Related papers: Engineering Ferrimagnetic Interactions in Molecula…
Antiferromagnetic and ferro/ferrimagnetic orders are typically exclusive in nature, thus, their co-existence in atomic-scale proximity is expected only in heterostructures. Breaking this paradigm and broadening the range of unconventional…
We investigate from first principles a variety of low-dimensional open quantum spin systems based on magnetic nanographene structures that contain spin-1/2 and spin-1 triangulenes and/or olympicenes. These graphene nanostructures behave as…
Quasi-one-dimensional quantum antiferromagnets formed by a d-dimensional hypercubic lattice of weakly coupled spin-1/2 antiferromagnetic Heisenberg chains are studied by combining exact results in one-dimension and renormalization group…
Quasiperiodic structures possess long range positional order, but are freed of constraints imposed by translational invariance. For spins interacting via Heisenberg couplings, one may expect therefore to find novel magnetic configurations…
We present an antiferromagnetic quantum spin-1/2 model on honeycomb lattice. It has two parts, one of which is the usual nearest-neighbor Heisenberg model. The other part is a certain multiple spin interaction term, introduced by us, which…
We discuss spin-$S$ antiferromagnetic Heisenberg chains with three-spin interactions, next-nearest-neighbor interactions, and bond alternation. First, we prove rigorously that there exist parameter regions of the exact dimerized ground…
The ground state, magnetization scenario and the local bipartite quantum entanglement of a mixed spin-$1/2$ Ising--Heisenberg model in a magnetic field on planar lattices formed by identical corner-sharing bipyramidal plaquettes is examined…
Quantum spin networks having engineered geometries and interactions are eagerly pursued for quantum simulation and access to emergent quantum phenomena such as spin liquids. Spin-1/2 centers are particularly desirable because they readily…
Magnetic interactions between localized spins-1/2 play a central role in quantum magnetism, spin-based quantum computing, and quantum simulation. The range and strength of these interactions are key figures of merit. Here, we probe exchange…
An $S=1/2$ ferromagnetic (F) - antiferromagnetic (AF) random alternating Heisenberg quantum spin chain model is investigated in connection to its realization compound: (CH$_3$)$_2$CHNH$_3$Cu(Cl$_x$Br$_{1-x}$)$_3$. The exchange interaction…
Quantum-mechanical correlations of interacting fermions result in the emergence of exotic phases. Magnetic phases naturally arise in the Mott-insulator regime of the Fermi-Hubbard model, where charges are localized and the spin degree of…
Frustrated magnetic compounds, in particular low-dimensional, are topical research due to persistent uncover of novel nontrivial quantum states and potential applications. The problem of this field is that many important results are…
Strongly correlated systems with geometric frustrations can host the emergent phases of matter with unconventional properties. Here, we study the spin $S = 1$ Heisenberg model on the honeycomb lattice with the antiferromagnetic first-…
We investigate the spin $S=1/2$ Heisenberg model on the body centered cubic lattice in the presence of ferromagnetic and antiferromagnetic nearest-neighbor $J_{1}$, second-neighbor $J_{2}$, and third-neighbor $J_{3}$ exchange interactions.…
Long-range interactions can qualitatively reorganize correlated-electron ground states. In the square-lattice Hubbard model, on-site repulsion produces antiferromagnetic spin and charge stripes upon doping. We show that including a…
The calculation of interatomic magnetic exchange interactions entering the Heisenberg model from the standpoint of the density functional theory (DFT) is outlined for two Fe-based molecular magnets: a trinuclear complex with a Schiff base…
Motivated by recent experimental breakthroughs, we propose a strategy to design two-dimensional spin lattices with competing interactions that lead to non-trivial emergent quantum states. We consider $S=1/2$ nanographenes with $C_3$…
We work out the magnetization and susceptibility of Heisenberg- and XXZ-model antiferromagnet spin-1/2 systems in $D$ dimensions under a rigorous constraint of single particle site occupancy. Quantum fluctuations are taken into account up…
Triangulenes are prototypical examples of open-shell nanographenes. Their magnetic properties, arising from the presence of unpaired $\pi$ electrons, can be extensively tuned by modifying their size and shape or by introducing heteroatoms.…
We introduce a spin-symmetry-broken extension of the connected determinant algorithm [Phys. Rev. Lett. 119, 045701 (2017)]. The resulting systematic perturbative expansions around an antiferromagnetic state allow for numerically exact…