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The magnetic properties of the quasi-two-dimensional van der Waals magnet Fe$_{5-\delta}$GeTe$_2$ (F5GT), which has a high ferromagnetic ordering temperature $T_{\text{C}}$ $\sim$ 315 K, remains to be better understood. It has been…

Strongly Correlated Electrons · Physics 2023-04-26 Xiang Chen , Wei Tian , Yu He , Hongrui Zhang , Tyler L. Werner , Saul Lapidus , Jacob P. C. Ruff , Ramamoorthy Ramesh , Robert J. Birgeneau

Intercalated van der Waals (vdW) magnetic materials host unique magnetic properties due to the interplay of competing interlayer and intralayer exchange couplings, which depend on the intercalant concentration within the van der Waals gaps.…

We have investigated the nature of ferromagnetic order and phase transitions in two dimensional (2D) van der Waals (vdW) layered material, Fe$_4$GeTe$_2$ through measurements of magnetization, magneto-caloric Effect (MCE), and heat…

We present a thorough magnetization and magneto-transport study of the diluted Fe-intercalated CrTe2 family member, Fe1/5CrTe2, a van der Waals ferromagnet. Fe1/5CrTe2 shows an elevated Curie transition temperature of 182 K in comparison to…

Strongly Correlated Electrons · Physics 2026-04-07 M. Lamba , P. Saha , K. Yadav , N. Kamboj , S. Patnaik

We have systematically studied the magnetic properties of chromium chalcogene compounds FeCr$_2$Se$_{4-x}$Te$_x$. The FeCr2Se4 undergoes antiferromagnetic ordering below 222 K. Substitution of tellurium lowers the antiferromagnetic ordering…

Materials Science · Physics 2019-04-16 C. S. Yadav , S. K. Pandey , P. L. Paulose

The magnetism in Mn$_3$Si$_2$Te$_6$ has been investigated using thermodynamic measurements, first principles calculations, neutron diffraction and diffuse neutron scattering on single crystals. These data confirm that Mn$_3$Si$_2$Te$_6$ is…

We report on neutron diffraction, thermal expansion, magnetostriction, dielectric, and specific heat measurements on polycrystalline FeCr2S4 in external magnetic fields. The ferrimagnetic ordering temperatures $T_{\mathrm{C}}\approx 170$ K…

The quasi-two-dimensional van der Waals magnet Fe$_{5-\delta}$GeTe$_2$ has emerged as a promising platform for electronic and spintronic functionalities at room temperature, owing to its large ferromagnetic ordering temperature…

Crystallographic and magnetic properties of Fe5PB2, Fe4CoPB2, Fe4MnPB2, Fe5SiB2, Fe4CoSiB2, and Fe4MnSiB2 are reported. All adopt the tetragonal Cr5B3 structure-type and are ferromagnetic at room temperature with easy axis of magnetization…

Materials Science · Physics 2015-09-10 Michael A. McGuire , David S. Parker

We report a detailed study of the magnetic, transport, and thermodynamic properties of Ce$_2$Te$_5$ single crystals, a layered $f$-electron van der Waals magnet. Four consecutive transitions at $\sim$ 5.2, 2.1, 0.9, and 0.4 K were observed…

Strongly Correlated Electrons · Physics 2022-10-17 Yu Liu , M. M. Bordelon , A. Weiland , P. F. S. Rosa , S. M. Thomas , J. D. Thompson , F. Ronning , E. D. Bauer

To tune the magnetic properties of hexagonal ferrites, a family of magnetoelectric multiferroic materials, by atomic-scale structural engineering, we studied the effect of structural distortion on the magnetic ordering temperature (TN).…

Using density-functional theory calculations and experimental investigations on structural, magnetic and dielectric properties, we have elucidated a unique tetragonal ground state for MnTi2O4, a Ti^{3+} (3d^1)-ion containing spinel-oxide.…

Strongly Correlated Electrons · Physics 2019-10-09 A. Rahaman , M. Chakraborty , T. Paramanik , R. K. Maurya , S. Mahana , R. Bindu , D. Topwal , P. Mahadevan , D. Choudhury

Enhancement of Curie temperature ($T_\mathrm{C}$) of two-dimensional (2D) magnets is immensely desirable for room temperature spintronic applications. Fe$_{5}$GeTe$_{2}$ is an exceptional van der Waals metallic ferromagnet due to its…

Materials Science · Physics 2023-05-09 Sukanya Ghosh , Soheil Ershadrad , Biplab Sanyal

We have grown a series of nickel substituted single crystals of the layered ferromagnet (FM) Fe$_3$GeTe$_2$. The large single crystalline samples of (Fe$_{1-x}$Ni$_x$)$_3$GeTe$_2$ with $x = 0-0.84$ were characterized with single crystal…

Van der Waals magnetic materials are building blocks for novel kinds of spintronic devices and playgrounds for exploring collective magnetic phenomena down to the two-dimensional limit. Chromium-tellurium compounds are relevant in this…

The structural and magnetic properties of Mn$_2$FeSbO$_6$ single-crystalline mineral and ceramic samples synthesized under thermobaric treatment have been investigated, and compared to theoretical predictions based on first-principles…

Strongly Correlated Electrons · Physics 2011-05-20 R. Mathieu , S. A. Ivanov , G. V. Bazuev , M. Hudl , P. Lazor , I. V. Solovyev , P. Nordblad

We investigate the electronic structure of Chromium Nitride (CrN) across the first-order magneto-structural transition at T_N ~ 286 K. Resonant photoemission spectroscopy shows a gap in the 3d partial density of states at the Fermi level…

Fe5-xGeTe2 is a van der Waals material with one of the highest reported bulk Curie temperatures, $T_C$ ~ 310K. In this study, theoretical calculations and experiments are utilized to demonstrate that the magnetic ground state is highly…

Materials Science · Physics 2020-08-20 Andrew F. May , Mao-Hua Du , Valentino R. Cooper , Michael A. McGuire

We report the results of Mn substitution for Ni in CeNi0.8Bi2, (i.e. CeNi0.8-xMnxBi2). All the samples have an antiferromagnetic ordered state below TN = 5.0 K due to localized 4f-magnetic moment on the Ce ions. Besides this…

Strongly Correlated Electrons · Physics 2015-06-19 Soo-Whan Kim , Kyu Joon Lee , D. T. Adroja , F. Demmel , J. W. Taylor , Myung-Hwa Jung

In order to tune the magnetic properties of the cleavable high-Curie temperature ferromagnet Fe$_{5-x}$GeTe$_2$, the effect of increasing the electron count through arsenic substitution has been investigated. Small additions of arsenic (2.5…

Materials Science · Physics 2021-11-15 Andrew F. May , Jiaqiang Yan , Raphael Hermann , Mao-Hua Du , Michael A. McGuire
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