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In a collinear magnet, the predominant magnetic moments are collectively aligned along a specific spatial orientation, and this alignment may yield intriguing phenomena such as spin orientation driven polarization. It is well known that…

Materials Science · Physics 2025-12-12 Yixun Zhang , Longju Yu , Yizhou Tong , Ying Sun , Xu Li , Hong Jian Zhao , Yanming Ma

Type-II multiferroics, where spin order induces ferroelectricity, exhibit strong magnetoelectric coupling. However, for the typical 2D type-II multiferroic NiI$_2$, the underlying magnetoelectric mechanism remains unclear. Here, applying…

Spin-driven multiferroics exhibit strong magnetoelectric coupling, with notable polarization changes under a magnetic field, but these effects are usually limited to high-Z magnetic insulators with low electronic polarization. In this work,…

Materials Science · Physics 2024-12-31 Ranquan Cao , Ruizhi Dong , Ruixiang Fei , Yugui Yao

The coupling between magnetic order and ferroelectricity has been under intense investigation in a wide range of transition-metal oxides. The strongest coupling is obtained in so-called magnetically-induced multiferroics where…

Materials Science · Physics 2015-05-13 V. S. Zapf , M. Kenzelmann , F. Wolff-Fabris , F. Balakirev , Y. Chen

We introduce a microscopic model for collinear multiferroics capable to reproduce, as a consequence of magnetic frustration and easy-axis anisotropy, the so-called "uudd" (or antiphase) magnetic ordering observed in several type II…

Strongly Correlated Electrons · Physics 2021-04-21 D. C. Cabra , A. O. Dobry , C. J. Gazza , G. L. Rossini

Altermagnetism, an emergent magnetic phase featuring compensated collinear magnetic moments and momentum-dependent spin splittings, has recently garnered widespread interest. A critical issue concerns whether the unconventional spin…

Materials Science · Physics 2026-05-28 Wen-Ti Guo , Junqi Xu , Yurong Yang , Haijun Zhang , Huaiqiang Wang

There has been tremendous research activity in the field of magneto-electric (ME) multiferroics after Kimura et al. [1] showed that antiferromagnetic and ferroelectric order coexist in orthorhom- bically distorted perovskite TbMnO3 and are…

Achieving multiferroic two-dimensional (2D) materials should enable numerous functionalities in nanoscale devices. Until now, however, predicted 2D multiferroics are very few and with coexisting yet only loosely coupled (type-I)…

Materials Science · Physics 2019-07-11 Jun-Jie Zhang , Linfang Lin , Yang Zhang , Menghao Wu , Boris I. Yakobson , Shuai Dong

Multiferroic materials, in which electric polarization and magnetic order coexist and couple, offer rich opportunities for both fundamental discovery and technology. However, multiferroicity remains rare due to conflicting electronic…

Materials Science · Physics 2025-10-14 Y. Sun , Y. Ahn , D. Sapkota , H. S. Arachchige , R. Xue , S. Mozaffari , D. G. Mandrus , L. Zhao , J. Orenstein , V. Sunko

Multiferroics, showing simultaneous ordering of electrical and magnetic degrees of freedom, are remarkable materials as seen from both the academic and technological points of view. A prominent mechanism of multiferroicity is the…

Strongly Correlated Electrons · Physics 2012-08-31 P. Lunkenheimer , J. Müller , S. Krohns , F. Schrettle , A. Loidl , B. Hartmann , R. Rommel , M. de Souza , C. Hotta , J. A. Schlueter , M. Lang

A systematic microscopic theory of magnetically induced ferroelectricity and lattice modulation is presented for all electron configurations of Mott-insulating transition-metal oxides. Various mechanisms of polarization are identified in…

Strongly Correlated Electrons · Physics 2009-11-13 Chenglong Jia , Shigeki Onoda , Naoto Nagaosa , Jung Hoon Han

We clarify that the antiferromagnetic order in the distorted tetrahedral quasi-one dimensional spin system induces electric polarizations. In this system, the effects of the low dimensionality and the magnetic frustration are expected to…

The coupling between ferroelectrics and magnetism presents a promising avenue for low-dissipation spintronic devices. However, such couplings remain rare, and the direct realization of magnetic order driven by ferroelectric switching in…

We uncover a new pathway towards multiferroicity, showing how magnetism can drive ferroelectricity without relying on inversion symmetry breaking of the magnetic ordering. Our free-energy analysis demonstrates that any commensurate…

Materials Science · Physics 2009-11-11 Joseph J. Betouras , Gianluca Giovannetti , Jeroen van den Brink

Using first principles calculations, we study the microscopic origin of ferroelectricity (FE) induced by magnetic order in the orthorhombic HoMnO3. We obtain the largest ferroelectric polarization observed in the whole class of improper…

Materials Science · Physics 2009-11-13 Silvia Picozzi , Kunihiko Yamauchi , Biplab Sanyal , Ivan A. Sergienko , Elbio Dagotto

We present an approach for first principles investigations on the spin driven electric polarization in type II multiferroics. We propose a parametrization of the polarization with the parameters calculated using the Korringa-Kohn-Rostoker…

Materials Science · Physics 2025-12-02 Sergiy Mankovsky , Svitlana Polesya , Jan Minar , Hubert Ebert

We report a neutron diffraction study of the multiferroic mechanism in (ND4)2FeCl5D2O, a molecular compound that exhibits magnetically induced ferroelectricity. This material exhibits two successive magnetic transitions on cooling: a…

Although multiferroics have undergone extensive examination for several decades, the occurrence of ferroelectricity induced by orbital order is only scarcely documented. In this study, we propose the existence of spontaneous ferroelectric…

Materials Science · Physics 2025-01-07 Xiao-Feng Luo , Xu He , Rui Wang , Hongjun Xiang , Jin-Zhu Zhao

Symmetry analysis provides crucial insights into the magnetoelectric coupling effect in type-II multiferroics. In this Letter, we comprehensively investigate couplings between electric polarization and inhomogeneous magnetization across all…

Materials Science · Physics 2026-01-30 Xinhai Tu , Di Wang , Hanjing Zhou , Songsong Yan , Huimei Liu , Hongjun Xiang , Xiangang Wan

Within the broad class of multiferroics (compounds showing a coexistence of magnetism and ferroelectricity), we focus on the subclass of "improper electronic ferroelectrics", i.e. correlated materials where electronic degrees of freedom…

Materials Science · Physics 2012-07-26 Silvia Picozzi , Alessandro Stroppa
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