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Producing currents predominantly from a single valley, namely valley-polarized currents, at optical-cycle timescales is an important aspect of the petahertz valleytronics, yet it remains less developed. This work exhibits the feasibility of…

Optics · Physics 2025-03-13 Wenqing Li , Xiaosong Zhu , Liang Li , Wanzhu He , Jie Long , Pengfei Lan , Peixiang Lu

Nonlinear transport plays a vital role in probing the quantum geometry of Bloch electrons, valley chirality, and carrier scattering mechanisms. The nonlinear Hall effect, characterized by a nonlinear scaling of Hall voltage with…

Mesoscale and Nanoscale Physics · Physics 2024-12-05 Xin Liao , Xing-Yu Liu , An-Qi Wang , Qing Yin , Tong-Yang Zhao , Zhi-Min Liao

We show that, because of the inevitable twist and lattice mismatch in heterobilayers of transition metal dichalcogenides, interlayer excitons have six-fold degenerate light cones anomalously located at finite velocities on the parabolic…

Mesoscale and Nanoscale Physics · Physics 2015-11-05 Hongyi Yu , Yong Wang , Qingjun Tong , Xiaodong Xu , Wang Yao

Valleytronics has emerged as a promising paradigm, enabling comprehensive control of the valley degree of freedom (DoF) for energy-efficient and high-speed information processing. However, backscattering-induced valley depolarization…

Valleytronics exploits non-equivalent energy extrema in the electronic band structure of crystalline solids -- the valley degree of freedom -- to encode, manipulate, and read out information. The advent of 2D materials, first graphene and…

Nonlinear light-matter interaction and, in particular, high-harmonic generation (HHG) are fundamentally interesting and frequently discussed as versatile probes of quantum materials with potential for optical information processing…

Mesoscale and Nanoscale Physics · Physics 2026-04-15 Jessica O. de Almeida , Wilton J. M. Kort-Kamp , Mathias S. Scheurer

Alloyed transition metal dichalcogenides provide an opportunity for coupling band engineering with valleytronic phenomena in an atomically-thin platform. However, valley properties in alloys remain largely unexplored. We investigate the…

Mesoscale and Nanoscale Physics · Physics 2020-01-17 Sean M. Oliver , Joshua Young , Sergiy Krylyuk , Thomas L. Reinecke , Albert V. Davydov , Patrick M. Vora

A recent scientific debate has arisen: Which processes underlie the actual ground of the valley Hall effect (VHE) in two-dimensional materials? The original VHE emerges in samples with ballistic transport of electrons due to the anomalous…

Mesoscale and Nanoscale Physics · Physics 2021-02-03 I. Vakulchyk , V. M. Kovalev , I. G. Savenko

Semiconducting transition metal dichalcogenide monolayers have emerged as promising candidates for future valleytronics-based quantum information technologies. Two distinct momentum-states of tightly-bound electron-hole pairs in these…

Mesoscale and Nanoscale Physics · Physics 2017-03-16 Gerd Plechinger , Tobias Korn , John M. Lupton

We study the role of transition rule in high-order harmonic generation from solids driven by linearly polarized laser elds. The orientation-dependent transition dipoles can regulate the emergence of the multi-plateau structure. In the…

Optics · Physics 2019-03-07 Tao-Yuan Du , Si-Jing Ding

We develop multipolar theory of nonlinear generation of entangled photons from subwavelength dielectric particles due to the spontaneous parametric downconversion. We demonstrate that optical excitation in resonance with the high-quality…

Optics · Physics 2018-08-15 Alexander N. Poddubny , Daria A. Smirnova

Degenerate extrema in the energy dispersion of charge carriers in solids, also referred to as valleys, can be regarded as a binary quantum degree of freedom, which can potentially be used to implement valleytronic concepts in van der Waals…

The nonlinear optical response of a system of molecules often contains contributions whereby the products of lower-order processes in two separate molecules give signals that appear on top of a genuine direct higher-order process with a…

Quantum Physics · Physics 2017-04-05 Kochise Bennett , Vladimir Y. Chernyak , Shaul Mukamel

Two-dimensional hexagonal materials such as transition metal dichalcogenides exhibit valley degrees of freedom, offering fascinating potential for valley-based quantum computing and optoelectronics. In nonlinear optics, the K and K' valleys…

Valley, as a degree of freedom, has been exploited to realize valley-selective Hall transport and circular dichroism in two-dimensional layered materials. On the other hand, orbital angular momentum of light with helical phase distribution…

Optics · Physics 2017-08-02 Xiaodong Chen , Min Chen , Jianwen Dong

In multivalley systems, the valley pseudospin offers rich physics going from encoding of information by its polarization (valleytronics), to exploring novel phases of matter when its degeneracy is changed. Here, by strain engineering, we…

The nonlinear processes of frequency conversion like second harmonic generation (SHG) usually obey certain selection rules, resulting from the preservation of different kind of physical quantities, e.g., the angular momentum. For SHG…

Optics · Physics 2020-04-09 Florian Spreyer , Ruizhe Zhao , Lingling Huang , Thomas Zentgraf

We theoretically introduce the fundamentally fastest induction of a significant population and valley polarization in a monolayer of a transition metal dichalcogenide (i.e., $\mathrm{MoS_2}$ and $\mathrm{WS_2}$). This may be extended to…

Mesoscale and Nanoscale Physics · Physics 2018-08-22 S. Azar Oliaei Motlagh , Jhih-Sheng Wu , Vadym Apalkov , Mark I. Stockman

Valley-contrasting Hall transport conventionally relies on the inversion symmetry breaking in two-dimensional systems, which greatly limits the selection range of valley materials. In particular, while monolayer transition metal…

Mesoscale and Nanoscale Physics · Physics 2024-12-30 Zhichao Zhou , Ruijing Fang , Zhen Zhang , Xiaoyu Wang , Jiayan Rong , Xiao Li

The nonlinear optical behavior of quantum systems plays a crucial role in various photonic applications. This study introduces a novel framework for understanding these nonlinear effects by incorporating gauge-covariant formulations based…

General Physics · Physics 2025-03-11 Jingxu Wu , Chenjia Li
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