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We employ ultrabroadband terahertz (THz) spectroscopy to expose the high-frequency transport properties of Dirac fermions in monolayer graphene. By controlling the carrier concentration via tunable electrical gating, both equilibrium and…

Mesoscale and Nanoscale Physics · Physics 2024-10-29 G. Coslovich , R. P. Smith , S. -F. Shi , J. H. Buss , J. T. Robinson , F. Wang , R. A. Kaindl

A non-perturbative model for graphene optical nonlinearity is developed for the study of ultrafast pulse propagation along a monolayer, as in the case of graphene-comprising nanophotonic integrated waveguides. This graphene `hot electron'…

Optics · Physics 2022-03-18 Alexandros Pitilakis , Emmanouil E. Kriezis

Optical harmonic generation occurs when high intensity light ($>10^{10}$W/m$^{2}$) interacts with a nonlinear material. Electrical control of the nonlinear optical response enables applications such as gate-tunable switches and frequency…

Understanding the ultrafast dynamics of photoexcited charges in graphene is essential, as the microscopic mechanisms underlying these dynamics determine many of graphene's optical, optothermal, and optoelectronic properties. These are…

Mesoscale and Nanoscale Physics · Physics 2026-04-02 Hai I. Wang , Xiaoyu Jia , Anand Nivedan , Mischa Bonn , Aron W. Cummings , Alessandro Principi , Klaas-Jan Tielrooij

Graphene is a unique platform for tunable opto-electronic applications thanks to its linear band dispersion, which allows electrical control of resonant light-matter interactions. Tuning the nonlinear optical response of graphene is…

Materials with massless Dirac fermions can possess exceptionally strong and widely tunable optical nonlinearities. Experiments on graphene monolayer have indeed found very large third-order nonlinear responses, but the reported variation of…

Graphene is emerging as a viable alternative to conventional optoelectronic, plasmonic, and nanophotonic materials. The interaction of light with carriers creates an out-of-equilibrium distribution, which relaxes on an ultrafast timescale…

Mesoscale and Nanoscale Physics · Physics 2013-06-25 D. Brida , A. Tomadin , C. Manzoni , Y. J. Kim , A. Lombardo , S. Milana , R. R. Nair , K. S. Novoselov , A. C. Ferrari , G. Cerullo , M. Polini

Two-dimensional materials constitute an exciting platform for nonlinear optics with large nonlinearities that are tunable by gating. Hence, gate-tunable harmonic generation and intensity-dependent refraction have been observed in e.g.…

Mesoscale and Nanoscale Physics · Physics 2019-05-15 F. Hipolito , Darko Dimitrovski , T. G. Pedersen

The ability to tune the optical response of a material via electrostatic gating is crucial for optoelectronic applications, such as electro-optic modulators, saturable absorbers, optical limiters, photodetectors and transparent electrodes.…

Graphene is an ideal material to study fundamental Coulomb- and phonon-induced carrier scattering processes. Its remarkable gapless and linear band structure opens up new carrier relaxation channels. In particular, Auger scattering bridging…

We describe very fast electron dynamics for a graphene nanoribbon driven by a control electromagnetic field in the terahertz regime. The mobility as a function of bias possesses a large threshold value when entering a nonlinear transport…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 Danhong Huang , Godfrey Gumbs , O. Roslyak

Hot electron effects in graphene are significant because of graphene's small electronic heat capacity and weak electron-phonon coupling, yet the dynamics and cooling mechanisms of hot electrons in graphene are not completely understood. We…

Graphene is conceivably the most nonlinear optoelectronic material. Its nonlinear optical coefficients in the terahertz (THz) frequency range surpass those of other materials by many orders of magnitude. This, in particular, allows one to…

For many of the envisioned optoelectronic applications of graphene it is crucial to understand the sub-picosecond carrier dynamics immediately following photoexcitation, as well as the effect on the electrical conductivity - the…

The transient evolution of carriers in an intrinsic graphene under ultrafast excitation, which is caused by the collisionless interband transitions, is studied theoretically. The energy relaxation due to the quasielastic acoustic phonon…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 P. N. Romanets , F. T. Vasko

Graphene is a promising material for nonlinear THz applications owing to its high third-order susceptibility and tunable optical properties. Its strong nonlinear response, driven by free-carrier thermodynamics, facilitates efficient…

The equilibrium optical phonons of graphene are well characterized in terms of anharmonicity and electron-phonon interactions, however their non-equilibrium properties in the presence of hot charge carriers are still not fully explored.…

Mesoscale and Nanoscale Physics · Physics 2018-02-15 C. Ferrante , A. Virga , L. Benfatto , M. Martinati , D. De Fazio , U. Sassi , C. Fasolato , A. K. Ott , P. Postorino , D. Yoon , G. Cerullo , F. Mauri , A. C. Ferrari , T. Scopigno

The temporal dynamics of charge carriers determines the speed with which electronics can be realized in condensed matter, and their direct manipulation with optical fields promises electronic processing at unprecedented petahertz…

Graphene has recently been shown to possess giant nonlinearity; however, the utility of this nonlinearity is limited due to high losses and small interaction volume. We show that by performing waveguide engineering to graphene's…

Mesoscale and Nanoscale Physics · Physics 2014-11-19 Kelvin J. A. Ooi , Lay Kee Ang , Dawn T. H. Tan

Exploration of optical non-linear response of graphene predominantly relies on ultra-short time domain measurements. Here we propose an alternate technique that uses frequency modulated continuous wavefront optical fields, thereby probing…

Mesoscale and Nanoscale Physics · Physics 2019-03-18 Ashutosh Singh , Saikat Ghosh , Amit Agarwal
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