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High harmonic generation is a convenient way to obtain extreme ultraviolet light from table-top laser systems and the experimental tools to exploit this simple and powerful light source for time-resolved spectroscopy are being developed by…

Atomic and Molecular Clusters · Physics 2013-12-20 Jakob Grilj , Emily Sistrunk , Markus Koch , Markus Gühr

The atomic response to an ultra-intense driving field produces a characteristic high-harmonic spectrum featuring a rapid drop in intensity for the lower harmonics, followed by a plateau and a sharp cutoff. This response vanishes for…

Quantum Physics · Physics 2026-01-06 Lidija Petrovic , Philipp Stammer , Maciej Lewenstein , Javier Rivera-Dean

We establish time-resolved high harmonic generation (tr-HHG) as a powerful spectroscopy for photoinduced dynamics in strongly correlated materials through a detailed investigation of the insulator-to-metal transitions in vanadium dioxide.…

A theory for laser-driven electron dynamics and high-harmonic generation in bulk solids with two lattice sites per unit cell of arbitrary dimension is formulated. In tight-binding approximation, such solids can be described by $2\times 2$…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Daniel Moos , Hannah Jürß , Dieter Bauer

The high harmonic generation in periodically corrugated submicrometer waveguides is studied numerically. Plasmonic field enhancement in the vicinity of the corrugations allows to use low pump intensities. Simultaneously, periodic placement…

Optics · Physics 2017-07-12 Anton Husakou

We theoretically investigate high-order harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should to exceed…

Atomic Physics · Physics 2016-07-08 Y. Tikman , I. Yavuz , M. F. Ciappina , A. Chacon , Z. Altun , M. Lewenstein

High-harmonic generation (HHG) is a highly nonlinear optical process that typically requires an intense laser to trigger emissions at integer multiples of the driving field frequency. However, the strong fields required for conventional HHG…

Optics · Physics 2025-12-05 Lu Wang , Andrew M. Parks , Adam Thorpe , Graeme Bart , Giulio Vampa , Thomas Brabec

Single-photon sources are in high demand for quantum information applications. A paradigmatic way to achieve single-photon emission is through anharmonicity in the energy levels, such that the absorption of a single photon from a coherent…

Quantum Physics · Physics 2024-04-15 Anael Ben-Asher , Antonio I. Fernández-Domínguez , Johannes Feist

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

Strongly Correlated Electrons · Physics 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì

Interferometric measurements of high-harmonics induced by multiple laser fields in an emerging field of research that promises optimized yield of harmonics, and time and space-resolved nonlinear spectroscopy. Most of the measurements have…

Employing non-Hermitian Floquet theory, the strong-field process of high harmonic (HH) generation by a classical continuous-wave field irradiating ground-state atom is discovered to be controllable by placing the irradiated atom inside a…

Quantum Physics · Physics 2025-09-05 Zohar Amitay , Nimrod Moiseyev

Ultrafast manipulation of vibrational coherence is an emergent route to control the structure of solids. However, this strategy can only induce long-range correlations and cannot modify atomic structure locally, which is required in many…

We numerically demonstrate inhibition of absorption, optical transparency, and anomalous momentum states of phase locked harmonic pulses in semiconductors, at UV and extreme UV frequencies, in spectral regions where the dielectric constant…

Metasurfaces control optical wavefronts via arrays of nanoscale resonators laid out across a surface. When combined with III-V semiconductors with strong optical nonlinearities, a variety of nonlinear effects such as harmonic generation and…

Optics · Physics 2022-07-20 Sylvain D. Gennaro , Raktim Sarma , Igal Brener

A high-power laser pulse at normal incidence onto a plane solid target will generate odd harmonics of its frequency. However, the spacing of the harmonic lines in this configuration is fixed. Here, we study harmonic generation using two…

Optics · Physics 2025-01-20 Raoul Trines , Holger Schmitz , Martin King , Paul McKenna , Robert Bingham

Although solid-state platforms underpin modern electronics, little is known about how intense ultrashort light pulses carrying orbital angular momentum (OAM) interact with solids. This gap persists even though, for more conventional…

High-order harmonic generation (HHG) provides a powerful optical tool for probing ultrafast dynamics on the attosecond timescale. While its mechanisms in gases and solids are well-established, understanding nonlinear optical responses in…

Nonlinear optical phenomena are at the heart of various technological domains such as high-speed data transfer, optical logic applications, and emerging fields such as non-reciprocal optics and photonic time crystal design. However,…

We introduce a modular approach for efficiently interfacing photonic integrated circuits with deep-sub-wavelength hybrid plasmonic functionality. We demonstrate that an off-the-shelf silicon-on-insulator waveguide can be post-processed into…

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