Related papers: A Dual-Sideband Attosecond Interferometry Setup
We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…
We theoretically explore a variant of RABBITT spectroscopy in which the attosecond-pulse train comprises isolated pairs of consecutive harmonics of the fundamental infrared probe frequency. In this scheme, one-photon and two-photon…
We employ the recently developed multi-photon R-matrix method for molecular above-threshold photoionization to obtain second-order ionization amplitudes that govern the interference in RABITT experiments. This allows us to extract RABITT…
Attosecond measurements reveal new physical insights in photo ionization dynamics from atoms, molecules and condensed matter. However, on such time scales even small timing jitter can significantly reduce the time resolution in pump-probe…
Attosecond photoelectron spectroscopy is often performed with interferometric experimental setups that require outstanding stability. We demonstrate and characterize in detail an actively stabilized, versatile, high spectral resolution…
Parity mixing in photoionization, i.e. when emitted electrons have different parities but the same energy, causes interference observable only in angle-resolved measurements. The interference typically manifests as a symmetry violation in…
Attosecond Pulse Trains (APT) generated by high-harmonic generation (HHG) of high-intensity near-infrared (IR) laser pulses have proven valuable for studying the electronic dynamics of atomic and molecular species. However, the high…
A frequency doubled I/Q modulator based optical single-sideband (OSSB) laser system is demonstrated for atomic physics research, specifically for atom interferometry where the presence of additional sidebands causes parasitic transitions.…
We analyze interference processes in atomic ionization induced by a two-color laser with fundamental frequency $\omega $ and its second harmonic $2\omega $. The interplay between inter- and intracycle interference processes give rise to…
We present an analytical model that characterizes two-photon transitions in the presence of autoionising states. We applied this model to interpret resonant RABITT spectra, and show that, as a harmonic traverses a resonance, the phase of…
The two basic approaches underlying the metrology of attosecond pulse trains are compared, i.e. the 2nd order Intensity Volume Autocorrelation and the Resolution of Attosecond Beating by Interference of Two photon Transitions (RABITT). They…
We develop a first-principles simulation method for attosecond time-resolved photoelectron spectroscopy. This method enables us to directly simulate the whole experimental processes, including excitation, emission and detection on equal…
We develop a novel technique for modeling of atomic and molecular ionization in superposition of XUV and IR fields with characteristics typical for attosecond streaking and RABBITT experiments. The method is based on solving the…
Attosecond interferometry in a two-color field is central to attosecond metrology and spectroscopy. In this technique, a photoelectron wave packet is released when a single photon from an extreme ultraviolet comb is absorbed. The wave…
We simulate the transient absorption of attosecond pulses of infrared-laser-dressed atoms by considering a three-level system with the adiabatic approximation. The delay-dependent interference features are investigated from the perspective…
Reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) is a powerful photoelectron spectroscopy, offering direct access to internal dynamics of the target. It is being increasingly applied to molecular…
Following up on a previous paper on two-color photoionization of Ar(3p) [Bharti et al., Phys. Rev. A 103 (2021) 022834], we present measurements and calculations for a modified three-sideband (3-SB) version of the "reconstruction of…
We present an innovative beamline for extreme ultraviolet (XUV)-infrared (IR) pump-probe reflection spectroscopy in solids with attosecond temporal resolution. The setup uses an actively stabilized interferometer, where attosecond pulse…
This paper reports on a detailed performance characterization of a recently developed optical single-sideband (OSSB) laser system based on an IQ modulator and second-harmonic generation for rubidium atom interferometry experiments. The…
The process of reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) can become resonant with a discrete atomic level either in the intermediate or the final continuous states. Experimental observations of…