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To understand the recently observed mysterious non-adiabatic energy transfer for hyperthermal H atom scattering from a semiconductor surface, Ge(111)c(2*8), we present a mixed quantum-classical non-adiabatic molecular dynamics model based…

Adiabatic quantum computing (AQC) is a promising approach for discrete and often NP-hard optimization problems. Current AQCs allow to implement problems of research interest, which has sparked the development of quantum representations for…

Machine Learning · Computer Science 2024-05-02 Jan-Nico Zaech , Martin Danelljan , Tolga Birdal , Luc Van Gool

We extend the rigorous adiabatic coupled-channel formalism to ultracold nonreactive atom-molecule collisions in the presence of an external magnetic field. The wavefunction of the collision complex is expanded in adiabatic basis states…

Chemical Physics · Physics 2025-12-01 Nathan S. Prins , Timur V. Tscherbul

An one dimensional adiabatic model has been proposed for fusion of loosely bound and halo light nuclei with various heavy targets. It is shown that fusion cross sections at near and sub-barrier energies can be explained using a simple WKB…

Nuclear Theory · Physics 2010-11-23 Ajit Kumar Mohanty

Astrophysical modeling of processes in environments that are not in local thermal equilibrium requires the knowledge of state-to-state rate coefficients of rovibrational transitions in molecular collisions. These rate coefficients can be…

Chemical Physics · Physics 2022-07-13 Taha Selim , Ad van der Avoird , Gerrit C. Groenenboom

The development of advanced quantum technologies and the quest for a deeper understanding of many-particle quantum mechanics requires control over the quantum state of interacting particles to a high degree of fidelity. However, the quickly…

Quantum Physics · Physics 2016-03-17 Albert Benseny , Jérémie Gillet , Thomas Busch

We review recent theoretical calculations of charge transfer through mesoscopic devices in response to slowly-oscillating, spatially-confined, potentials. The discussion is restricted to non-interacting electrons, and emphasizes the role of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Ora Entin-Wohlman , Amnon Aharony , Vyacheslavs Kashcheyevs

We perform on-the-fly non-adiabatic molecular dynamics simulations using the symmetrical quasi-classical (SQC) approach with the recently suggested molecular Tully models: ethylene and fulvene. We attempt to provide benchmarks of the SQC…

Chemical Physics · Physics 2021-09-15 Braden M. Weight , Arkajit Mandal , Pengfei Huo

Dissociative chemisorption is a key process in hydrogen-metal surface chemistry, where nonadiabatic effects due to low-lying electron-hole-pair excitations may affect reaction outcomes. Molecular dynamics with electronic friction…

Chemical Physics · Physics 2025-05-26 Wojciech G. Stark , Connor L. Box , Matthias Sachs , Nils Hertl , Reinhard J. Maurer

Many physically interesting models show a quantum phase transition when a single parameter is varied through a critical point, where the ground state and the first excited state become degenerate. When this parameter appears as a coupling…

Quantum Physics · Physics 2008-09-24 Gernot Schaller

We consider quantum statistics of charge transmitted through a mesoscopic device in the adiabatic pumping process. A general formula for the distribution function of the transmitted charge in terms of the time-dependent S-matrix is…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Anton Andreev , Alex Kamenev

We study the onset of particle statistics effects as the temperature is lowered in strongly correlated two-dimensional Hubbard models. We utilize numerical linked-cluster expansions and focus on the properties of interacting lattice…

Strongly Correlated Electrons · Physics 2012-08-31 Ehsan Khatami , Marcos Rigol

Adiabatic quantum algorithms represent a promising approach to universal quantum computation. Whilst in a closed system these algorithms are limited by avoided level crossings, where the gap becomes exponentially small in the system size,…

Quantum Physics · Physics 2016-10-12 Dominik S. Wild , Sarang Gopalakrishnan , Michael Knap , Norman Y. Yao , Mikhail D. Lukin

Microscopic thermal machines promise to play an important role in future quantum technologies. Making such devices widely applicable will require effective strategies to channel their output into easily accessible storage systems like…

Statistical Mechanics · Physics 2024-10-02 Joshua Eglinton , Federico Carollo , Igor Lesanovsky , Kay Brandner

Density-functional theory calculations are performed to investigate hydrogen transport in the proton conductor BaSnO$_3$. Structural optimizations in the stable and saddle point configurations for transfer and reorientation allow…

Materials Science · Physics 2014-11-13 Grégory Geneste , Alistar Ottochian , Jessica Hermet , Guilhem Dezanneau

A quantum statistical model of nuclear multifragmentation is proposed. The recurrence equation method used within the canonical ensemble makes the model solvable and transparent to physical assumptions and allows to get results without…

Nuclear Theory · Physics 2009-10-31 A. S. Parvan , V. D. Toneev , M. Ploszajczak

It is shown that statistical mechanics is applicable to isolated quantum systems with finite numbers of particles, such as complex atoms, atomic clusters, or quantum dots in solids, where the residual two-body interaction is sufficiently…

Statistical Mechanics · Physics 2016-08-31 V. V. Flambaum , A. A. Gribakina , G. F. Gribakin , I. V. Ponomarev

The design of new quantum algorithms has proven to be an extremely difficult task. This paper considers a different approach to the problem, by studying the problem of 'quantum state generation'. This approach provides intriguing links…

Quantum Physics · Physics 2007-05-23 Dorit Aharonov , Amnon Ta-Shma

In this paper we study up to which extent we can apply adiabatic control strategies to a quantum control model obtained by rotating wave approximation. In particular, we show that, under suitable assumptions on the asymptotic regime between…

Optimization and Control · Mathematics 2021-01-12 Nicolas Augier , Ugo Boscain , Mario Sigalotti

A theoretical method for the estimation of cross sections and rates for excitation and charge transfer processes in low-energy hydrogen atom collisions with neutral atoms, based on an asymptotic two-electron model of ionic-covalent…

Atomic Physics · Physics 2016-05-04 Paul S. Barklem