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We propose a modified Stark-chirped rapid adiabatic passage technique for a robust rovibrational population transfer in the gas phase molecules in the presence of certain inhomogeneous electric fields. As an example application, the new…

Atomic Physics · Physics 2025-06-06 Emil Zak , Jochen Küpper , Andrey Yachmenev

In recent demonstrations of the quantum charge-coupled device (QCCD) computer architecture, circuit times are dominated by cooling. Some motional modes of multi-ion crystals take orders-of-magnitude longer to cool than others because of low…

Quantum Physics · Physics 2024-03-19 M. I. Fabrikant , P. Lauria , I. S. Madjarov , W. C. Burton , R. T. Sutherland

Magnetically trapped neutral atoms can be cooled with the evaporation technique. This is typically done by using a radiofrequency (rf) field that adiabatically couples trapped and untrapped internal atomic states for atoms with kinetic…

Atomic Physics · Physics 2009-10-31 K. -A. Suominen , E. Tiesinga , P. S. Julienne

We show that the optical absorbance detection of nuclear spin echo gives direct access to the spin concentration, unlike most coherent signal detection techniques where the signal intensity/amplitude is difficult to connect experimentally…

Quantum Physics · Physics 2011-06-14 R. Lauro , T. Chaneliere , J. -L. Le Gouet

Coupled electron-nuclear spins represent a promising quantum system, where the optically induced electron spin polarization can be dynamically transferred to nuclear spins via the hyperfine interaction. Most experiments on dynamic nuclear…

Materials Science · Physics 2026-01-13 A. N. Anisimov , A. V. Poshakinskiy , G. V. Astakhov

We present a hyperfine-resolved state preparation scheme for thallium fluoride (TlF) molecules based on microwave-driven adiabatic passage (AP) in a spatially varying electric field. This method enables efficient and robust population…

Precision measurements based on optically detected nuclear magnetic resonance offer exquisite sensitivity to absolute shifts in spin transition frequencies, with potential applications in fundamental physics experiments and inertial…

We apply the transitionless quantum driving method to control the electron spin of a two-electron double quantum dot with spin-orbit coupling by time-dependent electric fields. The $x$ and $y$ components of applied electric fields in each…

Quantum Physics · Physics 2012-12-14 Yue Ban

Nuclear spin hyperpolarization provides a promising route to overcome the challenges imposed by the limited sensitivity of nuclear magnetic resonance. Here we demonstrate that dissolution of spin-polarized pentacene-doped naphthalene…

We use microwave induced adiabatic passages for selective spin flips within a string of optically trapped individual neutral Cs atoms. We position-dependently shift the atomic transition frequency with a magnetic field gradient. To flip the…

We present the APLIP process (Adiabatic Passage by Light Induced Potentials) for the adiabatic transfer of a wave packet from one molecular potential to the displaced ground vibrational state of another. The process uses an intermediate…

Chemical Physics · Physics 2009-10-30 B. M. Garraway , K. -A. Suominen

We propose shortcuts to adiabaticity which achieve fast and stable control of the state of a charged particle in an electromagnetic field. In particular we design a non-adiabatic change of the magnetic field strength in a Penning trap which…

Quantum Physics · Physics 2017-03-14 A. Kiely , J. P. L. McGuinness , J. G. Muga , A. Ruschhaupt

By using highly time-resolved spectroscopy with an alternative {\sigma}+/{\sigma} - laser pulse modulation technique, we are able to measure the fast buildup and decay times of the dynamical nuclear spin polarization (DNSP) at 5 K for a…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 X. M. Dou , B. Q. Sun , D. S. Jiang , H. Q. Ni , Z. C. Niu

In dissolution-dynamic nuclear polarization, nuclear spins are hyperpolarized at cryogenic temperatures using radicals and microwave irradiation. The hyperpolarized solid is dissolved with hot solvent and the solution is transferred to a…

Instrumentation and Detectors · Physics 2019-06-20 Karel Kouřil , Hana Kouřilová , Samuel Bartram , Malcolm H. Levitt , Benno Meier

Accurate control of a quantum system is a fundamental requirement in many areas of modern science ranging from quantum information processing to high-precision measurements. A significantly important goal in quantum control is to prepare a…

We experimentally demonstrate high degree of polarization of 13C nuclear spins weakly interacting with nitrogen-vacancy (NV) centers in diamond. We combine coherent microwave excitation pulses with optical illumination to provide controlled…

Quantum Physics · Physics 2019-10-25 Jiwon Yun , Kiho Kim , Dohun Kim

We experimentally demonstrate a method for obtaining nuclear spin hyperpolarization, that is, polarization significantly in excess of that expected for a thermal equilibrium. By exploiting a modified Overhauser process, we obtain more than…

Materials Science · Physics 2009-02-26 D. R. McCamey , J. van Tol , G. W. Morley , C. Boehme

Stimulated Raman Adiabatic Passage (STIRAP) is a widely used method for adiabatic population transfer in a multilevel system. In this work, we study STIRAP under novel conditions and focus on the fractional, F-STIRAP, which is known to…

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

We demonstrate a method of adiabatic population transfer from a single quantum state into a coherent superposition of states. The transfer is executed with femtosecond pulses, spectrally shaped in simple and intuitive manner, which does not…

Quantum Physics · Physics 2015-05-14 S. Zhdanovich , E. A. Shapiro , J. W. Hepburn , M. Shapiro , V. Milner