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Revealing the dynamic structural evolution and lithium transport properties during the charge/discharge processes is crucial for optimizing graphite anodes in lithium-ion batteries, enabling high stability and fast-charging performance.…

Materials Science · Physics 2025-08-11 Liqi Wang , Xuhe Gong , Zicun Li , Ruijuan Xiao , Hong Li

We explore the effect of lattice anisotropy on the charge-ordered superconductor 2H-NbSe$_{2}$. Using a novel strain apparatus, we measure the superconducting transition temperature $T_{sc}$ as a function of uniaxial strain. It is found…

Electrides are unique compounds where most of the electrons reside at interstitial regions of the crystal behaving as anions, which strongly determines its physical properties. Interestingly, the magnitude and distribution of interstitial…

Superconductivity · Physics 2019-03-11 Ziyuan Zhao , Shoutao Zhang , Tong Yu , Haiyang Xu , Aitor Bergara , Guochun Yang

The superconducting (SC) state of iron-based compounds in both tetragonal and orthorhombic phases is studied on the basis of an effective Hamiltonian composed of the kinetic energy including the five Fe 3d-orbitals, the orthorhombic…

Strongly Correlated Electrons · Physics 2015-05-28 Naoya Arakawa , Masao Ogata

In the development of low cost, sustainable, and energy-dense batteries, chloride-based compounds are promising catholyte materials for solid-state batteries owing to their high Na-ion conductivities and oxidative stabilities. The ability…

We analyze the electronic structure of lithium ionic conductors, ${\rm Li_3PO_4}$ and ${\rm Li_3PS_4}$, using the electronic stress tensor density and kinetic energy density with special focus on the ionic bonds among them. We find that, as…

Chemical Physics · Physics 2016-08-17 Hiroo Nozaki , Yosuke Fujii , Kazuhide Ichikawa , Taku Watanabe , Yuichi Aihara , Akitomo Tachibana

Strain is a powerful experimental tool to explore new electronic states and understand unconventional superconductivity. Here, we investigate the effect of uniaxial strain on the nematic and superconducting phase of single crystal FeSe…

We present a theory for carrier transport in semiconducting nanoscale heterostructures that emphasizes the effects of strain at the interface between two different crystal structures. An exactly solvable model shows that the interface…

Mesoscale and Nanoscale Physics · Physics 2012-06-25 Mark C. Sweeney , Joel D. Eaves

The large volume change of the silicon (Si) during lithiation and delithiation process has long been a problem impeding its application as one of the most promising anode materials for LIBs. In this paper, we proposed a conceptually new…

Applied Physics · Physics 2020-08-04 Zhenbin Guo , Haimin Yao

To elucidate different photoinduced melting dynamics of charge orders observed in quasi-two-dimensional organic conductors $ \theta $-(BEDT-TTF)$_2$RbZn(SCN)$_4$ and $ \alpha $-(BEDT-TTF)$_2$I$_3$…

Strongly Correlated Electrons · Physics 2010-03-11 Satoshi Miyashita , Yasuhiro Tanaka , Shinichiro Iwai , Kenji Yonemitsu

This study presents a comprehensive Multiphysics model for zinc-ion batteries (ZIBs), incorporating electrochemical aspects. The model integrates the mass transport of Zn2+ ions, charge transfer, and solid diffusion to predict performance…

Materials Science · Physics 2025-05-06 Roya Rajabi , Shichen Sun , Booker Wu , Jamil Khan , Kevin Huang

Two-dimensional iron-chalcogenide intercalates display a remarkable correlation of the interlayer spacing with the enhancement of the superconducting critical temperature ($T_c$). In this work, synchrotron x-ray absorption ($XAS$, at Fe and…

A gap in understanding the link between continuum theories of ion transport in ionic liquids and the underlying microscopic dynamics has hindered the development of frameworks for transport phenomena in these concentrated electrolytes.…

Soft Condensed Matter · Physics 2015-09-11 Alpha A. Lee , Svyatoslav Kondrat , Dominic Vella , Alain Goriely

The properties of the mixed system LiBH4 LiCl P2S5 are studied with respect to all-solid-state batteries. The studied material undergoes an amorphization upon heating above 601C, accompanied with increased Li+ conductivity beneficial for…

Rechargeable lithium ion batteries are an attractive alternative power source for a wide variety of applications. To optimize their performances, a complete description of the solvation properties of the ion in the electrolyte is crucial. A…

Solid-state electrolytes, by enabling lithium metal anodes, may significantly increase the energy density of current lithium-ion batteries. However, similar to their liquid counterparts, these hard and stiff electrolytes can still be…

Chemical Physics · Physics 2024-10-04 Rajeev Gopal , Longan Wu , Youngju Lee , Jinzhao Guo , Peng Bai

We report the ion transport mechanisms in succinonitrile (SN) loaded solid polymer electrolytes containing polyethylene oxide (PEO) and dissolved lithium bis(trifluoromethane)sulphonamide (LiTFSI) salt using molecular dynamics simulations.…

Energy efficient, safe and reliable Li-ion batteries (LIBs) are required for a wide range of applications. Charging capabilities of thick electrodes still holding their stored high-energy is a most desirable characteristic in future…

Efficient and safe energy storage technologies are essential for realizing a sustainable and electrified society. Among the key challenges, the design of superionic conductors for all-solid-state batteries often faces a fundamental…

Materials Science · Physics 2025-11-06 Rikuya Ishikawa , Kyohei Takae , Rei Kurita

Cerium-based ternary compounds CeNi$_2$Cd$_{20}$ and CePd$_2$Cd$_{20}$ do not exhibit long-range order down to millikelvin temperature range. Given the large separation between cerium ions which significantly reduces the superexchange…

Superconductivity · Physics 2023-08-15 Suman Raj Panday , Maxim Dzero