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Two dimensional van der Waals ferromagnets with honeycomb structures are expected to host the bosonic version of Dirac particles in their magnon excitation spectra. Using inelastic neutron scattering, we study spin wave excitations in…

Strongly Correlated Electrons · Physics 2021-10-29 Lebing Chen , Matthew B. Stone , Alexander I. Kolesnikov , Barry Winn , Wonhyuk Shon , Pengcheng Dai , Jae-Ho Chung

CrI3 is a prototypical van der Waals ferromagnet with a magnetic honeycomb lattice. Previous inelastic neutron scattering studies have suggested topological nature of its magnetic excitations with a magnon gap at the Dirac points, which are…

Materials Science · Physics 2024-03-14 Chunqiang Xu , Heda Zhang , Caitlin Carnahan , Pengpeng Zhang , Di Xiao , Xianglin Ke

In two dimensional honeycomb ferromagnets, bosonic magnon quasiparticles (spin waves) may either behave as massless Dirac fermions or form topologically protected edge states. The key ingredient defining their nature is the next-nearest…

Strongly Correlated Electrons · Physics 2018-11-21 Lebing Chen , Jae-Ho Chung , Bin Gao , Tong Chen , Matthew B. Stone , Alexander I. Kolesnikov , Qingzhen Huang , Pengcheng Dai

Magnons dominate the magnetic response of the recently discovered insulating ferromagnetic two dimensional crystals such as CrI$_3$. Because of the arrangement of the Cr spins in a honeycomb lattice, magnons in CrI$_3$ bear a strong…

Mesoscale and Nanoscale Physics · Physics 2020-02-04 A. T. Costa , D. L. R. Santos , N. M. R. Peres , J. Fernández-Rossier

CrBr$_3$ is an excellent realization of the two-dimensional honeycomb ferromagnet, which offers a bosonic equivalent of graphene with Dirac magnons and topological character. We perform inelastic neutron scattering (INS) measurements using…

Strongly Correlated Electrons · Physics 2022-11-01 S. E. Nikitin , B. Fåk , K. W. Krämer , T. Fennell , B. Normand , A. M. Läuchli , Ch. Rüegg

In this work, we study the magnon-magnon interaction effect in typical honeycomb ferromagnets consisting of van der Waals-bonded stacks of honeycomb layers, e.g., chromium trihalides CrX3 (X = F, Cl, Br, and I), that display two spin-wave…

Mesoscale and Nanoscale Physics · Physics 2023-05-03 Hao Sun , Dhiman Bhowmick , Bo Yang , Pinaki Sengupta

The search for topological spin excitations in recently discovered two-dimensional (2D) van der Waals (vdW) magnetic materials is important because of their potential applications in dissipation-less spintronics. In the 2D vdW ferromagnetic…

We study the effects of magnon-magnon interactions in the two-dimensional van der Waals ferromagnet CrBr$_3$ focusing on its honeycomb lattice structure. Motivated by earlier theoretical predictions of temperature-induced spectral shifts…

Materials Science · Physics 2025-09-05 Saikat Banerjee , Stephan Humeniuk

The discovery of 2-dimensional (2D) materials, such as CrI3, that retain magnetic ordering at monolayer thickness has resulted in a surge of research in 2D magnetism from both pure and applied perspectives. Here, we report a magneto-Raman…

Bosonic Dirac materials are testbeds for dissipationless spin-based electronics. In the quasi two-dimensional honeycomb lattice of CrX$_{3}$ (X=Cl, Br, I), Dirac magnons have been predicted at the crossing of acoustical and optical spin…

Materials Science · Physics 2024-05-14 John A. Schneeloch , Yu Tao , Yongqiang Cheng , Luke Daemen , Guangyong Xu , Qiang Zhang , Despina Louca

Two-dimensional (2D) magnetism has been long sought-after and only very recently realized in atomic crystals of magnetic van der Waals materials. So far, a comprehensive understanding of the magnetic excitations in such 2D magnets remains…

We conduct a comprehensive study of three different magnetic semiconductors, CrI$_3$, CrBr$_3$, and CrCl$_3$, by incorporating both few- and bi-layer samples in van der Waals tunnel junctions. We find that the interlayer magnetic ordering,…

CrCl3, a layered van der Waals (vdW) magnet, exhibits in-plane magnetic anisotropy and enhanced interlayer coupling upon stacking, making it an ideal platform to host exotic nanoscale magnetic phenomena such as magnon hydrodynamics and…

Higher-order exchange interactions and quantum effects are widely known to play an important role in describing the properties of low-dimensional magnetic compounds. Here we identify the recently discovered two-dimensional (2D) van der…

We study the microscopical origin of anisotropic ferromagnetism in the van der Waals magnet CrI3. We conclude that the nearest neighbors exchange is well described by the Heisenberg-Kitaev-Gamma (HKGamma) model, and we also found a nonzero…

Mesoscale and Nanoscale Physics · Physics 2021-05-19 Rodrigo Jaeschke-Ubiergo , Eric Suarez Morell , Alvaro Sebastian Nunez

Two-dimensional (2D) honeycomb ferromagnets, such as monolayer chromium-trihalides, are predicted to behave as topological magnon insulators - characterized by an insulating bulk and topologically protected edge states, giving rise to a…

Mesoscale and Nanoscale Physics · Physics 2023-08-10 M. Soenen , M. V. Milosevic

In this article, we calculate the magnon spectrum of Kitaev-Heisenberg magnets. This model has been recently proposed as a spin Hamiltonian to model $\text{CrI}_3$ and other two-dimensional magnets. It is a minimal spin Hamiltonian that…

Materials Science · Physics 2020-07-15 Esteban Aguilera , Rodrigo Jaeschke-Ubiergo , Nicolas Vidal-Silva , Luis Foa , Alvaro Núñez

Dirac magnons, the bosonic counterparts of Dirac fermions in graphene, provide a unique platform to explore symmetry-protected band crossings and quantum geometry in magnetic insulators, while promising high-velocity, low-dissipation spin…

Strongly Correlated Electrons · Physics 2026-05-07 Rintaro Eto , Ignacio Salgado-Linares , Masahito Mochizuki , Johannes Knolle , Alexander Mook

We performed inelastic neutron scattering experiments on single-crystal samples of the honeycomb lattice magnet, ilmenite NiTiO3. Below the Neel temperature of 22 K, spin wave excitations with a band energy of 3.7 meV were observed. The…

Strongly Correlated Electrons · Physics 2025-01-22 Hodaka Kikuchi , Makoto Ozeki , Nobuyuki Kurita , Shinichiro Asai , Travis J. Williams , Tao Hong , Takatsugu Masuda

Chromium triiodide is an intrinsically magnetic van der Waals material down to the single-layer limit. Here, we provide a first-principles description of finite-temperature magnetic and spectral properties of monolayer (ML) CrI$_3$ based on…

Strongly Correlated Electrons · Physics 2022-05-24 Yaroslav O. Kvashnin , Alexander N. Rudenko , Patrik Thunström , Malte Rösner , Mikhail I. Katsnelson
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