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Magnetoelectric multiferroics are highly sought after for applications in low-power electronics and for advancing fundamental research, including axion insulators and dark matter detection. However, achieving a combination of ferroic spin…

Materials Science · Physics 2024-12-02 Libor Šmejkal

Hexagonal LuFe2O4 is a promising charge-order (CO) driven multiferroic material with high charge and spin ordering temperatures. The coexisting charge and spin orders on Fe3+/Fe2+ sites result in novel magnetoelectric behaviors, but the…

The relationship between magnetic order and ferroelectric properties has been investigated for MnWO$_4$ with long-wavelength magnetic structure. Spontaneous electric polarization is observed in an elliptical spiral spin phase. The…

Strongly Correlated Electrons · Physics 2009-11-11 K. Taniguchi , N. Abe , T. Takenobu , Y. Iwasa , T. Arima

Density-functional calculations are carried out to investigate incommensurate magnetic structures and ferroelectric polarization in newly discovered multiferroic material MnI$_2$. The exchange interactions among local moments on Mn are…

Strongly Correlated Electrons · Physics 2013-05-30 Xianxin Wu , Yingxiang Cai , Qing Xie , Hongming Weng , Heng Fan , Jiangping Hu

In this paper we predict that the magnetoelectric response of two-dimensional (2D) antiferromagnets is determined by the topology of the ground state. This topological magnetoelectric response, encoded in the spin magnetoelectric…

Strongly Correlated Electrons · Physics 2025-12-08 Jörn W. F. Venderbos , Paola Gentile , Carmine Ortix

The ferroelectric polarization of triangular-lattice antiferromagnets induced by helical spin-spiral order is not explained by any existing model of magnetic-order-driven ferroelectricity. We resolve this problem by developing a general…

Strongly Correlated Electrons · Physics 2011-10-11 H. J. Xiang , E. J. Kan , Y. Zhang , M. -H. Whangbo , X. G. Gong

We present a computational search for spin spiral ground states in two-dimensional transition metal halides that are experimentally known as van der Waals bonded bulk materials. Such spin spirals break the rotational symmetry of the lattice…

Materials Science · Physics 2023-06-14 Joachim Sødequist , Thomas Olsen

We address a systematic microscopic theory of spin-dependent electric polarization in 3d oxides starting with a generic three-site two-hole cluster. A perturbation scheme realistic for 3d oxides is applied which implies the quenching of…

Strongly Correlated Electrons · Physics 2009-11-13 A. S. Moskvin , S. -L. Drechsler

Magnetic toroidal order features a loop-like arrangement of magnetic dipole moments, thus breaking both spatial inversion (P) and time-reversal (T) symmetries while preserving their combined PT sym-metry. This PT symmetry enables a linear…

Materials Science · Physics 2025-09-18 Chuangtang Wang , Xiaoyu Guo , Zixin Zhai , Meixin Cheng , Sang-Wook Cheong , Adam W. Tsen , Bing Lv , Liuyan Zhao

A pseudospin model for description of the influence of the electric field, confined to the plane of sublattice polarization, on the two-dimensional squaric acid antiferroelectrics is developed. The system behavior is analyzed in terms of…

Materials Science · Physics 2021-06-09 A. P. Moina

Using a joint approach of density functional theory and model calculations, we demonstrate that a prototypical charge ordered half-doped manganite, La$_{1/2}$Ca$_{1/2}$MnO$_3$ is multiferroic. The combination of a peculiar charge-orbital…

Materials Science · Physics 2010-07-15 Gianluca Giovannetti , Sanjeev Kumar , Jeroen van den Brink , Silvia Picozzi

Two-dimensional (2D) semiconducting multiferroics that can effectively couple magnetic and polarization (P) orders have great interest for both fundamental research and technological applications in nanoscale, which are, however, rare in…

Materials Science · Physics 2023-03-01 Baishun Yang , Bin Shao , Jianfeng Wang , ChiYung Yam , Shengbai Zhang , Bing Huang

It is shown that interlayer spin-singlet Cooper pairing is induced by magnetic interactions in a metallic antiferromagnet of stacked conductive layers in which each layer is ferromagnetically polarized and they order antiferromagnetically…

Superconductivity · Physics 2007-05-23 Hiroshi Shimahara

By performing accurate ab-initio density functional theory calculations, we study the role of $4f$ electrons in stabilizing the magnetic-field-induced ferroelectric state of DyFeO$_{3}$. We confirm that the ferroelectric polarization is…

Materials Science · Physics 2015-05-14 Alessandro Stroppa , Martijn Marsman , Georg Kresse , Silvia Picozzi

The noncollinear cycloidal magnetic order breaks the inversion symmetry in CaMn$_{7}$O$_{12}$, generating one of the largest spin-orbit driven ferroelectric polarizations measured to date. In this Letter, the microscopic origin of the…

Materials Science · Physics 2018-01-17 Jin Soo Lim , Diomedes Saldana-Greco , Andrew M. Rappe

The realization of multiferroic altermagnets featuring giant intrinsic spin splitting, hold great promise for next-generation spintronics. In this work, based on the recently proposed concept of spin-antiferroelectric (spin-AFE), we…

Materials Science · Physics 2026-04-14 Zesen Fu , Aolin Li , Wenzhe Zhou , Fangping Ouyang , Fawei Zheng , Yugui Yao

The two-dimensional (2D) multiferroic materials have widespread of application prospects in facilitating the integration and miniaturization of nanodevices. However, it is rarely coupling between the magnetic, ferroelectric, and ferrovalley…

Materials Science · Physics 2024-03-05 Wei Xun , Chao Wu , Hanbo Sun , Weixi Zhang , Yin-Zhong Wu , Ping Li

The bulk photovoltaic effect that is intimately associated with crystalline symmetry has been extensively studied in various nonmagnetic materials, especially ferroelectrics with a switchable electric polarization. In order to further…

Materials Science · Physics 2022-12-28 Chunmei Zhang , Ping Guo , Jian Zhou

We report the observation of a magnetic polarization of the O\,$2p$-states in YMn$_2$O$_5$ through the use of soft X-ray resonant scattering at the oxygen $K$-edge. Remarkably, we find that the temperature dependence of the integrated…

Strongly Correlated Electrons · Physics 2015-03-19 S. Partzsch , S. B. Wilkins , J. P. Hill , E. Schierle , E. Weschke , D. Souptel , B. Büchner , J. Geck

Magnetoelectric (ME) materials displaying strong magnetically induced polarization have attracted considerable interest due to their potential applications in spintronics and various fast electrically controlled magnetic devices.…