kiethe , Axel Heuer , Andreas Jechow

Previous theoretical calculations show azetidinium has the right radial size to form a 3D perovskite with lead halides [1], and has been shown to impart, as the A-site cation of ABX3 unit, beneficial properties to ferroelectric perovskites…

The parametric amplification of ultrashort (femtosecond) laser pulses in crystals with a regular domain structure (RDS) of the 5%Mg : PPLN type has been investigated theoretically. The focus was on the formation of a signal pulse in…

Optics · Physics 2024-05-07 O. I. Sobirov , D. B. Yusupov , N. A. Akbarova , U. K. Sapaev

Bridging the "terahertz (THz) gap" relies upon synthesizing arbitrary waveforms in the THz domain enabling applications that require both narrow band sources for sensing and few-cycle drives for classical and quantum objects. However,…

Four wave mixing (FWM) is an important way to generate supercontinuum and frequency combs in the mid-infrared band. Here, we obtain simultaneous synthetic FWM in the visible and mid-infrared bands by cascading quadratic nonlinear processes…

We demonstrated broadband highly efficient optical nonlinear processes in on-chip integrated lithium niobate (LN) microdisk resonators. The Q factors of the micro-resonators fabricated by femtosecond laser writing and chemo-mechanical…

The recent development of devices based on novel nonlinear materials like chalcogenides (ChGs), silicon (Si) and other semi-conductors has revolutionized the field of nonlinear photonics [1,2,3]. Among the nonlinear effects observed in…

Optics · Physics 2015-06-04 Raja Ahmad , Martin Rochette

Excursions far from their equilibrium structures can bring crystalline solids through collective transformations including transitions into new phases that may be transient or long-lived. Direct spectroscopic observation of…

Optical nonlinearities are crucial for advanced photonic technologies since they allow photons to be managed by photons. Exciton-polaritons resulting from strong light-matter coupling are hybrid in nature: they combine small mass and high…

Quantum wells made of two-dimensional organic-inorganic hybrid perovskites (2D-PKs) offer a high degree of flexibility in tailoring optoelectronic properties through carrier confinement and functional interlayers. Compared to their 3D…

Organic-inorganic halide perovskites, especially methylammonium lead halide, have recently led to a remarkable breakthrough in photovoltaic devices. However, due to the environmental and stability concerns of the heavy metal, lead, in these…

Materials Science · Physics 2015-09-29 Shijing Sun , Satoshi Tominaka , Jung-Hoon Lee , Fei Xie , Paul D. Bristowe , Anthony K. Cheetham

We report on the observation of broadband (40 THz) bright twin beams through high-gain parametric down-conversion in an aperiodically poled lithium niobate crystal. The output photon number is shown to scale exponentially with the pump…