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The subtle interplay between spin-orbit coupling, exchange interactions, and cation ordering can lead to exotic magnetic states in transition-metal ions. We report a comprehensive study of the Re-based (5$d^1$) ordered double perovskite…

We present the magnetic structure of $\mathrm{TmMn_3O_6}$, solved via neutron powder diffraction - the first such study of any $R\mathrm{Mn_3O_6}$ A-site columnar-ordered quadruple perovskite to be reported. We demonstrate that long range…

Strongly Correlated Electrons · Physics 2019-03-27 A. M. Vibhakar , D. D. Khalyavin , P. Manuel , L. Zhang , K. Yamaura , P. G. Radaelli , A. A. Belik , R. D. Johnson

Thermal properties of the $S=1/2$ kagome Heisenberg antiferromagnet at low temperatures are investigated by means of the Hams-de Raedt method for clusters of up to 36 sites possessing a full symmetry of the lattice. The specific heat…

Strongly Correlated Electrons · Physics 2016-10-26 Tokuro Shimokawa , Hikaru Kawamura

The intriguing interplay between competing degrees of freedom in frustrated magnets can lead to non-trivial magnetic phenomena with exotic low-energy excitations that are highly relevant for addressing some of the fundamental questions in…

Strongly Correlated Electrons · Physics 2026-03-20 A. Yadav , U. Jena , A. Pradhan , Satish K. , P. Khuntia

New double perovskites LaPbMSbO6, where M2+ = Mn2+, Co2+, and Ni2+, were synthesized as polycrystals by an aqueous synthetic route at temperatures below 1000 oC. All samples are monoclinic, space group P21/n, as obtained from Rietveld…

Materials Science · Physics 2013-03-11 D. G. Franco , R. E. Carbonio , G. Nieva

Double-perovskite oxides that contain both 3d and 5d transition metal elements have attracted growing interest as they provide a model system to study the interplay of strong electron interaction and large spin-orbit coupling (SOC). Here,…

Strongly Correlated Electrons · Physics 2016-09-01 W. K. Zhu , J. -C. Tung , W. Tong , L. Ling , M. Starr , J. M. Wang , W. C. Yang , Y. Losovyj , H. D. Zhou , Y. Q. Wang , P. -H. Lee , Y. -K. Wang , Chi-Ken Lu , S. X. Zhang

We propose a minimal model describing magnetic behavior of Fe-based superconductors. The key ingredient of the model is a dynamical mixing of quasi-degenerate spin states of Fe2+ ion by intersite electron hoppings, resulting in an effective…

Strongly Correlated Electrons · Physics 2013-05-31 Jiří Chaloupka , Giniyat Khaliullin

The low-doped magnetic perovskite La_{7/8}Sr_{1/8}MnO_3 undergoes within the paramagnetic-semiconducting phase a first-order structural transition due to antiferrodistorsive ordering of Jahn-Teller deformed MnO_6 octahedra. This allows to…

Strongly Correlated Electrons · Physics 2009-10-31 P. Wagner , I. Gordon , S. Mangin , V. V. Moshchalkov , Y. Bruynseraede , L. Pinsard , A. Revcolevschi

Magnetic state is a partial ordered state if only part of the electrons in the system give contribution to the magnetic order. We study Heisenberg model of two sublattice spin system, on the body-centered cubic lattice, with…

Strongly Correlated Electrons · Physics 2024-09-20 N. Karchev

Quantum-disordered magnetic ground states are challenging to identify in three-dimensional (3D) oxides, where strong exchange pathways typically favour long-range magnetic order or spin freezing. The quadruple perovskite…

Strongly Correlated Electrons · Physics 2026-05-11 J. Ming , Abhisek Bandyopadhyay , G. B. G. Stenning , M. T. F. Telling , N. N. Wang , G. Wang , J. -G. Cheng , D. T. Adroja

Disorder can have a dominating influence on correlated and quantum materials leading to novel behaviors which have no clean limit counterparts. In magnetic systems, spin and exchange disorder can provide access to quantum criticality,…

Among the 3d transition metal ions doped polar Ni3TeO6, Mn-doped Ni3TeO6 has stimulated great interest due to its high magnetic ordering temperature and complex magnetic phases, but the mechanism of magnetoelectric (ME) coupling is far from…

Transport and magnetic studies of Ca3Ru2O7 for temperatures ranging from 0.4 K to 56 K and magnetic fields, B, up to 45 T leads to strikingly different behavior when the field is applied along the different crystal axes. A ferromagnetic…

Strongly Correlated Electrons · Physics 2009-11-11 X. N. Lin , Z. X. Zhou , V. Durairaj , P. Schlottmann , G. Cao

The samples LaCoO3 with dilute substitutions on cobalt sites have been studied using the resistivity, thermopower and magnetic susceptibility measurements over the temperature range up to ~900 K. The Co-site substitution does not affect the…

Materials Science · Physics 2010-07-30 J. Hejtmanek , Z. Jirak , K. Knizek , M. Marysko , M. Veverka , C. Autret

Detailed structural measurements were conducted on a new perovskite, ScMnO3, and on orthorhombic LuMnO3. Complementary density functional theory (DFT) calculations were carried out, and predict that ScMnO3 possesses E-phase magnetic order…

Strongly Correlated Electrons · Physics 2015-06-19 T. Yu , T. A. Tyson , H. Y. Chen , A. M. M. Abeykoon , Y. -S. Chen , K. H. Ahn

We report on a 59Co NMR investigation of the trigonal cobaltate Ca3Co2O6 carried out on a single crystal, providing precise determinations of the electric field gradient and chemical shift tensors, and of the internal magnetic fields at the…

Strongly Correlated Electrons · Physics 2015-05-20 G. Allodi , R. De Renzi , S. Agrestini , C. Mazzoli , M. R. Lees

We use ab initio electronic structure calculations in combination with Monte Carlo simulations to investigate the magnetic and ferroelectric properties of bulk orthorhombic HoMnO$_3$ and ErMnO$_3$. Our goals are to explain the…

Materials Science · Physics 2018-12-12 Natalya S. Fedorova , Amadé Bortis , Christoph Findler , Nicola A. Spaldin

We report a neutron scattering study of the magnetic order and dynamics of the bilayer perovskite Sr$_3$Fe$_2$O$_7$, which exhibits a temperature-driven metal-insulator transition at 340 K. We show that the Fe$^{4+}$ moments adopt…

We have studied the magnetic properties and spin-dynamics of the structurally-ordered double perovskite Sr$_2$CoOsO$_6$. Our neutron diffraction, muon spin relaxation and ac-susceptibility measurements reveal two antiferromagnetic (AFM)…

One of the key questions concerning frustrated lattices that has lately emerged is the role of disorder in inducing spin-liquid-like properties. In this context, the quantum kagome antiferromagnets YCu$_3$(OH)$_6$Cl$_3$, which has been…

Strongly Correlated Electrons · Physics 2019-07-02 A. Zorko , M. Pregelj , M. Klanjšek , M. Gomilšek , Z. Jagličić , J. S. Lord , J. A. T. Verezhak , T. Shang , W. Sun , J. -X. Mi