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We demonstrate, numerically, the possibility of manipulating the spin states of molecular nanomagnets with shaped microwave pulses designed with quantum optimal control theory techniques. The state-to-state or full gate transformations can…

Quantum Physics · Physics 2021-12-01 Alberto Castro , Adrian Garcia Carrizo , David Zueco , Fernando Luis

Pulsed magnetic resonance is a wide-reaching technology allowing the quantum state of electronic and nuclear spins to be controlled on the timescale of nanoseconds and microseconds respectively. The time required to flip either dilute…

We introduce a novel control method for robust quantum information processing suited for quantum integrated photonics. We utilize off-resonant detunings as control parameters to derive a new family of composite pulses for high-fidelity…

Quantum Physics · Physics 2019-10-02 Elica Kyoseva , Hadar Greener , Haim Suchowski

The development of quantum computers based on superconductors requires the improvement of the qubit state control approach aimed at the increase of the hardware energy efficiency. A promising solution to this problem is the use of…

Quantum Physics · Physics 2023-10-19 Vsevolod Vozhakov , Marina Bastrakova , Nikolay Klenov , Arkady Satanin , Igor Soloviev

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

High-fidelity state transfer is fundamentally limited by time-reversal symmetry: one qubit emits a photon with a certain temporal pulse shape, whereas a second qubit requires the time-reversed pulse shape to efficiently absorb this photon.…

Quantum Physics · Physics 2025-12-24 Zeyu Kuang , Oliver Diekmann , Lorenz Fischer , Stefan Rotter , Carlos Gonzalez-Ballestero

Quantum computing is an advanced area of computing that leverages the principles of quantum mechanics. Quantum computing holds the potential to revolutionize various fields by handling problems that are currently intractable for classical…

Quantum Physics · Physics 2024-10-28 Xiaoan Lin

Recent advances in engineering and control of nanoscale quantum sensors have opened new paradigms in precision metrology. Unfortunately, hardware restrictions often limit the sensor performance. In nanoscale magnetic resonance probes, for…

Quantum Physics · Physics 2017-07-05 A. Ajoy , Y. X. Liu , K. Saha , L. Marseglia , J. -C. Jaskula , U. Bissbort , P. Cappellaro

We present a continuous-time, neural-network-based approach to optimal control in quantum systems, with a focus on pulse engineering for quantum gates. Leveraging the framework of neural ordinary differential equations, we construct control…

Coupled pairs of spin-1/2 nuclei support one singlet state and three triplet states. In many circumstances the nuclear singlet order, defined as the difference between the singlet population and the mean of the triplet populations, is a…

Quantum Physics · Physics 2022-10-19 Mohamed Sabba , Nino Wili , Christian Bengs , Lynda J. Brown , Malcolm H. Levitt

Efficient hyperpolarisation of nuclear spins via optically active defect centers, such as the nitrogen vacancy (NV) center in diamond, has great potential for enhancing NMR based quantum information processing and nanoscale magnetic…

Dynamical nuclear polarisation (DNP) is an important technique that uses polarisation transfer from electron to nuclear spins to achieve nuclear hyperpolarisation. As the electron spin of the nitrogen vacancy (NV) centres in diamond can be…

We investigate the spin-dependent dynamical response of a quantum ring with a spin-orbit interaction upon the application of linearly polarized, picosecond, asymmetric electromagnetic pulses. The oscillations of the generated dipole moment…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Zhen-Gang Zhu , Jamal Berakdar

Numerically we simulate the effect of optimized coherent control pulses with a finite duration on a qubit in a bath of spins. The pulses of finite duration are compared with ideal instantaneous pulses. In particular, we show that properly…

Quantum Physics · Physics 2008-08-26 P. Karbach , S. Pasini , G. S. Uhrig

The coherence of an electronic spin in a semiconductor quantum dot decays due to its interaction with the bath of nuclear spins in the surrounding isotopes. This effect can be reduced by subjecting the system to an external magnetic field…

Mesoscale and Nanoscale Physics · Physics 2018-07-18 Philipp Schering , Jan Hüdepohl , Götz S. Uhrig , Benedikt Fauseweh

Control protocol to drive finite dimensional quantum systems to an arbitrary target state using square pulses is proposed explicitly. It is a multi-cycle control process and in each cycle we apply square pulses to cause single or a few…

Quantum Physics · Physics 2013-12-19 Jianju Tang , H. C. Fu

Finding control fields (pulse sequences) that can compensate for the dispersion in the parameters governing the evolution of a quantum system is an important problem in coherent spectroscopy and quantum information processing. The use of…

Quantum Physics · Physics 2015-06-04 Philip Owrutsky , Navin Khaneja

In pulsed dynamic nuclear polarization (DNP), enhancement of the polarization of bulk nuclei requires the repeated application of a microwave pulse sequence. So far, analysis of a one-time transfer of electron spin polarization to a…

Chemical Physics · Physics 2025-07-24 Shebha Anandhi Jegadeesan , Yujie Zhao , Graham M. Smith , Ilya Kuprov , Guinevere Mathies

Quantum optimal control theory (QOCT) can be used to design the shape of electromagnetic pulses that implement operations on quantum devices. By using non-trivially shaped waveforms, gates can be made significantly faster than those built…

Quantum Physics · Physics 2026-02-27 Alonso Hernández-Antón , Fernando Luis , Alberto Castro

Radio-frequency pulses are widespread for the control of quantum bits and the execution of operations in quantum computers. The ability to tune key pulse parameters such as time-dependent amplitude, phase, and frequency is essential to…

Quantum Physics · Physics 2024-08-19 Jan Ole Ernst , Jan Snoeijs , Mitchell Peaks , Jochen Wolf