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Explaining the formation pathways of amides on ice-grain mantels is crucial to understanding the prebiotic chemistry in an interstellar medium. In this computational study, we explore different radical-neutral formation pathways for some of…

Astrophysics of Galaxies · Physics 2024-07-10 Gabriela Silva-Vera , Giulia M. Bovolenta , Namrata Rani , Sebastian Vera , Stefan Vogt-Geisse

Radical recombination has been proposed to lead to the formation of complex organic molecules (COMs) in CO-rich ices in the early stages of star formation. These COMs can then undergo hydrogen addition and abstraction reactions leading to a…

Astrophysics of Galaxies · Physics 2018-06-07 S. Álvarez-Barcia , P. Russ , J. Kästner , T. Lamberts

Hydrogen hydrates (HH) are a unique class of materials composed of hydrogen molecules confined within crystalline water frameworks. Among their multiple phases, the filled ice structures, particularly the cubic C2 phase, exhibit…

Recent interstellar detections include a significant number of molecules containing vinyl (C2H3) and ethyl (C2H5) groups in their structure. For several of these molecules, there is not a clear experimental or theoretical evidence that…

Astrophysics of Galaxies · Physics 2022-09-07 German Molpeceres , Victor M. Rivilla

Hydrogen cyanide (HCN) is a critical reactive source of nitrogen for building key biomolecules relevant for the origin of life. Still, many HCN reactions remain uncharacterized by experiments and theory, and the complete picture of HCN…

Earth and Planetary Astrophysics · Physics 2022-01-05 Ben K. D. Pearce , Karan Molaverdikhani , Ralph E. Pudritz , Thomas Henning , Eric Hébrard

The modelling of emission spectra of molecules seen in interstellar clouds requires the knowledge of collisional rate coefficients. Among the commonly observed species, N$_2$H$^+$ is of particular interest since it was shown to be a good…

Astrophysics of Galaxies · Physics 2015-06-23 François Lique , Fabien Daniel , Laurent Pagani , Nicole Feautrier

The abundance of interstellar ice constituents is usually expressed with respect to the water ice because, in denser regions, a significant portion of the interstellar grain surface would be covered by water ice. The binding energy (BE), or…

Astrophysics of Galaxies · Physics 2021-06-01 Ankan Das , Milan Sil , Rana Ghosh , Prasanta Gorai , Soutan Adak , Subhankar Samanta , Sandip K. Chakrabarti

Aims. We present a new sub-grid model, HYACINTH -- HYdrogen And Carbon chemistry in the INTerstellar medium in Hydro simulations -- for computing the non-equilibrium abundances of ${\rm H_2}$ and its carbon-based tracers, namely ${\rm CO}$,…

Astrophysics of Galaxies · Physics 2024-07-02 Prachi Khatri , Cristiano Porciani , Emilio Romano-Díaz , Daniel Seifried , Alexander Schäbe

The knowledge of the binding energy of molecules on astrophysically relevant ices can help to obtain an estimate of the desorption rate, i.e. the molecules residence time on the surface. This represents an important parameter for…

The formation of hydrides by gas-phase reactions between H2 and a heavy element atom is a very selective process. Reactions with ground-state neutral carbon, oxygen, nitrogen, and sulfur atoms are very endoergic and have high energy…

Astrophysics of Galaxies · Physics 2022-08-31 Javier R. Goicoechea , Octavio Roncero

H2 is the simplest and the most abundant molecule in the ISM, and its formation precedes the formation of other molecules. Understanding the dynamical influence of the environment and the interplay between the thermal processes related to…

Astrophysics of Galaxies · Physics 2016-02-24 Valeska Valdivia , Patrick Hennebelle , Maryvonne Gérin , Pierre Lesaffre

We studied the abundance of HCN, H13CN, and HN13C in a sample of prestellar cores, in order to search for species associated with high density gas. We used the IRAM 30m radiotelescope to observe along the major and the minor axes of L1498,…

Astrophysics of Galaxies · Physics 2015-05-30 M. Padovani , C. M. Walmsley , M. Tafalla , P. Hily-Blant , G. Pineau des Forêts

Context: Hydrogenation reactions are expected to be among the most important surface reactions on interstellar ices. However, solid state astrochemical laboratory data on reactions of H-atoms with common interstellar ice constituents are…

Astrophysics · Physics 2009-11-13 S. E. Bisschop , G. W. Fuchs , E. F. van Dishoeck , H. Linnartz

HNC and HCN, typically used as dense gas tracers in molecular clouds, are a pair of isomers that have great potential as a temperature probe because of temperature dependent, isomer-specific formation and destruction pathways. Previous…

Astrophysics of Galaxies · Physics 2015-06-19 Dawn Graninger , Eric Herbst , Karin I. Oberg , Anton I. Vasyunin

We investigate how the existence of hydrogen molecules on grain surfaces may affect H$_2$ formation efficiency in diffuse and translucent clouds. Hydrogen molecules are able to reduce the desorption energy of H atoms on grain surfaces in…

Astrophysics of Galaxies · Physics 2022-03-30 Gang Zhao , Qiang Chang , Xia Zhang , Donghui Quan , Yong Zhang , Xiao-Hu Li

Interaction of NH$_3$$^{+}$ (ND$_3$$^{+}$) and NH$^{+}$ with a hydrocarbon-covered tungsten surface kept at room temperature and heated to 150{\deg}C and 300{\deg}C showed a series of reactions between the projectile ion and hydrocarbons…

Atomic and Molecular Clusters · Physics 2018-05-04 Martina Harnisch , Paul Scheier , Zdenek Herman

The Hugoniot for Deuterium is calculated using the classical-map hyper-netted-chain (CHNC) approach using several models of the effective temperature that may be assigned to the electron-ion interaction. This effective temperature embodies…

Chemical Physics · Physics 2017-07-28 M. W. C. Dharma-wardana

Condensation of H 2 in the interstellar medium (ISM) has long been seen as a possibility, either by deposition on dust grains or thanks to a phase transition combined with self-gravity. H 2 condensation might explain the observed low…

Astrophysics of Galaxies · Physics 2018-06-06 Andreas Füglistaler , Daniel Pfenniger

Developing solid-state hydrogen storage materials is as pressing as ever, which requires a comprehensive understanding of the dehydrogenation chemistry of a solid-state hydride. Transition state search and kinetics calculations are…

Materials Science · Physics 2024-04-30 Chaoqun Li , Weijie Yang , Hao Liu , Xinyuan Liu , Xiujing Xing , Zhengyang Gao , Shuai Dong , Hao Li

The formation of interstellar water has been commonly accepted to occur on the surfaces of icy dust grains in dark molecular clouds at low temperatures (10-20 K), involving hydrogenation reactions of oxygen allotropes. As a result of the…

Astrophysics of Galaxies · Physics 2014-10-22 Thanja Lamberts , Herma Cuppen , Gleb Fedoseev , Sergio Ioppolo , Ko-Ju Chuang , Harold Linnartz
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