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Self-assembled hybrid perovskite quantum wells have attracted attention due to their tunable emission properties, ease of fabrication and device integration. However, the dynamics of excitons in these materials, especially how they couple…

A system of several Wannier-Mott excitons interacting with phonons in a bulk material is considered. We show that strong exciton-phonon coupling causes the formation of a coherent two-exciton state -- the exciton pair. Unlike the…

Materials Science · Physics 2025-12-30 Vladimir Al. Osipov , Boris Fainberg

The efficiency of two-dimensional Dion-Jacobson-type materials relies on the complex interplay between electronic and lattice dynamics; however, questions remain about the functional role of exciton-phonon interactions. This study…

Phonon polaritons (PhPs) are long-lived electromagnetic modes that originate from the coupling of infrared photons with the bound ionic lattice of a polar crystal. Cubic-Boron nitride (cBN) is such a polar, semiconductor material, which due…

Polaron binding energy and effective mass are calculated for semiconductors with wurtzite crystalline structure from the first order electron-phonon corrections to the self-energy. A recently introduced Frohlich-like electron-phonon…

Materials Science · Physics 2019-08-17 M. E. Mora-Ramos , F. J. Rodriguez , L. Quiroga

A phonoriton is an elementary excitation that is predicted to emerge from hybridization between exciton, phonon and photon. Besides the intriguing many-particle structure, phonoritons are of interest as they could serve as functional nodes…

Materials Science · Physics 2021-06-09 Simone Latini , Umberto De Giovannini , Edbert J. Sie , Nuh Gedik , Hannes Hübener , Angel Rubio

We theoretically investigate the corrections of exciton binding energy in monolayer transition metal dichalcogenides (TMDs) due to the exciton-optical phonon coupling in the Fr$\ddot{o}$hlich interaction model by using the linear operator…

Mesoscale and Nanoscale Physics · Physics 2017-01-04 Zi-Wu Wang , Yao Xiao , Wei-Ping Li , Run-Ze Li , Zhi-Qing Li

Electrons commonly couple through Fr\"ohlich interactions with longitudinal optical phonons to form polarons. However, trions possess a finite angular momentum and should therefore couple instead to rotational optical phonons. This creates…

Phonon polaritons (PhPs) in freestanding and supported multilayers (MuLs) of hexagonal boron nitride (hBN) are systematically studied using a macroscopic optical-phonon model. The PhP properties such as confinement, group velocity,…

Mesoscale and Nanoscale Physics · Physics 2022-03-14 Jian-zhong Zhang

Boron nitride single layer belongs to the family of 2D materials whose optical properties are currently receiving considerable attention. Strong excitonic effects have already been observed in the bulk and still stronger effects are…

Quantum emitters based on atomic defects in layered hexagonal Boron Nitride (hBN) have emerged as promising solid state 'artificial atoms' with atom-like photophysical and quantum optoelectronic properties. Similar to other atom-like…

Employing the density-functional theory with local density approximation, we show that the fully hydrogenated monolayer-hexagonal boron nitride (H$_2$BN) has a direct-band gap of 2.96 eV in the blue-light region while the pristine…

Superconductivity · Physics 2021-10-04 Takat B. Rawal , Ling-Hua Chang , Hao-Dong Liu , Hong-Yan Lu , C. S. Ting

We investigate optical nonlinearities that are induced and enhanced due to the strong phonon resonance in hexagonal boron nitride. We predict and observe large sub-picosecond duration signals due to four-wave mixing (FWM) during resonant…

Excitons consist of electrons and holes held together by their attractive Coulomb interaction. Although excitons are neutral excitations, spatial fluctuations in their charge density couple with the ions of the crystal lattice. This…

Materials Science · Physics 2024-01-18 Zhenbang Dai , Chao Lian , Jon Lafuente-Bartolome , Feliciano Giustino

We study experimentally and theoretically the exciton-phonon interaction in MoSe2 monolayers encapsulated in hexagonal BN, which has an important impact on both optical absorption and emission processes. The exciton transition linewidth…

We report $ab$ $initio$ band diagram and optical absorption spectra of hexagonal boron nitride ($h$-BN), focusing on unravelling how the completeness of basis set for $GW$ calculations and how electron-phonon interactions (EPIs) impact on…

Materials Science · Physics 2020-07-22 Tong Shen , Xiao-Wei Zhang , Honghui Shang , Min-Ye Zhang , Xinqiang Wang , En-Ge Wang , Hong Jiang , Xin-Zheng Li

Hyperbolic polaritons exhibit large photonic density of states and can be collimated in certain propagation directions. The majority of hyperbolic polaritons are sustained in man-made metamaterials. However, natural-occurring hyperbolic…

Mesoscale and Nanoscale Physics · Physics 2021-09-28 Fanjie Wang , Chong Wang , Andrey Chaves , Chaoyu Song , Guowei Zhang , Shenyang Huang , Yuchen Lei , Qiaoxia Xing , Lei Mu , Yuangang Xie , Hugen Yan

Polaritons enable the resonant coupling of excitons and photons to vibrations in the application-relevant super high frequency (SHF, 3-30 GHz) domain. We introduce a novel platform for coherent optomechanics based on the coupling of…

Applied Physics · Physics 2021-04-28 Alexander S. Kuznetsov , Diego H. O. Machado , Klaus Biermann , Paulo V. Santos

Strong coupling between molecular vibrations and microcavity modes has been demonstrated to modify physical and chemical properties of the molecular material. Here, we study the much less explored coupling between lattice vibrations…

The unique physical, mechanical, chemical, optical, and electronic properties of hexagonal boron nitride (hBN) make it a promising two-dimensional material for electronic, optoelectronic, nanophotonic, and quantum devices. Here we report on…

Materials Science · Physics 2023-06-26 E. Janzen , H. Schutte , J. Plo , A. Rousseau , T. Michel , W. Desrat , P. Valvin , V. Jacques , G. Cassabois , B. Gil , J. H. Edgar