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We generalized the recently introduced new impurity solver based on the diagrammatic expansion around the atomic limit and Quantum Monte Carlo summation of the diagrams. We present generalization to the cluster of impurities, which is at…

Strongly Correlated Electrons · Physics 2009-11-11 Kristjan Haule

The dynamics and decoherence of an electronic spin-1/2 qubit coupled to a bath of nuclear spins via hyperfine interactions in a quantum dot is studied. We show how exact results from the integrable solution can be used to understand the…

Strongly Correlated Electrons · Physics 2010-10-22 Michael Bortz , Sebastian Eggert , Christian Schneider , Robert Stubner , Joachim Stolze

Perturbative schemes utilizing a spectral moment expansion are well known and extensively used for investigating the physics of model Hamiltonians and real material systems. The advantages they offer, in terms of being computationally…

Strongly Correlated Electrons · Physics 2016-11-09 Nagamalleswararao Dasari , Wasim Raja Mondal , Peng Zhang , Juana Moreno , Mark Jarrell , N. S. Vidhyadhiraja

We present a time-domain iteration scheme for solving the Dynamical Mean-Field Theory (DMFT) self-consistent equations using retarded Green's functions in real time. Unlike conventional DMFT approaches that operate in imaginary time or…

Strongly Correlated Electrons · Physics 2026-01-28 Chakradhar Rangi , Aadi Singh , Ka-Ming Tam

We introduce various exchange interactions in a model Hamiltonian for Ce$^{3+}$ ions in cubic symmetry with three configurations ($f^0$,$f^1$,$f^2$). With the impurity pseudo spin $S_I=1/2$, our Hamiltonian includes: (i) One-channel…

Condensed Matter · Physics 2009-10-28 Tae-Suk Kim , D. L. Cox

Although selected configuration interaction (SCI) algorithms can tackle much larger Hilbert spaces than the conventional full CI (FCI) method, the scaling of their computational cost with respect to the system size remains inherently…

Chemical Physics · Physics 2024-12-02 Abdallah Ammar , Anthony Scemama , Pierre-François Loos , Emmanuel Giner

We propose a mixed-configuration approximation based on single-band impurity solvers to efficiently study nonequilibrium multi-orbital systems at moderate computational cost. In this work, we merge the approach with the so-called auxiliary…

Strongly Correlated Electrons · Physics 2025-07-16 Tommaso Maria Mazzocchi , Daniel Werner , Markus Aichhorn , Enrico Arrigoni

We study the quench dynamics of an Anderson impurity model using the configuration interaction (CI) method. In particular, we focus on the relaxation behavior of the impurity occupation. The system is found to behave very differently in the…

Strongly Correlated Electrons · Physics 2015-10-26 Chungwei Lin , Alexander A. Demkov

We present a quantum-classical hybrid algorithm for calculating the ground state and its energy of the quantum many-body Hamiltonian by proposing an adaptive construction of a quantum state for the quantum-selected configuration interaction…

Quantum Physics · Physics 2024-12-12 Yuya O. Nakagawa , Masahiko Kamoshita , Wataru Mizukami , Shotaro Sudo , Yu-ya Ohnishi

We present a very efficient solver for the general Anderson impurity problem. It is based on the perturbation around a solution obtained from exact diagonalization using a small number of bath sites. We formulate a perturbation theory which…

Searching for potential active compounds in large databases is a necessary step to reduce time and costs in modern drug discovery pipelines. Such virtual screening methods seek to provide predictions that allow the search space to be…

Biomolecules · Quantitative Biology 2023-05-23 Rafael Mena-Yedra , Juana L. Redondo , Horacio Pérez-Sánchez , Pilar M. Ortigosa

We study cubic cardinality-constrained portfolio optimization, a higher-order extension of the standard Markowitz formulation where three-way sector co-movement terms augment the quadratic risk-return objective. Classical heuristics like…

Computational Finance · Quantitative Finance 2026-03-18 Greg Serbarinov

We study several approaches to orbital optimization in selected configuration interaction plus perturbation theory (SCI+PT) methods, and test them on the ground and excited states of three molecules using the semistochastic heatbath…

Chemical Physics · Physics 2021-07-14 Yuan Yao , C. J. Umrigar

We investigate the in- and out-of-equilibrium phenomena of a rotational impurity -- specifically, a linear molecule -- coupled to a nonconventional environment, a helium nanodroplet. By employing a Lee-Low-Pines-like transformation combined…

Quantum Gases · Physics 2025-04-23 Wei Zhang , Zhongda Zeng , Tao Shi

We propose to calculate spectral functions of quantum impurity models using the Time Evolving Block Decimation (TEBD) for Matrix Product States. The resolution of the spectral function is improved by a so-called linear prediction approach.…

Strongly Correlated Electrons · Physics 2015-10-28 Martin Ganahl , Markus Aichhorn , Patrik Thunström , Karsten Held , Hans Gerd Evertz , Frank Verstraete

Vibrational heat-bath configuration interaction (VHCI) -- a selected configuration interaction technique for vibrational structure theory -- has recently been developed in two independent works [J. Chem. Phys. 154, 074104 (2021); Mol. Phys.…

Chemical Physics · Physics 2023-07-26 Henry K. Tran , Timothy C. Berkelbach

This work explores the ability of classical electronic structure methods to efficiently represent (compress) the information content of full configuration interaction (FCI) wave functions. We introduce a benchmark set of four hydrogen model…

Chemical Physics · Physics 2020-08-20 Nicholas H. Stair , Francesco A. Evangelista

We develop a method to study quantum impurity models, small interacting quantum systems linearly coupled to an environment, in presence of an additional Markovian quantum bath, with a generic non-linear coupling to the impurity. We aim at…

Quantum Physics · Physics 2025-03-10 Orazio Scarlatella , Marco Schirò

We study impurities in integrable models from the viewpoint of generalized hydrodynamics (GHD). An impurity can be thought of as a boundary condition for the GHD equation, relating the state on the left and right side. We find that in…

Statistical Mechanics · Physics 2024-06-27 Friedrich Hübner

We solve the impurity problem which arises within nonequilibrium dynamical mean-field theory for the Hubbard model by means of a self-consistent perturbation expansion around the atomic limit. While the lowest order, known as the…

Strongly Correlated Electrons · Physics 2013-05-29 Martin Eckstein , Philipp Werner