Related papers: Second-Order Nonlinear Response in Centrosymmetric…
We demonstrate that the toroidal dipolar response can be realized in the optical regime by designing a feasible nanostructured metamaterial, comprising asymmetric double-bar magnetic resonators assembled into a toroid-like configuration. It…
We use scanning near-field optical microscopy to study the response of hexagonal boron nitride nanocones at infrared frequencies, where this material behaves as a hyperbolic medium. The obtained images are dominated by a series of hot rings…
We study the formation of second harmonic double-resonance cones in hyperbolic metamaterials. An electric dipole on the surface of the structure induces second harmonic light to propagate into two distinct volume plasmon-polariton channels:…
The second order optical response of centrosymmetric materials manifests itself mostly at their surface, being strongly suppressed in their bulk. However, the overall surface response is also suppressed in nanoparticles with a…
Noble metals with well-defined crystallographic orientation constitute an appealing class of materials for controlling light-matter interactions on the nanoscale. Nonlinear optical processes, being particularly sensitive to anisotropy, are…
We propose to use optical antennas made out of natural hyperbolic material hexagonal boron nitride (hBN), and we demonstrate that this medium is a promising alternative to plasmonic and all-dielectric materials for realizing efficient…
We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…
We present experimental results on the observation of a bulk second-order nonlinear susceptibility derived from both free-space and integrated measurements in silicon nitride. Phase-matching is achieved through dispersion engineering of the…
The theory of Bloembergen and Pershan for the light waves at the boundary of nonlinear media is extended to a nonlinear two-dimensional atomic crystal, i.e. a single planar atomic lattice, placed in between linear bulk media. The crystal is…
Nonlinear optical processes in low dimensional materials are often weak or symmetry forbidden, limiting their use in nanoscale light sources and on chip frequency conversion. Here, we show that combining two weakly nonlinear systems,…
In this work, we investigate the generation of second harmonic light by gold nanorods and demonstrate that the collected nonlinear intensity depends upon a phase interplay between different modes available in the nanostructure. By recording…
Optical response of free-electron gas leads to inherent nonlinear optical behaviour of nanostructured plasmonic materials enabled via both strong local field enhancements and inherent complex electron dynamics. We present a comprehensive…
We report our theoretical results on the emergence of a nonlinear frequency-asymmetric optical response characteristic of chiral crystal systems with neither spatial inversion symmetry nor mirror symmetry. Based on the group theoretical…
Optical spectroscopy based on second-order nonlinearity is a critical technique for characterizing two-dimensional (2D) crystals as well as bioimaging and quantum optics. It is generally believed that second-harmonic generation (SHG) in…
Systematic exploration of amorphous ABC heterostructures revealed that nanoscale morphological modifications markedly improved their artificial bulk second-order susceptibility. These amorphous birefringent heterostructures were fabricated…
Plasmonic metasurfaces have emerged as a promising platform for enhancing a range of nonlinear optical processes, offering compact geometry and flexibility in light manipulation. Second order nonlinear processes, like second harmonic…
We report the fabrication of artificial unidimensional crystals exhibiting an effective bulk second-order nonlinearity. The crystals are created by cycling atomic layer deposition of three dielectric materials such that the resulting…
Crystal quartz is a well-known anisotropic medium with optically active phonons in the THz region where hyperbolic phonon-polaritons can be excited. Here, we use this material to illustrate how the behavior of bulk and surface hyperbolic…
We report about the experimental observation and characterization of nonlinear optical properties of individual silicon nanowires of different dimensions. Our results show that the nonlinear light has different components, one of them…
Planar chiral structures possess a two dimensional handedness that is associated with broken mirror symmetry. Such motifs span vast length scales; examples include certain pinwheel molecules, nautilus shells, cyclone wind patterns and…