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High harmonic generation (HHG) has developed in recent years as a promising tool for ultrafast materials spectroscopy. At the forefront of these advancements, several works proposed to use HHG as an all-optical probe for topology of quantum…

Topological insulators with unique gapless edge states have revolutionized the understanding of electronic properties in solid materials. These gapless edge states are dictated by the topological invariants associated with the quantization…

Mesoscale and Nanoscale Physics · Physics 2019-06-05 Xiujuan Zhang , Hai-Xiao Wang , Zhi-Kang Lin , Yuan Tian , Biye Xie , Ming-Hui Lu , Yan-Feng Chen , Jian-Hua Jiang

Efficient nonlinear wave mixing is of paramount importance for a wide range of applications. However, weak optical nonlinearities pose significant challenges for accessing nonlinear light-matter interaction in compact systems. Here, we…

Toroidal vortex is a kind of novel and exotic structured light with potential applications in photonic topology and quantum information. Here, we present the study on high harmonic generation (HHG) from the interaction of the intense…

Optics · Physics 2024-10-10 Zijian Lyu , Yiqi Fang , Yunquan Liu

Van der Waals stacking presents new opportunities for nonlinear optics with its remarkable tunability and scalability. However, the fundamental role of interlayer interactions in modifying the overall nonlinear optical susceptibilities…

Materials Science · Physics 2026-03-11 Kanchan Shaikh , Taejun Yoo , Zeyuan Zhu , Qiuyang Li , Amalya C. Johnson , Hui Deng , Fang Liu , Yuki Kobayashi

Time-varying metamaterials rely on large and fast changes of the linear permittivity. Beyond the linear terms, however, the effect of a non-perturbative modulation of the medium on harmonic generation and the associated nonlinear…

Second harmonic generation has been applied to study lattice, electronic and magnetic proprieties in atomically thin materials. However, inversion symmetry breaking is usually required for the materials to generate a large signal. In this…

Materials Science · Physics 2022-05-12 Zhuoliang Ni , Nan Huang , Amanda V. Haglund , David G. Mandrus , Liang Wu

Nonlinear optical phenomena are at the heart of various technological domains such as high-speed data transfer, optical logic applications, and emerging fields such as non-reciprocal optics and photonic time crystal design. However,…

We report a coherent layer-by-layer high-order harmonic generation (HHG) build-up in artificially stacked transition metal dichalcogenides (TMDC) crystals in their various stacking configurations. In the experiments, millimeter-sized single…

We investigate the high harmonic generation (HHG) from solids by simulating the dynamics of a single active electron in periodic potentials. The corresponding time-dependent Schr\"odinger equations (TDSE) are solved numerically by using…

Atomic Physics · Physics 2016-03-31 Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

We study nonlinear effects in two-dimensional photonic metasurfaces supporting topologically-protected helical edge states at the nanoscale. We observe strong third-harmonic generation mediated by optical nonlinearities boosted by…

We investigate theoretically the strong-field regime of light-matter interactions in the topological-insulator class of quantum materials. In particular, we focus on the process of non-perturbative high-order harmonic generation from the…

Mesoscale and Nanoscale Physics · Physics 2022-01-24 Denitsa Baykusheva , Alexis Chacón , Dasol Kim , Dong Eon Kim , David A. Reis , Shambhu Ghimire

Optical modulation of high-harmonics generation in solids enables the detection of material properties such as the band structure and promising new applications such as super-resolution imaging in semiconductors. Various recent studies have…

We present a combined experimental and theoretical study of enhanced third-harmonic generation (THG) in silicon nitride metasurfaces. These structures exhibit strong resonant nonlinear responses, enabling up to two orders of magnitude…

High harmonic generation (HHG) in solids has emerged as a powerful spectroscopic method for resolving ultrafast electron dynamics and band structure properties across a wide range of materials. However, quantitative HHG studies require…

Optics · Physics 2025-12-16 S. Mandal , P. Kumar , Z. Pi , H. Y. Kim , M. Zhan , E. Goulielmakis

We investigate high-order harmonic generation (HHG) in graphene with a quantum master equation approach. The simulations reproduce the observed enhancement in HHG in graphene under elliptically polarized light [N. Yoshikawa et al, Science…

Materials Science · Physics 2021-02-03 Shunsuke A. Sato , Hideki Hirori , Yasuyuki Sanari , Yoshihiko Kanemitsu , Angel Rubio

Improving the conversion efficiency is critical for advancing nonlinear photonic devices, enabling applications in ultrafast optics, quantum light sources, and high-resolution imaging. Herein, we present a bilayer waveguide integrated with…

Optics · Physics 2025-08-21 Xin Huang , Qi Lin , Sheng-Xuan Xia , Xiang Zhai , Gui-Dong Liu

High-harmonic spectroscopy in solids gives insight into the inner workings of solids, such as reconstructing band structures or probing the topological phase of materials. High-harmonic generation (HHG) is a highly non-linear phenomena and…

Quantum Physics · Physics 2025-12-16 Asger Weeth , Lars Bojer Madsen

We develop a general theory of high-harmonic generation (HHG) in solid-state systems, based on a weak-correlation expansion of photonic and matter degrees of freedom. Unlike standard HHG theories, which treat light-matter dynamics through…

Mesoscale and Nanoscale Physics · Physics 2026-04-23 Denis Ilin , Alexander S. Solntsev , Ivan Iorsh

High-order harmonic generation (HHG) is a fundamental process which can be simplified as the production of high energetic photons from a material subjected to a strong driving laser field. This highly nonlinear optical process contains rich…

Optics · Physics 2021-12-21 Dasol Kim , Yeon Lee , Alexis Chacón , Dong Eon Kim