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Heralded multi-photon entanglement generation is a central bottleneck for photonic quantum computing, where resource costs typically skyrocket with target size. We explore efficient methods for generating photon states with tunable…

Quantum Physics · Physics 2025-11-10 Suren A. Fldzhyan , Stanislav S. Straupe , Mikhail Yu. Saygin

We use extreme-ultraviolet interferometry to measure the phase of high-order harmonic generation from transiently aligned CO2 molecules. We unambiguously observe a reversal in phase of the high order harmonic emission for higher harmonic…

Atomic Physics · Physics 2009-11-13 Xibin Zhou , Robynne Lock , Wen Li , Nick Wagner , Margaret. M. Murnane , Henry C. Kapteyn

High-order harmonic generation by femtosecond laser pulse in the presence of a moderately strong terahertz (THz) field is studied under the strong field approximation, showing a simple proportionality of near-cutoff even-order harmonic…

Optics · Physics 2020-12-07 Bing-Yu Li , Yizhu Zhang , Tian-Min Yan , Y. H. Jiang

High harmonic generation (HHG) in solids has recently emerged as a powerful all-optical approach for probing material properties and ultrafast electron dynamics in quantum systems. It has been widely applied for studying two-dimensional and…

Optics · Physics 2026-04-28 Eyal Uzner , Ofer Neufeld

We show that a single, trapped, laser-driven atom in a high-finesse optical cavity allows for the quantum-coherent generation of entangled light pulses on demand. Schemes for generating simultaneous and temporally separated pulse pairs are…

Quantum Physics · Physics 2009-11-11 Giovanna Morigi , Jürgen Eschner , Stefano Mancini , David Vitali

The cut-off regime of high-order harmonic generation (HHG) by atoms in an intense laser field is studied numerically and analytically. We find that the cut-off regime is characterized by equal dephasing between the successive harmonics. The…

Atomic Physics · Physics 2016-04-27 M. A. Khokhlova , V. V. Strelkov

The atomic response to an ultra-intense driving field produces a characteristic high-harmonic spectrum featuring a rapid drop in intensity for the lower harmonics, followed by a plateau and a sharp cutoff. This response vanishes for…

Quantum Physics · Physics 2026-01-06 Lidija Petrovic , Philipp Stammer , Maciej Lewenstein , Javier Rivera-Dean

We introduce and demonstrate a new approach to measuring coherent electron wave packets using high-harmonic spectroscopy. By preparing a molecule in a coherent superposition of electronic states, we show that electronic coherence opens…

Chemical Physics · Physics 2014-07-09 P. M. Kraus , S. B. Zhang , A. Gijsbertsen , R. R. Lucchese , N. Rohringer , H. J. Wörner

A theory of ultra-fast pump-probe experiments proposed by us earlier [F.H.M. Faisal et al., Phys. Rev. Lett. 98, 143001 (2007) and F.H.M. Faisal and A. Abdurrouf, Phys. Rev. Lett. 100, 123005 (2008)] is developed here fully and applied to…

Atomic and Molecular Clusters · Physics 2009-11-13 A. Abdurrouf , F. H. M. Faisal

We produce oriented rotational wave packets in CO and measure their characteristics via high harmonic generation. The wavepacket is created using an intense, femtosecond laser pulse and its second harmonic. A delayed 800 nm pulse probes the…

The tunnelling of an electron through a suppressed atomic potential followed by its motion in the continuum, is the fundamental mechanism underlying strong-field laser-atom/molecule interactions. Due to its quantum nature, the interaction…

The production of brighter coherent XUV radiation by intense laser pulses through the process of high-harmonic generation (HHG) is a central challenge in contemporary nonlinear optics. We study the generation and spatial propagation of high…

Optics · Physics 2025-06-03 Margarita Khokhlova , Vasily Strelkov

Since the new millennium coherent extreme ultra-violet and soft x-ray radiation has revolutionized the understanding of dynamical physical, chemical and biological systems at the electron's natural timescale. Unfortunately, coherent…

High-harmonic generation (HHG), an extreme nonlinear effect, introduces an unprecedented paradigm to detect emergent quantum phases and electron dynamics inconceivable in the framework of linear and low-order nonlinear processes. As an…

The generation of high-order harmonics in bulk solids subjected to intense ultrashort laser pulses has opened up new avenues for research in extreme nonlinear optics and light-matter interaction on sub-cycle timescales. Despite significant…

Lasers provide intense coherent radiation, essential to cool and trap atoms into a Bose-Einstein condensate or can alternatively drive the non-linear dynamics of high-order harmonic generation. Yet, these two fundamental processes remained…

Quantum Physics · Physics 2025-10-14 Philipp Stammer

The generation of high harmonics (HHG) in atomic systems by the highly non-linear response to an intense laser field is a prominent pathway to the synthesis of ever shorter laser pulses at increasingly higher photon energies. Extensions of…

Atomic Physics · Physics 2022-11-23 Mohammad Monfared , Elnaz Irani , Christoph Lemell , Joachim Burgdörfer

Emerging technologies that employ quantum physics offer fundamental enhancements in information processing tasks, including sensing, communications, and computing. Here, we introduce the quantum phased array, which generalizes the operating…

Quantum Physics · Physics 2024-06-14 Volkan Gurses , Samantha I. Davis , Neil Sinclair , Maria Spiropulu , Ali Hajimiri

In the realm of open quantum systems, steady states and high-harmonic generation (HHG) existing far from equilibrium have become core pillars of ultrafast science. Most solid-state research explores charge HHG with limited investigations…

Strongly Correlated Electrons · Physics 2024-08-20 Negin Moharrami Allafi , Michael H. Kolodrubetz , Marin Bukov , Vadim Oganesyan , Mohsen Yarmohammadi

We demonstrate a coherent imaging system based on a terahertz (THz) frequency quantum cascade laser (QCL) phase-locked to a near-infrared fs-laser comb. The phase locking enables coherent electro-optic sampling of the continuous-wave…