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Interferometric scattering microscopy has been a very promising technology for highly sensitive label-free imaging of a broad spectrum of biological nanoparticles from proteins to viruses in a high-throughput manner. Although it can reveal…

Optics · Physics 2021-08-11 Celalettin Yurdakul , Haonan Zong , Yeran Bai , Ji-Xin Cheng , M. Selim Unlu

We study effects of electron-electron interactions and confinement potential on the magneto-optical absorption spectrum in the far-infrared range of lateral quantum dot molecules. We calculate far-infrared (FIR) spectra for three different…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. Helle , A. Harju , R. M. Nieminen

Infrared (IR) spectroscopy can be used as an important and effective tool for probing periodic networks of quantum wires or nanotubes (quantum crossbars, QCB) at finite frequencies far from the Luttinger liquid fixed point. Plasmon…

Strongly Correlated Electrons · Physics 2009-11-10 I. Kuzmenko , S. Gredeskul , K. Kikoin , Y. Avishai

We present an interferometric pump-probe technique for the characterization of attosecond electron wave packets (WPs) that uses a free WP as a reference to measure a bound WP. We demonstrate our method by exciting helium atoms using an…

Upon absorbing a photon, the ionized electron sails through the target force field in attoseconds to reach free space. This navigation probes details of the potential landscape that get imprinted into the phase of the ionization amplitude.…

Atomic Physics · Physics 2024-12-12 Sajad Azizi , Mohamed El-Amine Madjet , Zheng Li , Jan M. Rost , Himadri S. Chakraborty

Ultraintense pulses from X-ray free-electron lasers can drive, within femtoseconds, multiple processes in the inner shells of atoms and molecules in all phases of matter. The ensuing complex ionization pathways of outer-shell electrons from…

We study the effects of electron-electron correlations and confinement potential on the far-infrared spectrum of a lateral two-electron quantum dot molecule by exact diagonalization. The calculated spectra directly reflect the lowered…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. Marlo , A. Harju , R. M. Nieminen

We propose a new technique to fully characterize the temporal structure of extreme ultraviolet pulses by ionizing a bound coherent electronic wavepacket. The populated energy levels make it possible to interfere different spectral…

Optics · Physics 2016-07-19 Stefan Pabst , Jan Marcus Dahlström

Mapping equations of motion of the highly exited classical atom in a monochromatic field are generalized for the two-frequency microwave field. Analysis of the obtained equations indicates to the weak sensitivity of the position of the…

Atomic Physics · Physics 2016-09-08 B. Kaulakys , D. Grauzhinis , G. Vilutis

The electron motion in atoms and molecules is at the heart of all phenomena in nature that occur outside the nucleus. Recently, ultrafast electron and X-ray imaging tools have been developed to image the ultrafast dynamics of matter in real…

We study laser-assisted photoionization by attosecond pulses using a time-independent formalism based on diagrammatic many-body perturbation theory. Our aim is to provide an ab inito route to the "delays" for this above-threshold ionization…

Atomic Physics · Physics 2015-06-12 J. M. Dahlström , T. Carette , E. Lindroth

The screened electron-electron interaction in a multi-band electron system is calculated within the random phase approximation and in the tight-binding representation. The obtained dielectric matrix contains, beside the usual site-site…

Condensed Matter · Physics 2009-10-28 P. Zupanovic , A. Bjelis , S. Barisic

Chiral molecules exhibit enantiosensitive light-matter interactions, with photoelectron circular dichroism (PECD) serving as a sensitive probe of molecular chirality through the asymmetry in the photoelectron wavepacket amplitude. Here, we…

Atomic Physics · Physics 2025-05-07 Zheming Zhou , Yang Li , Xu Zhang , Yueming Zhou , Peixiang Lu

In a double-slit experiment with a bipartite system, the visibility of interference fringes depends on the availability of which-way information. Here, we report the formation of a Bell-like state of photoelectron and residual ion in the…

We demonstrate imaging of ions in an atomic gas with ion-Rydberg atom interaction induced absorption. This is made possible by utilizing a multi-photon electromagnetically induced transparency (EIT) scheme and the extremely large electric…

Atomic Physics · Physics 2023-04-03 Christian Gross , Thibault Vogt , Wenhui Li

We reflect on the prospect of exploiting the recoil associated with absorption and emission of photons to perform spectroscopy of a single molecular ion. For this recoil to be detectable, the molecular ion is sympathetically cooled by a…

The complex Kohn variational method is extended to compute light-driven electronic transitions between continuum wavefunctions in atomic and molecular systems. This development enables the study of multiphoton processes in the perturbative…

Atomic Physics · Physics 2018-08-15 Nicolas Douguet , Barry I. Schneider , Luca Argenti

We study photoionization of argon atoms excited by attosecond pulses using an interferometric measurement technique. We measure the difference in time delays between electrons emitted from the $3s^2$ and from the $3p^6$ shell, at different…

Attosecond physics enables the study of ultrafast coherent electron dynamics in matter upon photoexcitation and photoionization, revealing spectacular effects such as hole migration and coherent Auger dynamics in molecules. In the…

Atomic Physics · Physics 2024-01-15 Marco Ruberti , Vitali Averbukh , Florian Mintert

We present velocity map imaging data on intramolecular ion-pair dissociation (IPD) of carbonyl sulfide (OCS) induced by electron impact over the 20 eV to 45 eV energy range. Two distinct IPD pathways were resolved: CO+ + S- (threshold 14.8…

Atomic and Molecular Clusters · Physics 2026-04-21 Narayan Kundu , Soumya Ghosh , Dhananjay Nandi