Related papers: On Sub-Sevenfold Symmetries in LH2 Stacked Ring Sc…
We perform a quantum mechanical study of the peptides that are part of the LH2 complex from Rhodopseudomonas acidophila, a non-sulfur purple bacteria that has the ability of producing chemical energy from photosynthesis. The electronic…
The remarkable rotational symmetry of the photosynthetic antenna complexes of purple bacteria has long been thought to enhance their light harvesting and excitation energy transport. We study the role of symmetry by modeling hypothetical…
Photosynthesis, the process by which energy from sunlight drives cellular metabolism, relies on a unique organization of light-harvesting and reaction center complexes. Recently, the organization of light-harvesting LH2 complexes and…
Electronic 2D spectroscopy allows nontrivial quantum effects in chemistry and biology to be explored in unprecedented detail. Here, we apply recently developed fluorescence detected coherent 2D spectroscopy to study the light harvesting…
Photosynthetic organisms use networks of chromophores to absorb sunlight and deliver the energy to reaction centres, where charge separation triggers a cascade of chemical steps to store the energy. We present a detailed model of the…
One of the important nonclassical effects in quantum optics is the anti-bunching, which has been observed in a large class of physical systems - including light-harvesting antennas with cyclic structures. The units of the ring couple with…
We review recent theoretical calculations of quantum entanglement in photosynthetic light harvesting complexes. These works establish, for the first time, a manifestation of this characteristically quantum mechanical phenomenon in…
Some species of purple bacteria as, e.g., Rhodobacter sphaeroides contain the protein PufX. Concurrently, the light harvesting complexes 1 (LH1) form dimers of open rings. In mutants without PufX, the LH1s are closed rings and…
For more than 50 years we have known that photosynthetic systems harvest solar energy with almost unit {\it quantum efficiency}. However, recent experimental evidence of {\it quantum coherence} during the excitonic energy transport in…
Using the reduced density matrix formalism the exciton scattering in light-harvesting systems of purple bacteria is calculated. The static disorder (fluctuations of the site energies) as well as the dynamic disorder (dissipation) is taken…
Large scale simulations of light-matter interaction in natural photosynthetic antenna complexes containing more than one hundred thousands chlorophyll molecules, comparable with natural size, have been performed. Photosynthetic antenna…
To understand the photophysics of molecular aggregates, exciton model of J- and H-aggregate has been extensively utilized. However, it lacks consideration of crystal symmetry. Although discrete molecules may lack symmetry, their aggregates…
We study the supersymmetric properties of D7-branes in the warped deformed conifold. We consider the $\kappa$-symmetry conditions on D7-branes in this specific warped background, taking into account the background NS-NS 2-form flux. While…
Entangled photons exhibit non-classical light-matter interactions that create new opportunities in materials and molecular science. For example, in entangled two-photon absorption, the intensity-dependence scales linearly as if only one…
In this paper, we show that any non-arithmetic hyperbolic $2$-bridge link complement admits no hidden symmetries. As a corollary, we conclude that a hyperbolic $2$-bridge link complement cannot irregularly cover a hyperbolic $3$-manifold.…
We experimentally generate and tomographically characterize a mixed, genuinely non-Gaussian bipartite continuous-variable entangled state. By testing entanglement in 2$\times$2-dimensional two-qubit subspaces, entangled qubits are localized…
The LH-II of purple bacteria Rhodospirillum (Rs.) molischianum and Rhodopseudomonas (Rps.) acidophila adopts a highly symmetrical ring shape, with a radius of about 7 nm. In the case of Rps. acidophila the ring has a ninefold symmetry axis,…
We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by…
A minimal, one-parameter model of the excitonic Hamiltonian for the light harvesting complex of purple bacteria (LH2) based on ab initio calculation of the excitonic energies is proposed. The set of input parameters contains positions of…
Photosynthetic organisms rely on a network of light-harvesting protein-pigment complexes to efficiently absorb sunlight and transfer excitation energy to reaction center proteins for charge separation. In photosynthetic purple bacteria,…