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Layered NbOX$_2$ ($X=\mathrm{Cl,\,Br,\,I}$), a member of the van der Waals ferroelectric family, exhibits intrinsic ferroelectricity and pronounced nonlinear optical responses, making it a promising candidate for integrated nanophotonics…

Monolayer transition metal dichalcogenides (TMDs) exhibit high nonlinear optical (NLO) susceptibilities. Experiments on MoS$_2$ have indeed revealed very large second-order ($\chi^{(2)}$) and third-order ($\chi^{(3)}$) optical…

Second-order nonlinear optical interactions, including second harmonic generation (SHG) and sum-frequency generation (SFG), can reveal a wealth of information about chemical, electronic, and vibrational dynamics at the nanoscale. Here, we…

Second-harmonic generation in resonant structures is commonly evaluated in terms of intracavity field enhancement at the fundamental and harmonic frequencies. Here, we formulate nonlinear frequency conversion within a symmetry-resolved…

Intense laser-driven nonlinear optical phenomena in two-dimensional (2D) nodal-line semimetals (NLS) exhibit complex mechanisms, particularly in the NbSi$_{x}$Te$_{2}$ material systems characterized by nonsymmorphic symmetry-protected band…

Optics · Physics 2025-08-25 Navdeep Rana , M. S. Mrudul , Amar Bharti , Sucharita Giri , Gopal Dixit

Strong periodic driving with light offers the potential to coherently manipulate the properties of quantum materials on ultrafast timescales. Recently, strategies have emerged to drastically alter electronic and magnetic properties by…

Strongly Correlated Electrons · Physics 2022-06-20 Jun-Yi Shan , M. Ye , Sungmin Lee , Je-Geun Park , L. Balents , D. Hsieh

The existence of large nonlinear optical coefficients is one of the preconditions for using nonlinear optical materials in nonlinear optical devices. For a crystal, such large coefficients can be achieved by matching photon energies with…

Materials Science · Physics 2018-12-27 J. L. Cheng , J. E. Sipe , S. W. Wu , Chunlei Guo

Recent techniques have allowed transition metal dichalcogenides (TMD) monolayers to be grown and adequately characterised. Of particular interest, their nonlinear optical response presents many promising opportunities for future…

Mesoscale and Nanoscale Physics · Physics 2020-03-06 David N. Carvalho , Fabio Biancalana

The van der Waals coefficients and the separation dependent retardation functions of the interactions between the atomically thin films of the multi-layered transition metal molybdenum disulfide (MoS$_2$) dichalcogenides with the alkali…

Materials Science · Physics 2020-08-12 Shankar Dutt , Sukhjit Singh , A. Mahajan , Bindiya Arora , B. K. Sahoo

Hyperbolic phonon polaritons (HPhPs) in orthorhombic-phase molybdenum trioxide ($\alpha$-MoO3) show in-plane hyperbolicity, great wavelength compression and ultra-long lifetime, therefore holding great potential in nanophotonic…

Materials Science · Physics 2020-11-25 Weikang Dong , Ruishi Qi , Tiansheng Liu , Yi Li , Ning Li , Ze Hua , Zirui Gao , Shuyuan Zhang , Kaihui Liu , Jiandong Guo , Peng Gao

Black phosphorus stands out from the family of two-dimensional materials as a semiconductor with a direct, layer-dependent bandgap in energy corresponding to the spectral range from the visible to the mid-infrared (mid-IR), as well as many…

Optics · Physics 2017-10-10 Ruoming Peng , Kaveh Khaliji , Nathan Youngblood , Roberto Grassi , Tony Low , Mo Li

The non-linear propagation of the intense near-infrared (NIR) driving field in wide bandgap materials pose a challenge and an opportunity to control the spectral properties of high harmonic generation (HHG) in solids. Here, we have…

Optics · Physics 2023-07-06 Mukhtar Hussain , Gareth O Williams , Tayyab Imran , Marta Fajardo

Nonlinear optics lies at the heart of classical and quantum light generation. The invention of periodic poling revolutionized nonlinear optics and its commercial applications by enabling robust quasi-phase-matching in crystals such as…

Second harmonic generation is a powerful tool directly connected to the symmetry of materials. Phase transitions, lattice rotations or electromagnetic coupling in multiferroic compounds can be revealed by using second harmonic…

Optics · Physics 2010-01-11 Pablo Molina , Mariola O Ramirez , Basilio J. Garcia , Luisa E. Bausa

Integrating two-dimensional (2D) crystals into optical fibers can grant them optoelectronic properties and extend their range of applications. However, our ability to produce complicated structures is limited by the challenges of chemical…

Applied Physics · Physics 2018-07-03 Yi-feng Xiong , Jin-hui Chen , Fei Xu

Second-harmonic generation is of paramount importance in several fields of science and technology, including frequency conversion, self-referencing of frequency combs, nonlinear spectroscopy and pulse characterization. Advanced…

We review recent work on low-frequency Floquet engineering and its application to quantum materials driven by light, emphasizing van der Waals systems hosting Moir\'e superlattices. These non-equilibrium systems combine the twist-angle…

Mesoscale and Nanoscale Physics · Physics 2021-04-09 Martin Rodriguez-Vega , Michael Vogl , Gregory A. Fiete

Hybrid materials are crucial in photovoltaics where the overall efficiency of the heterostructure is closely related to the level of charge transfer at the interface. Here, using various metal / poly(3-hexylthiophene)(P3HT) heterostructure…

Materials Science · Physics 2019-08-20 V. Ongun Özçelik , Yingmin Li , Wei Xiong , Francesco Paesani

Optical nonlinearities, one of the most fascinating properties of two-dimensional (2D) materials, are essential for exploring novel physics in 2D systems and developing next-generation nonlinear optical applications. While tremendous…

The biaxial van der Waals semiconductor $\alpha$-phase molybdenum trioxide ($\alpha$-MoO$_3$) has recently received significant attention due to its ability to support highly anisotropic phonon polaritons (PhPs) -infrared (IR) light coupled…