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Off-stoichiometric Ni$_2$MnIn Heusler alloys have drawn recent attention due to their large magnetocaloric entropy change associated with the first-order magneto-structural transition. Here we present crystal structural, calorimetric and…

Earlier investigation of Co_{0.2}Zn_{0.8}Fe_{1.95}Ho_{0.05}O_{4} spinel has shown the existence of "super-ferromagnetic " clusters containing Fe^{3+} and Ho^{3+} ions along with small size clusters of Fe^{3+} ions (Bhowmik et al, J. Magn.…

Soft Condensed Matter · Physics 2007-05-23 R. N. Bhowmik , R. Ranganathan , R. Nagarajan

An important contribution to the thermoelectric and spin-caloric transport properties in magnetic materials at elevated temperatures is the formation of a spin-disordered state due to local moment fluctuations. This effect has not been…

Materials Science · Physics 2015-06-23 Roman Kováčik , Phivos Mavropoulos , Stefan Blügel

The AlCrTiV high entropy alloy undergoes an order-disorder transition from body centered cubic (Strukturbericht A2) at high temperatures to the CsCl structure (B2) at intermediate temperatures. We model this transition using first…

Materials Science · Physics 2024-07-02 Michael Widom

As various property studies continue to emerge on high entropy and entropy-stabilized ceramics, we seek further understanding of property changes across the phase boundary between \enquote{high-entropy} and \enquote{entropy-stabilized}. The…

We present a comprehensive study of the magnetic structure evolution across the spin reorientation transition in orthorhombic (Pnma) TmCrO3. Magnetic susceptibility reveals canted antiferromagnetic (CAFM) ordering at T_N = 125 K, two…

Strongly Correlated Electrons · Physics 2025-11-12 Vishesh Sharma , Gaurav Gautam , Poonam Yadav , Chin-Wei Wang , Kaya Wei , N. P. Lalla , Theo Siegrist , Shivani Sharma

The cubic spinel FeCr2S4 has been receiving immense research interest because of its emergent phases and the interplay of spin, orbital and lattice degrees of freedom. Despite the intense research, several fundamental questions are yet to…

We report the magnetic properties of mechanically milled Co$_{0.2}$Zn$_{0.8}$Fe$_2$O$_4$ spinel oxide. After 24 hours milling of the bulk sample, the XRD spectra show nanostructure with average particle size $\approx$ 20 nm. The as milled…

Soft Condensed Matter · Physics 2009-11-07 R. N. Bhowmik , R. Ranganathan , S. sarkar , C. Bansal , R. Nagarajan

The rise of high-entropy oxides as a major functional materials design principle in recent years has prompted us to investigate how compositional disorder affects long-range magnetic ordering in double perovskite oxides. Since ferromagnetic…

Single crystals of SrMn2P2 and CaMn2P2 were grown using Sn flux and characterized by single-crystal x-ray diffraction, electrical resistivity rho, heat capacity Cp, and magnetic susceptibility chi = M/H measurements versus temperature T and…

Strongly Correlated Electrons · Physics 2021-11-01 N. S. Sangeetha , Santanu Pakhira , Q. -P. Ding , H. -C. Lee , V. Smetana , A. -V. Mudring , Y. Furukawa , D. C. Johnston

Many new families of quasicrystal-forming magnetic alloys have been synthesized and studied in recent years. For small changes of composition, the alloys can go from quasiperiodic to periodic (approximant crystals) while conserving most of…

Strongly Correlated Electrons · Physics 2026-03-31 Anuradha Jagannathan

We used femtosecond optical spectroscopy to study ultrafast spin and orbital ordering dynamics in the antiferromagnetic Mott insulator $\alpha$-Sr$_2$CrO$_4$. This chromate system possesses multiple spin and orbital ordered phases, and…

We have carried out neutron diffraction and small angle neutron scattering measurements on a high quality single crystal of the cubic lacunar spinel multiferroic, GaV$_4$S$_8$, as a function of magnetic field and temperature to determine…

We report on the synthesis of a new $\gamma$-phase of the spin $S$~=~$\frac{3}{2}$ compound SrCo$_2$(PO$_4$)$_2$ together with a detailed structural, magnetic and thermodynamic properties. The $\gamma$-phase of SrCo$_2$(PO$_4$)$_2$…

Strongly Correlated Electrons · Physics 2021-03-30 Arvind Yogi , T. Chakrabarty , P. L. Paulose , Ruta Kulkarni , Mayanak Kumar Gupta , Arumugam Thamizhavel

We have investigated the spin fluctuations in the langasite compound Ba3NbFe3Si2O14 in both the ordered state and as a function of temperature. The low temperature magnetic structure is defined by a spiral phase characterized by magnetic…

Strongly Correlated Electrons · Physics 2015-05-19 C. Stock , L. C. Chapon , A. Schneidewind , Y. Su , P. G. Radaelli , D. F. McMorrow , A. Bombardi , N. Lee , S. -W. Cheong

Dynamical properties of the lattice structure was studied by optical spectroscopy in ACr2O4 chromium spinel oxide magnetic semiconductors over a broad temperature region of T=10-335K. The systematic change of the A-site ions (A=Mn, Fe, Co,…

Strongly Correlated Electrons · Physics 2013-07-24 V. Kocsis , S. Bordács , D. Varjas , K. Penc , A. Abouelsayed , C. A. Kuntscher , K. Ohgushi , Y. Tokura , I. Kézsmárki

We have successfully synthesized single crystals, solved the crystal structure, and studied the magnetic properties of a new family of copper halides (C$_4$H$_{14}$N$_2$)Cu$_2X_6$ ($X$= Cl, Br). These compounds crystallize in an…

Materials Science · Physics 2023-06-28 P. Biswal , S. Guchhait , S. Ghosh , S. N. Sarangi , D. Samal , Diptikant Swain , Manoranjan Kumar , R. Nath

KCrF3 represents another prototypical orbital-ordered perovskite, where Cr2+ possesses the same electronic configuration of 3d4 as that of strongly Jahn-Teller distorted Mn3+ in many CMR manganites. The crystal and magnetic structures of…

Strongly Correlated Electrons · Physics 2013-09-30 Y. Xiao , Y. Su , H. -F. Li , C. M. N. Kumar , R. Mittal , J. Persson , A. Senyshyn , K. Gross , Th. Brueckel

In spinels ACr2O4 (A=Mg, Zn) realisation of the classical pyrochlore Heisenberg antiferromagnet model is complicated by a strong spin-lattice coupling: the extensive degeneracy of the ground state is lifted by a magneto-structural…

Neutron and synchrotron resonant X-ray magnetic scattering (RXMS) complemented by heat capacity and resistivity measurements reveal the evolution of the magnetic structures of Fe and Ce sublattices in single crystal CeFeAsO. The RXMS of…

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