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A simple and effective single-shot pump-probe technique is reported for studying the ultrafast dynamic processes in various materials. Using only two commercial gratings, a large time window of ~ 95.58 ps is spatially encoded in a single…

We show how two frequency combs $\mathcal{E}_1$, $\mathcal{E}_2$ can be used to measure single-photon, two-photon absorption (TPA), and Raman resonances in a molecule with three electronic bands, by detecting the radio frequency modulation…

Chemical Physics · Physics 2014-08-12 Rachel Glenn , Shaul Mukamel

We have measured the photon statistics of pump and probe beams after interaction with Rb atoms in a situation of Electromagnetically Induced Transparency. Both fields present super-poissonian statistics and their intensities become…

Quantum Physics · Physics 2009-11-07 C. L. Garrido Alzar , L. S. Cruz , J. G. Aguirre Gomez , M. Franca Santos , P. Nussenzveig

A two-step detection strategy is suggested for the precise measurement of the optical phase-shift. In the first step an unsharp, however, unbiased joint measurement of the phase and photon number is performed by heterodyning the signal…

Quantum Physics · Physics 2009-10-31 A. V. Chizhov , V. De Renzi , M. G. A. Paris

With the rapid development of quantum technologies in recent years, the need for high sensitivity measuring techniques has become a key issue. In particular, optical sensors based on quantum states of light have proven to be optimal…

Quantum Physics · Physics 2023-03-29 Laura T. Knoll , Gustavo M. Bosyk

It has been suggested that both quantum superpositions and nonlinear interactions are important resources for quantum metrology. However, to date the different roles that these two resources play in the precision enhancement are not well…

A photoacoustic (PA) sensor for spectroscopic measurements of NO$_2$-N$_2$ at ambient pressure and temperature is demonstrated. The PA sensor is pumped resonantly by a nanosecond pulsed single-mode mid-infrared (MIR) optical parametric…

Applied Physics · Physics 2017-12-29 Mikael Lassen , Laurent Lamard , David Balslev-Harder , Andre peremans , Jan C. Petersen

Critical quantum systems are a promising resource for quantum metrology applications, due to the diverging susceptibility developed in proximity of phase transitions. Here, we assess the metrological power of parametric Kerr resonators…

Quantum Physics · Physics 2023-03-30 R. Di Candia , F. Minganti , K. V. Petrovnin , G. S. Paraoanu , S. Felicetti

Ultrafast-optical-pump -- structural-probe measurements, including ultrafast electron and x-ray scattering, provide direct experimental access to the fundamental timescales of atomic motion, and are thus foundational techniques for studying…

We introduce the concept of spatial and spectral control of nonlinear parametric sidebands in multimode optical fibers by tailoring their linear refractive index profile. In all cases, the pump experiences Kerr self-cleaning, leading to a…

In pump-probe spectroscopy, one often needs to analyse the transmission or reflection of electromagnetic waves through optically pumped media. Here, it is common practice to approximate the analysis in order to extract non-equilibrium…

Optics · Physics 2019-02-26 Peter Karlsen , Euan Hendry

The determination of the nonlinear optical coefficient \( n_2 \) of pure water is of great interest for applications such as imaging biological systems, performing femtosecond laser surgery, and underwater ablation. Traditionally, probing…

Optics · Physics 2025-02-06 Ilyes Betka

We present a simple and inexpensive means to measure background-free photoinduced absorption spectra by implementing a dual optical modulation scheme. Our objective is to measure quasi-steady-state absorption spectra of long-lived…

A fiber taper waveguide is used to perform direct optical spectroscopy of a microdisk-quantum-dot system, exciting the system through the photonic (light) channel rather than the excitonic (matter) channel. Strong coupling, the regime of…

Quantum Physics · Physics 2009-11-13 Kartik Srinivasan , Oskar Painter

Our goal is to study optical signatures of quantum vacuum nonlinearities in strong macroscopic electromagnetic fields provided by high-intensity laser beams. The vacuum emission scheme is perfectly suited for this task as it naturally…

High Energy Physics - Phenomenology · Physics 2019-05-22 Alexander Blinne , Holger Gies , Felix Karbstein , Christian Kohlfürst , Matt Zepf

We show that the quantum Cram\'er-Rao bound on the precision of measurements of the optical phase gradient, or the wavefront tilt, with a beam of finite width is consistent with the Heisenberg uncertainty principle for a single-photon…

Quantum Physics · Physics 2020-07-22 Walker Larson , Bahaa E. A. Saleh

Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled…

Chemical Physics · Physics 2021-07-28 Yuta Fujihashi , Akihito Ishizaki

Near-infrared (NIR) hyperspectral imaging is widely used to reveal morphological and chemical information. However, conventional spectral imagers usually rely on costly focal plane arrays and suffer from data redundancy and inefficiencies…

Optics · Physics 2026-05-26 Ben Sun , Kun Huang , Zhibin Zhao , Beibei Dong , Jianan Fang , Heping Zeng

The development of many optical quantum technologies depends on the availability of solid-state single quantum emitters with near-perfect optical coherence. However, a standing issue that limits systematic improvement is the significant…

Based on the conventional Mach-Zehnder interferometer, we propose a metrological scheme to improve phase sensitivity. In this scheme, we use a coherent state and a squeezed vacuum state as input states, employ multi-photon-subtraction…

Quantum Physics · Physics 2025-05-08 Qisi Zhou , Qinqian Kang , Tao Jiang , Zekun Zhao , Teng Zhao , Cunjin Liu , Liyun Hu