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We demonstrate that ultrashort pulses carry the possibility for a new regime of light-matter interaction with nonadiabatic electron processes sensitive to the envelope-derivative of the light pulse. A standard single pulse with its two…

Optics · Physics 2018-02-21 Qi-Cheng Ning , Ulf Saalmann , Jan M. Rost

We outline an approach that streamlines considerably the construction and analysis of well-behaved nonlinear quantum dynamics, with completely positive extensions to entangled systems. A few notes are added on the issue of quantum…

Quantum Physics · Physics 2007-05-23 S. Gheorghiu-Svirschevski

Simulating nonlinear classical dynamics on a quantum computer is an inherently challenging task due to the linear operator formulation of quantum mechanics. In this work, we provide a systematic approach to alleviate this difficulty by…

In these four lectures I describe basic ideas and methods applicable to both classical and quantum systems displaying slow relaxation and non-equilibrium dynamics. The first half of these notes considers classical systems, and the second…

Statistical Mechanics · Physics 2018-05-30 Juan P. Garrahan

Boson Sampling is a task that is conjectured to be computationally hard for a classical computer, but which can be efficiently solved by linear-optical interferometers with Fock state inputs. Significant advances have been reported in the…

Quantum Physics · Physics 2023-04-14 Nicolò Spagnolo , Daniel J. Brod , Ernesto F. Galvão , Fabio Sciarrino

The quantum-classical Liouville equation describes the dynamics of a quantum subsystem coupled to a classical environment. It has been simulated using various methods, notably, surface-hopping schemes. A representation of this equation in…

Other Condensed Matter · Physics 2010-11-17 Hyojoon Kim , Ali Nassimi , Raymond Kapral

We consider a system of N non-relativistic spinless quantum particles (``electrons'') interacting with a quantized scalar Bose field (whose excitations we call ``photons''). We examine the case when the velocity v of the electrons is small…

Mathematical Physics · Physics 2008-11-26 L. Tenuta , S. Teufel

Nonlinear Optical Spectroscopy is a well-developed field with theoretical and experimental advances that have aided multiple fields including chemistry, biology and physics. However, accurate quantum dynamical simulations based on model…

Quantum Physics · Physics 2023-12-19 S. A. Shah , Hao Li , Eric R. Bittner , Carlos Silva , Andrei Piryatinski

We give a mathematical framework to describe the evolution of an open quantum systems subjected to finitely many interactions with classical apparatuses. The systems in question may be composed of distinct, spatially separated subsystems…

General Relativity and Quantum Cosmology · Physics 2007-05-23 R. Blute , I. T. Ivanov , P. Panangaden

Ab initio methods for electronic structure of molecules have reached a satisfactory accuracy for calculation of static properties, but remain too expensive for quantum dynamical calculations. We propose an efficient semiclassical method for…

Chemical Physics · Physics 2015-05-13 Baiqing Li , Cesare Mollica , Jiri Vanicek

We give new evidence that quantum computers -- moreover, rudimentary quantum computers built entirely out of linear-optical elements -- cannot be efficiently simulated by classical computers. In particular, we define a model of computation…

Quantum Physics · Physics 2010-11-16 Scott Aaronson , Alex Arkhipov

Ideally, strong non-linearities could be used to implement quantum gates for photonic qubits by well controlled two photon interactions. However, the dependence of the non-linear interaction on frequency and time makes it difficult to…

Quantum Physics · Physics 2009-08-11 Holger F. Hofmann , Hitoshi Nishitani

Quantum systems with a non-conserved probability can be described by means of non-Hermitian Hamiltonians and non-unitary dynamics. In this paper, the case in which the degrees of freedom can be partitioned in two subsets with light and…

Quantum Physics · Physics 2016-10-21 Alessandro Sergi

Achieving high-fidelity control of quantum systems is essential for realization of a practical quantum computer. Composite pulse sequences which suppress different types of errors can be nested to suppress a wide variety of errors but the…

Mesoscale and Nanoscale Physics · Physics 2019-12-09 Utkan Güngördü , J. P. Kestner

We develop a framework for identifying nonclassical speedups in systems with polarization, likewise spin degrees of freedom. By confining the dynamics to the manifold of angular momentum coherent states, which act as the classical reference…

Quantum Physics · Physics 2026-03-25 Tim Aßbrock , Jan Sperling , Laura Ares

Inspired by the classical phenomenon of random walk, the concept of quantum walk has emerged recently as a powerful platform for the dynamical simulation of complex quantum systems, entanglement production and universal quantum computation.…

The recent capability to use THz pulses to control the nuclear quantum degrees of freedom in crystals has opened promising avenues for the advanced manipulation of material properties. While numerical approaches exist for studying the time…

Materials Science · Physics 2025-12-04 Francesco Libbi , Boris Kozinsky

We investigate dynamics of atomic and molecular systems exposed to intense, shaped chaotic fields and a weak femtosecond laser pulse theoretically. As a prototype example, the photoionization of a hydrogen atom is considered in detail. The…

Quantum Physics · Physics 2015-05-18 Kamal P Singh , Jan M Rost

In broadband quantum optical systems, nonlinear interactions among a large number of frequency components induce complex dynamics that may defy heuristic analysis. In this work we introduce a perturbative framework for factoring out…

Quantum Physics · Physics 2023-11-08 Chris Gustin , Ryotatsu Yanagimoto , Edwin Ng , Tatsuhiro Onodera , Hideo Mabuchi

Single photons constitute a main platform in quantum science and technology: they carry quantum information over extended distances in the future quantum internet and can be manipulated in advanced photonic circuits enabling scalable…

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