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The insulator-bad metal transition observed in the Jahn-Teller (JT) magnets orthonickelates RNiO$_3$ (R = rare earth or yttrium Y) is considered to be a canonical example of the Mott transition, traditionally described in the framework of…

Strongly Correlated Electrons · Physics 2025-08-12 A. S. Moskvin

The orbital degree of freedom in rare-earth nickelates is typically inactive across the temperature-driven metal-insulator transition, where the system develops two inequivalent Ni sites associated with Ni-O bond disproportionation and…

Strongly Correlated Electrons · Physics 2026-04-22 Sangeeta Rajpurohit , Sheikh Rubaiat Ul Haque , Aaron M. Lindenberg , Peter E. Blöchl , Tadashi Ogitsu

For decades transition-metal oxides have generated a huge interest due to the multitude of physical phenomena they exhibit. In this class of materials, the rare-earth nickelates, $R$NiO$_3$, stand out for their rich phase diagram stemming…

Strongly Correlated Electrons · Physics 2023-09-18 Luca Binci , Michele Kotiuga , Iurii Timrov , Nicola Marzari

In LiNiO$_2$ Ni$^{3+}$ ion has $d^7$ configuration in cubic crystal field with one electron on double degenerate $e_g$ orbitals, and such ion is considered to be Jahn-Teller (JT) active. However despite the fact, that this compound is an…

Strongly Correlated Electrons · Physics 2019-01-09 Dm. M. Korotin , D. Novoselov , V. I. Anisimov

We use density functional plus $U$ methods to study the effects of a tensile or compressive substrate strain on the charge-ordered insulating phase of LuNiO$_3$. The numerical results are analyzed in terms of a Landau energy function, with…

Strongly Correlated Electrons · Physics 2015-06-03 Zhuoran He , Andrew J. Millis

A set of broken symmetry two-dimensional ground states are predicted in (111)-oriented (LaNiO$_3$)$_N$/(LaAlO$_3$)$_M$ ($N$/$M$) superlattices, based on density functional theory (DFT) calculations including a Hubbard $U$ term. An…

Strongly Correlated Electrons · Physics 2014-03-26 David Doennig , Warren E. Pickett , Rossitza Pentcheva

Rare-earth nickelates RNiO3 (R=rare-earth element) exhibit three kinds of phase transitions with decreasing temperature: a structural transition from a pseudo-cubic to a monoclinic phase, a metal- insulator transition (MIT), and a magnetic…

By employing first-principles electronic structure calculations we investigate nickelate superlattices [LaNiO$_3$]$_1$/[LaAlO$_3$]$_1$ and [LaNiO$_3$]$_1$/[SrTiO$_3$]$_1$ with (001) orientation under epitaxial tensile strain. Within density…

Strongly Correlated Electrons · Physics 2023-04-12 Heung-Sik Kim , Sang Hyeon Park , Myung Joon Han

We study a model for the metal-insulator (MI) transition in the rare-earth nickelates RNiO$_3$, based upon a negative charge transfer energy and coupling to a rock-salt like lattice distortion of the NiO$_6$ octahedra. Using exact…

Strongly Correlated Electrons · Physics 2014-03-12 Steve Johnston , Anamitra Mukherjee , Ilya Elfimov , Mona Berciu , George A. Sawatzky

The phase diagram of half-doped manganite systems of formula A_{0.5}A'_{0.5}MnO_3 is investigated within a single-orbital model incorporating magnetic double-exchange and superexchange, together with intersite Coulomb and electron-lattice…

Strongly Correlated Electrons · Physics 2009-10-31 S. Fratini , D. Feinberg , M. Grilli

We introduce an effective model for $e_g$ electrons to describe quasi-two-dimensional layered La$_{2-x}$Sr$_{x}$NiO$_4$ nickelates and study it using correlated wave functions on $8 \times 8 $ and $6 \times 6 $ clusters. The effective…

Strongly Correlated Electrons · Physics 2011-12-16 Krzysztof Rościszewski , Andrzej M. Oleś

The insulator-quasi-metal (bad metal) transition observed in Jahn-Teller (JT) magnets orthonickelates RNiO$_3$ (R = rare earth, or yttrium Y) is considered a canonical example of the Mott transition, traditionally described in the framework…

Strongly Correlated Electrons · Physics 2025-12-16 A. S. Moskvin , Yu. D. Panov

Using the DFT+dynamical mean-field theory method we revisit the pressure-temperature phase diagram of the prototypical correlated insulator NiO. We study the pressure-induced evolution of the electronic structure, magnetic state, and…

Strongly Correlated Electrons · Physics 2024-12-03 G. M. Gaifutdinov , I. V. Leonov

Motivated by the discovery of high-temperature superconductivity in bilayer nickelate La$_3$Ni$_2$O$_7$ under pressure, we investigate the ground-state phase diagram and correlation effects using determinant quantum Monte Carlo simulations…

Strongly Correlated Electrons · Physics 2025-02-07 Jian-Jian Yang , Dao-Xin Yao , Han-Qing Wu

The perovksite rare-earth nickelates, RNiO$_3$ (R=La ... Lu), are a class of materials displaying a rich phase-diagram of metallic and insulating phases associated with charge and magnetic order. Being in the charge transfer regime,…

Strongly Correlated Electrons · Physics 2015-04-14 John W. Freeland , Michel van Veenendaal , Jak Chakhalian

Rare-earth orthonickelates RNiO3 are Jahn-Teller magnets, unstable with respect to the anti-Jahn-Teller disproportionation reaction with the formation of a system equivalent to a system of effective spin-triplet composite bosons moving in a…

Statistical Mechanics · Physics 2025-11-18 V. S. Ryumshin , S. V. Nuzhin , Yu. D. Panov , A. S. Moskvin

At room temperature, bulk La$_{7/8}$Sr$_{1/8}$MnO$_3$ is in the dynamic Jahn--Teller O$^*$ phase, but undergoes a transition to a static, magnetically ordered Jahn--Teller phase at lower temperatures. Here we study a $6$ unit cells thin…

Controlled introduction of oxygen vacancies offers an effective route to induce metal-to-insulator transition in strongly correlated rare-earth nickelates ($R$NiO$_3$) at room temperature. However, the role played by the rare-earth cations…

Materials Science · Physics 2024-12-30 Devang Bhagat , Ranga Teja Pidathala , Badri Narayanan

The material class of rare earth nickelates with high Ni$^{3+}$ oxidation state is generating continued interest due to the occurrence of a metal-insulator transition with charge order and the appearance of non-collinear magnetic phases…

Strongly Correlated Electrons · Physics 2018-01-11 H. Guo , Z. W. Li , L. Zhao , Z. Hu , C. F. Chang , C. -Y. Kuo , W. Schmidt , A. Piovano , T. W. Pi , O. Sobolev , D. I. Khomskii , L. H. Tjeng , A. C. Komarek

Motivated by recent Fermi surface and transport measurements on LaNiO3, we study the Mott Metal-Insulator transitions of perovskite nickelates, with the chemical formula RNiO3, where R is a rare-earth ion. We introduce and study a minimal…

Strongly Correlated Electrons · Physics 2015-05-28 SungBin Lee , Ru Chen , Leon Balents
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