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Theoretical study of the indirect coupling of nuclear spins (qubits) embedded into a mesoscopic ring and in a finite length quantum wire in a magnetic field is presented. It is found that the hyperfine interaction, via the conduction…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Yu. V. Pershin , I. D. Vagner , P. Wyder

Spin-transfer and spin-orbit torques allow controlling magnetic degrees of freedom in various materials and devices. However, while the transfer of angular momenta between electrons has been widely studied, the contribution of nuclear spins…

Mesoscale and Nanoscale Physics · Physics 2023-10-16 Adam B. Cahaya , Alejandro O. Leon , Mohammad H. Fauzi

The use of nuclear spins as physical sensing systems is disadvantaged by their low signal responsivity, particularly when compared to sensing techniques based on electron spins. This primarily results from the small nuclear gyromagnetic…

Scalar couplings between covalently bound nuclear spins are a ubiquitous feature in nuclear magnetic resonance (NMR) experiments, imparting valuable information to NMR spectra regarding molecular structure and conformation. Such couplings…

Chemical Physics · Physics 2011-12-26 Micah Ledbetter , Giacomo Saielli , Alessandro Bagno , Nhan Tran , Michael Romalis

We studied the effect of nuclear-quadrupole interactions on the field-free impulsive alignment of different asymmetric-top molecules. Our analysis is focused on the influence of the hyperfine- and rotational-energy-level structures. These…

Atomic Physics · Physics 2024-08-05 Linda V. Thesing , Andrey Yachmenev , Rosario González-Férez , Jochen Küpper

The nuclear spin--rotation interaction in the hyperfine structure of the hydrogen molecular ion is investigated. The interaction constants are determined and are found to differ in sign and magnitude compared to another theory, but they are…

atom-ph · Physics 2008-02-03 James F. Babb

Molecular nanostructures may constitute the fabric of future quantum technologies, if their degrees of freedom can be fully harnessed. Ideally one might use nuclear spins as low-decoherence qubits and optical excitations for fast…

NMR spin-spin relaxation in solids in strong magnetic fields is normally described only with the help of the secular part of the full spin-spin interaction Hamiltonian. This approximation is associated with the averaging of the spin-spin…

Statistical Mechanics · Physics 2012-09-11 Chahan M. Kropf , Boris V. Fine

We present a theoretical study of the time-dependent laser alignment of molecules taking into account the hyperfine coupling due to nuclear-quadrupole interactions. The coupling of nuclear spins to the overall angular momentum of molecules…

Chemical Physics · Physics 2020-06-18 Linda V. Thesing , Andrey Yachmenev , Rosario González-Férez , Jochen Küpper

Nuclear magnetic resonance (NMR) is particularly relevant for studies of internuclear spin coupling at zero and ultra-low fields (ZULF), where spin-spin interactions dominate over Zeeman ones. Here we report on ZULF NMR in CdTe. In this…

Mesoscale and Nanoscale Physics · Physics 2024-03-27 V. M. Litvyak , P. Bazhin , R. André , M. Vladimirova , K. V. Kavokin

We present the first quantum mechanical study of hyperfine effects in the rotational cluster states of a symmetric triatomic molecule H$_2$S. Rotational clusters arise from spontaneous symmetry breaking induced by high-angular-momentum…

Atomic and Molecular Clusters · Physics 2025-03-27 Andrey Yachmenev , Guang Yang

We review and summarize recent theoretical and experimental work on electron spin dynamics in quantum dots and related nanostructures due to hyperfine interaction with surrounding nuclear spins. This topic is of particular interest with…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 John Schliemann , Alexander Khaetskii , Daniel Loss

We review recent theoretical and experimental advances toward understanding the effects of nuclear spins in confined nanostructures. These systems, which include quantum dots, defect centers, and molecular magnets, are particularly…

Mesoscale and Nanoscale Physics · Physics 2009-09-15 W. A. Coish , J. Baugh

We propose a method to measure the hyperfine vectors between a nitrogen-vacancy (NV) center and an environment of interacting nuclear spins. Our protocol enables the generation of tunable electron-nuclear coupling Hamiltonians while…

Quantum Physics · Physics 2016-05-12 Zhen-Yu Wang , Jan F. Haase , Jorge Casanova , Martin B. Plenio

The interplay of optical driving and hyperfine interaction between an electron confined in a quantum dot and its surrounding nuclear spin environment produces a range of interesting physics such as mode-locking. In this work, we go beyond…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Arian Vezvaee , Gargee Sharma , Sophia E. Economou , Edwin Barnes

Nuclear spins and paramagnetic centers in a solid randomly group to form clusters featuring nearly-degenerate, hybrid states whose dynamics are central to processes involving nuclear spin-lattice relaxation and diffusion. Their…

Nuclear magnetic resonance (NMR) is a powerful tool for applications ranging from chemical analysis to quantum information processing. Achieving optical initialization and detection of molecular nuclear spins promises new opportunities -…

The optically induced polarization of localized electron spins in an ensemble of quantum dots (QDs) dephases due to the interaction with the surrounding nuclear spins. Despite this dephasing, the spins in the QDs can be controlled to…

Mesoscale and Nanoscale Physics · Physics 2022-04-08 P. Schering , G. S. Uhrig

An unusual regime for liquid-state nuclear magnetic resonance (NMR) where the magnetic field strength is so low that the $J$-coupling (intramolecular spin-spin) interactions dominate the spin Hamiltonian opens a new paradigm with…

Atomic Physics · Physics 2019-10-02 Dmitry Budker

A theoretical study of spin dynamics in non-relativistic particle beams with interacting angular momenta traversing static, spatially varying magnetic fields is presented. The computational framework evaluates sinusoidal magnetic field…

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