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Time evolution of quantum systems is of interest in physics, in chemistry, and, more recently, in computer science. Quantum computers are suggested as one route to propagating quantum systems far more efficiently than ordinary numerical…

Quantum Physics · Physics 2015-02-13 James Daniel Whitfield

We present high-precision quantum computing simulations of three-body atoms (He, H$^-$) and molecules (H$_2^+$, HD$^+$), the latter being studied beyond the Born-Oppenheimer approximation. The Non-Iterative Disentangled Unitary Coupled…

Quantum Physics · Physics 2025-10-22 Mohammad Haidar , Hugo D. Nogueira , J. -Ph. Karr

We present a cascaded variational quantum eigensolver algorithm that only requires the execution of a set of quantum circuits once rather than at every iteration during the parameter optimization process, thereby increasing the…

Quantum Physics · Physics 2024-03-11 Daniel Gunlycke , C. Stephen Hellberg , John P. T. Stenger

We introduce a parallel, GPU-accelerated implementation of the iterative qubit coupled cluster (iQCC) method that overcomes the exponential growth of the transformed Hamiltonian -- the principal bottleneck for classical emulation of quantum…

Quantum Physics · Physics 2026-03-11 Seyyed Mehdi Hosseini Jenab , Brandon Henderson , Scott N. Genin

We introduce an architecture for neural quantum states for many-body quantum-mechanical systems, based on normalizing flows. The use of normalizing flows enables efficient uncorrelated sampling of configurations from the probability…

Quantum Physics · Physics 2024-06-05 Scott Lawrence , Arlee Shelby , Yukari Yamauchi

In this paper, we have developed a unitary variant of a double exponential coupled cluster theory, which is capable of mimicking the effects of connected excitations of arbitrarily high rank, using only rank-one and rank-two parametrization…

Chemical Physics · Physics 2022-11-23 Dipanjali Halder , V. S. Prasannaa , Rahul Maitra

Quantum cloud computing (QCC) offers a promising approach to efficiently provide quantum computing resources, such as quantum computers, to perform resource-intensive tasks. Like traditional cloud computing platforms, QCC providers can…

Quantum Physics · Physics 2023-07-26 Rakpong Kaewpuang , Minrui Xu , Dinh Thai Hoang , Dusit Niyato , Han Yu , Ruidong Li , Zehui Xiong , Jiawen Kang

The development of tailored materials for specific applications is an active field of research in chemistry, material science and drug discovery. The number of possible molecules that can be obtained from a set of atomic species grow…

We present a quantum algorithm for computational fluid dynamics based on the Lattice-Boltzmann method. Our approach involves a novel encoding strategy and a modified collision operator, assuming full relaxation to the local equilibrium…

The iterative qubit coupled cluster (iQCC) method is a systematic variational approach to solve the electronic structure problem on universal quantum computers. It is able to use arbitrarily shallow quantum circuits at expense of iterative…

Quantum Physics · Physics 2020-09-30 Ilya G. Ryabinkin , Artur F. Izmaylov , Scott N. Genin

We recently proposed a novel approach to converging electronic energies equivalent to high-level coupled-cluster (CC) computations by combining the deterministic CC($P$;$Q$) formalism with the stochastic configuration interaction (CI) and…

Chemical Physics · Physics 2021-03-23 J. Emiliano Deustua , Jun Shen , Piotr Piecuch

The increasing growth of data volume, and the consequent explosion in demand for computational power, are affecting scientific computing, as shown by the rise of extreme data scientific workflows. As the need for computing power increases,…

Emerging Technologies · Computer Science 2024-04-17 Sandeep Suresh Cranganore , Vincenzo De Maio , Ivona Brandic , Ewa Deelman

We employ the principle of minimum pressure gradient to transform problems in unsteady computational fluid dynamics (CFD) into a convex optimization framework subject to linear constraints. This formulation permits solving, for the first…

Fluid Dynamics · Physics 2025-01-15 Hussam Sababha , Haithem Taha , Mohammed Daqaq

A novel parallel hybrid quantum-classical algorithm for the solution of the quantum-chemical ground-state energy problem on gate-based quantum computers is presented. This approach is based on the reduced density-matrix functional theory…

In measurement-based quantum computing (MBQC), computation is carried out by a sequence of measurements and corrections on an entangled state. Flow, and related concepts, are powerful techniques for characterising the dependence of the…

Quantum Physics · Physics 2023-03-13 Robert I. Booth , Aleks Kissinger , Damian Markham , Clément Meignant , Simon Perdrix

Quantum computers hold immense potential in the field of chemistry, ushering new frontiers to solve complex many body problems that are beyond the reach of classical computers. However, noise in the current quantum hardware limits their…

Quantum Physics · Physics 2024-03-20 Chayan Patra , Sonaldeep Halder , Rahul Maitra

Molecular ground-state simulation is one of the most promising fields for demonstrating practical quantum advantage on near-term quantum computers. However, the Variational Quantum Eigensolver (VQE), a leading algorithm for this task, still…

Quantum Physics · Physics 2025-07-08 Runhong He , Qiaozhen Chai , Xin Hong , Ji Guan , Guolong Cui , Shengbin Wang , Shenggang Ying

Optimizing the properties of molecules (materials or drugs) for stronger toughness, lower toxicity, or better bioavailability has been a long-standing challenge. In this context, we propose a molecular optimization framework called Q-Drug…

Quantum Physics · Physics 2023-08-28 Zhaoping Xiong , Xiaopeng Cui , Xinyuan Lin , Feixiao Ren , Bowen Liu , Yunting Li , Manhong Yung , Nan Qiao

We present a novel combination of numerical techniques to improve the efficiency, accuracy, and robustness of multi-component compressible flow simulations. At the core of our approach is an Entropy-Stable formulation that preserves kinetic…

Computational Engineering, Finance, and Science · Computer Science 2025-06-17 Vahid Badrkhani , T. Jeremy P. Karpowsk , Christian Hasse

Quantum power flow (QPF) provides inspiring directions for tackling power flow's computational burdens leveraging quantum computing. However, existing QPF methods are mainly based on noise-sensitive quantum algorithms, whose practical…

Quantum Physics · Physics 2022-11-22 Fei Feng , Yifan Zhou , Peng Zhang