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Second-harmonic generation is of paramount importance in several fields of science and technology, including frequency conversion, self-referencing of frequency combs, nonlinear spectroscopy and pulse characterization. Advanced…

We report comparative experimental and theoretical studies of second and third harmonic generation from a 20nm-thick indium tin oxide layer in proximity of the epsilon-near-zero condition. Using a tunable OPA laser we record both spectral…

We demonstrate and explore an all-optical technique for direct monitoring the orientation dynamics of gas phase molecular ensembles. The technique termed 'MOISH' utilizes the transiently lifted inversion symmetry of polar gas media and…

Chemical Physics · Physics 2022-10-12 Amit Beer , Ran Damari , Yun Chen , Sharly Fleischer

High harmonic generation by relativistically intense laser pulses from overdense plasma layers is surveyed. High harmonics are generated in form of (sub-)attosecond pulses when the plasma surface rebounds towards the observer with…

Plasma Physics · Physics 2011-11-18 Daniel an der Brügge , Alexander Pukhov

An intense femtosecond laser pulse can generate ultraviolet air lasing, offering a promising remote light source. A long-standing hypothesis is whether it is seeded by a self-generated spectral component, such as the second harmonic that is…

Atomic Physics · Physics 2026-02-20 Jingsong Gao , Yang Wang , Jiahao Dong , Yi Liu , Chengyin Wu , Hongbing Jiang , Meng Han , Yunquan Liu

Nonlinear optical frequency conversion, in which optical fields interact with a nonlinear medium to produce new field frequencies, is ubiquitous in modern photonic systems. However, the nonlinear electric susceptibilities that give rise to…

Mesoscale and Nanoscale Physics · Physics 2015-04-22 Kyle L. Seyler , John R. Schaibley , Pu Gong , Pasqual Rivera , Aaron M. Jones , Sanfeng Wu , Jiaqiang Yan , David G. Mandrus , Wang Yao , Xiaodong Xu

Generation of second-harmonic waves is one of the universal nonlinear phenomena that have found numerous technical applications in many modern technologies, in particular, in photonics. This phenomenon also has great potential in the field…

Mesoscale and Nanoscale Physics · Physics 2024-03-01 K. O. Nikolaev , S. R. Lake , G. Schmidt , S. O. Demokritov , V. E. Demidov

High-order harmonic generation by the diffraction of an intense Laguerre-Gaussian (LG) laser beam through a small aperture is studied. It is found that the 2D peripheral electron dynamics on the rim can facilitate complex interplay between…

Plasma Physics · Physics 2025-06-27 Yao Meng , Runze Li , Longqing Yi

We investigate laser-induced nonsequential double ionization with linearly polarized bichromatic fields, focusing on the recollision-excitation with subsequent ionization (RESI) mechanism. Using the strong-field approximation, we assess how…

Atomic Physics · Physics 2025-08-06 S. Hashim , D. Habibović , C. Figueira de Morisson Faria

We use ultrafast laser pulses to experimentally demonstrate that the second-order optical response of bulk single crystals of the topological insulator Bi$_2$Se$_3$ is sensitive to its surface electrons. By performing surface doping…

Materials Science · Physics 2011-02-02 D. Hsieh , J. W. McIver , D. H. Torchinsky , D. R. Gardner , Y. S. Lee , N. Gedik

We study second and third harmonic generation in centrosymmetric semiconductors at visible and UV wavelengths in bulk and cavity environments. Second harmonic generation is due to a combination of symmetry breaking, the magnetic portion of…

We report the observation of optical second harmonic generation (SHG) in single-layer indium selenide (InSe). We measure a second harmonic signal of $>10^3$ $\textrm{cts/s}$ under nonresonant excitation using a home-built confocal…

Dynamical control of the nonlinear optical properties of solids -- with light itself -- will be essential for future ultrafast photonic technologies. Previously, methods to modulate nonlinear processes including second-harmonic generation…

Second harmonic generation is enhanced at the surface lattice resonance in plasmonic nanoparticle arrays. We carried out a parametric investigation on two-dimensional lattices composed of gold nanobars where the centrosymmetry is broken at…

The harmonic generation has always been of fundamental interest in studying the nonlinear nature of any physical system. In the present study, Particle - In - Cell (PIC) simulations have been carried out to explore the harmonic generation…

Plasma Physics · Physics 2023-07-12 Trishul Dhalia , Rohit Juneja , Laxman Prasad Goswami , Srimanta Maity , Amita Das

Here we experimentally map the dynamics of electron plasma waves in laser solid interaction. We do time resolved measurements of second harmonic and hard X-ray generation from interaction of intense ($10^{16} W cm^{-2}$, 100 fs, 800nm)…

Plasma Physics · Physics 2007-05-23 Arvinder S. Sandhu , G. Ravindra Kumar , S. Sengupta , A. Das , P. K. Kaw

Second-harmonic generation in resonant structures is commonly evaluated in terms of intracavity field enhancement at the fundamental and harmonic frequencies. Here, we formulate nonlinear frequency conversion within a symmetry-resolved…

We study the second-harmonic generation in left-handed metamaterials with a quadratic nonlinear response. We demonstrate a novel type of the exact phase matching between the backward propagating wave of the fundamental frequency and the…

Optics · Physics 2009-11-11 Ilya V. Shadrivov , Alexander A. Zharov , Yuri S. Kivshar

Vector beams with spatially structured polarization and intertwined spin-orbital angular momentum (SAM-OAM) provide powerful degrees of freedom for tailoring light-matter interactions. While such structured beams are well established in the…

We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…