Related papers: Plasmon Induced Delocalized Second-Harmonic Genera…
We report a systematic investigation into the processes behind a near hundredfold enhanced second harmonic wave generated from a laser-induced air plasma, by examining the temporal dynamics of the frequency conversion processes, and the…
We investigate optical second-harmonic generation (SHG) from metasurfaces where noncentrosymmetric V-shaped gold nanoparticles are ordered into regular array configurations. In contrast to expectations, a substantial enhancement of the SHG…
Monolayer transition metal dichalcogenides, coupled to metal plasmonic nanocavities, have recently emerged as new platforms for strong light-matter interactions. These systems are expected to have nonlinear optical properties that will…
The generation process of second harmonic (SH) radiation from holes periodically arranged on a metal surface is investigated. Three main modulating factors affecting the optical response are identified: the near-field distribution at the…
Nonlinear second harmonic optical activity of graphene covering a gold photon sieve was determined for different polarizations. The photon sieve consists of a subwavelength gold nanohole array placed on glass. It combines the benefits of…
The ability to engineer localized surface plasmon resonances at large scale usually relies on precise nanoscale patterning. Here, we demonstrate that mid-infrared plasmonic responses can instead emerge in unpatterned polysilicon films…
We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…
Plasmonic nanocavities have proven to be a powerful optical platform for confining light at a length scale much smaller than the diffraction limit. Enhanced electromagnetic fields within the cavity mode volume enable multiple significant…
We analytically investigate the effect of a non-centrosymmetric geometry in the optical second harmonic (SH) generation from a particle made of a centrosymmetric material, in the interior of which quadratic optical processes are suppressed.…
Second harmonic generation is a powerful tool directly connected to the symmetry of materials. Phase transitions, lattice rotations or electromagnetic coupling in multiferroic compounds can be revealed by using second harmonic…
We show that the lack of inversion symmetry in monolayer MoS2 allows strong optical second harmonic generation. Second harmonic of an 810-nm pulse is generated in a mechanically exfoliated monolayer, with a nonlinear susceptibility on the…
We theoretically show the existence of cascaded second-order surface plasmon solitons propagating at the interface between metal and linear dielectric. Nonlocal multipole nonlinearities originating from free conduction electron plasma of a…
Single surface plasmon polaritons are excited using photons generated via spontaneous parametric down-conversion. The mean excitation rates, intensity correlations and Fock state populations are studied. The observed dependence of the…
Digital holography is an interference-based imaging technique capable of recording both the amplitude and phase of an electromagnetic field. It can be obtained at the laser illumination wavelength, but also with second-harmonic generation,…
The excitation of localized or delocalized surface plasmon polaritons in nanostructured or extended graphene has attracted a steadily increasing attention due to their promising applications in sensors, switches, and filters. These single…
Since de discovery of graphene, the family of 2-dimensional materials has attracted much recent attention. In this work, the nonlinear optical properties of few-layer MoS2 two-dimensional crystals are studied using femtosecond laser pulses.…
We investigate Second Harmonic Generation from individual silicon nanowires and study the influence of resonant optical modes on the far-field nonlinear emission. We find that the polarization of the Second Harmonic has a size-dependent…
The plasmon-enhanced second harmonic generation in the subwavelength neutral metal cubic nanoparticles is calculated for the first time in the hydrodynamic and cold plasma approximations. The theory is developed that takes into account all…
The injection of a beam of free 50 keV electrons into an unstructured gold surface creates a highly localized source of traveling surface plasmons with spectrum centered around 1.8 eV. The plasmons were detected by a controlled decoupling…
We aim to clarify the role that absorption plays in nonlinear optical processes in a variety of metallic nanostructures and show how it relates to emission and conversion efficiency. We define a figure of merit that establishes the…