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Nonlinear phononics relies on the resonant optical excitation of infrared-active lattice vibrations to coherently induce targeted structural deformations in solids. This form of dynamical crystal-structure design has been applied to control…

Applied Physics · Physics 2021-05-19 Meredith Henstridge , Michael Först , Edward Rowe , Michael Fechner , Andrea Cavalleri

In recent years it has become clear that the transport of excitons and charge carriers in molecular systems can be enhanced by coherent coupling with photons, giving rise to the formation of hybrid excitations known as polaritons. Such…

Materials Science · Physics 2023-01-19 M. Balasubrahmaniyam , Arie Simkovich , Adina Golombek , Guy Ankonina , Tal Schwartz

We propose a theoretical and computational approach to investigate temporal behavior of a nonlinear polarization in perturbative regime induced by an intense and ultrashort pulsed electric field. First-principles time-dependent density…

Optics · Physics 2019-03-27 Mitsuharu Uemoto , Yuki Kuwabara , Shunsuke A. Sato , Kazuhiro Yabana

We study an intense-short pulse propagation in a saturable cubic-quintic nonlinear media in the presence of nonlinear dispersion within the framework of an extended variational approach. We derive an effective equation for the pulse width…

Atomic Physics · Physics 2021-10-14 Sudipta Das , Kajal Krishna Dey , Golam Ali Sekh

We consider theoretically the dynamics of exciton-polaritons in a zigzag chain of coupled elliptical micropillars subjected to incoherent excitation. The driven-dissipative nature of the system along with the naturally present polarization…

Mesoscale and Nanoscale Physics · Physics 2020-10-29 S. Mandal , R. Banerjee , Elena A. Ostrovskaya , T. C. H. Liew

We develop a fully quantum mechanical methodology to describe the static properties and the dynamics of a single anharmonic vibrational mode interacting with a quantized infrared cavity field in the strong and ultrastrong coupling regimes.…

Chemical Physics · Physics 2020-06-22 Johan F. Triana , Federico J. Hernández , Felipe Herrera

Optical nonlinearities are crucial for advanced photonic technologies since they allow photons to be managed by photons. Exciton-polaritons resulting from strong light-matter coupling are hybrid in nature: they combine small mass and high…

We present a study of the macroscopic dynamics of a polariton condensate formed by non-resonant optical excitation in a quasi-one-dimensional ring-shaped microcavity. The presence of a gradient in the cavity photon energy creates a…

The growing interest in exciton-polaritons has driven the need to manipulate their motion and engineer their band structures to the forefront of contemporary research. This study explores the band structures that emerge from a spatially…

Optics · Physics 2025-10-09 Xingran Xu , Chunyu Jia , Xin-Xin Yang

Strong coupling between plasmons and excitons gives rise to new hybrid polariton states with various fields of potential applications. Despite a plethora of research on plasmon--exciton systems, their transient behaviour is not yet fully…

Optics · Physics 2023-06-13 Felix Stete , Matias Bargheer , Wouter Koopman

We present a comprehensive study of exciton wave packet evolution in disordered lossless polaritonic wires. Our simulations reveal signatures of ballistic, diffusive, and subdiffusive exciton dynamics under strong light-matter coupling and…

Quantum Physics · Physics 2023-09-27 Gustavo J. R. Aroeira , Kyle Kairys , Raphael F. Ribeiro

This study investigates the dynamic behavior of polaritons in an optical cavity containing one million molecules, emphasizing the influence of molecular rotation and level disorder on the coupling between molecules and photons. Through…

Optics · Physics 2024-02-22 Wei Liu , Jingqi Chen , Wenjie Dou

Polariton lasing has recently been observed in strongly coupled crystalline anthracene microcavities. A simple model is developed describing the onset of the non-linear threshold based on a master equation including the relevant relaxation…

Mesoscale and Nanoscale Physics · Physics 2013-09-04 Leonardo Mazza , Stéphane Kéna-Cohen , Paolo Michetti , Giuseppe C. La Rocca

The influence of an electron-vibrational coupling on the laser control of electron transport through a molecular wire that is attached to several electronic leads is investigated. These molecular vibrational modes induce an effective…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Jörg Lehmann , Sigmund Kohler , Volkhard May , Peter Hänggi

The way molecules absorb, transfer, and emit light can be modified by coupling them to optical cavities. The extent of the modification is often defined by the cavity-molecule coupling strength, which depends on the number of coupled…

Optics · Physics 2021-06-11 Adarsh B Vasista , Kishan S Menghrajani , William L Barnes

The interaction between electronic and vibrational degrees of freedom is an important mechanism in nonequilibrium charge transport through molecular nanojunctions. While adiabatic polaron-type coupling has been studied in great detail, new…

Mesoscale and Nanoscale Physics · Physics 2022-06-10 Christoph Kaspar , André Erpenbeck , Jakob Bätge , Christian Schinabeck , Michael Thoss

In a recent preprint (arXiv:1401.1128v1) Cilibrizzi and co-workers report experiments and simulations showing the scattering of polaritons against a localised obstacle in a semiconductor microcavity. The authors observe in the linear…

Long-range energy transfer in organic molecules has been experimentally obtained by strongly coupling their electronic excitations to a confined electromagnetic cavity mode. Here, we shed light into the polariton-mediated mechanism behind…

Quantum Physics · Physics 2018-07-30 R. Sáez-Blázquez , J. Feist , A. I. Fernández-Domínguez , F. J. García-Vidal

Confined electromagnetic modes strongly couple to collective excitations in ensembles of quantum emitters, producing light-matter hybrid states known as polaritons. Under such conditions, the discrete multilevel spectrum of molecular…

Quantum Physics · Physics 2022-06-01 Jorge A. Campos-Gonzalez-Angulo , Joel Yuen-Zhou

We have developed a model in order to account for electron-vibrational effects on absorption, luminescence of molecular aggregates and exciton-polaritons in nanofibers. The model generalizes the mean-field electron-vibrational theory…

Mesoscale and Nanoscale Physics · Physics 2019-03-22 Boris D. Fainberg