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We enlarge our results from the study of the hopping mechanism of the oscillation excitation transport in 1D model of one biology-like macromolecular chain to the case of a system composed from two 1D parallel macromolecular chains with…

Mesoscale and Nanoscale Physics · Physics 2016-01-12 D. Čevizović , S. Petković , S. Galović , A. Chizhov , A. Reshetnyak

We investigate the spread of correlations carried by an excitation in a 1-dimensional lattice system with high on-site energy disorder and long-range couplings with a power-law dependence on the distance ($\propto r^{-\mu}$). The increase…

Disordered Systems and Neural Networks · Physics 2022-06-01 Karol Kawa , Paweł Machnikowski

Large exciton diffusion lengths generally improve the performance of organic semiconductor devices, since they enable energy to be transported farther during the exciton lifetime. However, the physics of exciton motion in disordered organic…

Chemical Physics · Physics 2023-03-17 Daniel Balzer , Ivan Kassal

The presence of static off-diagonal disorder promotes coherent exciton transport while diffusive motion can be recovered in the presence of fluctuations in the diagonal and off-diagonal elements of the Hamiltonian. Here we study the…

Statistical Mechanics · Physics 2018-10-12 Rajesh Dutta , Biman Bagchi

Understanding the transport mechanism of electronic excitations in conjugated polymers is key to advancing organic optoelectronic applications, such as solar cells, OLEDs and flexible electronics. While crystalline polymers can be studied…

Materials Science · Physics 2021-12-13 Francesco Campaioli , Jared H. Cole

Unravelling the nature of energy transport in multi-chromophoric photosynthetic complexes is essential to extract valuable design blueprints for light-harvesting applications. Long-range exciton transport in such systems is facilitated by a…

Moir\'e superlattices of transition-metal dichalcogenides (TMDs) host strongly interacting Bose-Fermi mixtures in which bosonic excitons coexist with correlated electron lattices. Using ultrafast, time- and energy-resolved photoluminescence…

We investigate exciton transport through one-dimensional molecular aggregates interacting strongly with a cavity mode. Unlike several prior theoretical studies treating the monomers as simple two-level systems, exciton-vibration coupling is…

Mesoscale and Nanoscale Physics · Physics 2019-03-14 Jingyu Liu , Qing Zhao , Ning Wu

Self-assembled aggregates of pigment molecules are potential building blocks for excitonic circuits that find their application in energy conversion and optical signal processing. Recent experimental studies of one-dimensional…

Mesoscale and Nanoscale Physics · Physics 2017-10-03 Semion K. Saikin , Mars A. Shakirov , Christoph Kreisbeck , Uri Peskin , Yurii N. Proshin , Alan Aspuru-Guzik

We present a theoretical model for the study of exciton dynamics in J-aggregated monolayers of fluorescent dyes. The excitonic evolution is described by a Monte-Carlo wave function approach which allows for a unified description of the…

Chemical Physics · Physics 2012-07-20 Stéphanie Valleau , Semion K. Saikin , Man-Hong Yung , Alán Aspuru-Guzik

Exciton dynamics dictate the evolution of photoexcited carriers in photovoltaic and optoelectronic devices. However, interpreting their experimental signatures is a challenging theoretical problem due to the presence of both electron-phonon…

Excitation energy transport can be significantly enhanced by strong light-matter interactions. In the present work, we explore intriguing features of coherent transient exciton wave packet dynamics on a lossless disordered polaritonic wire.…

Quantum Physics · Physics 2024-02-26 Gustavo J. R. Aroeira , Kyle T. Kairys , Raphael F. Ribeiro

We study transport of interacting particles in weakly disordered media. Our one-dimensional system includes (i) disorder: the hopping rate governing the movement of a particle between two neighboring lattice sites is inhomogeneous, and (ii)…

Statistical Mechanics · Physics 2009-05-13 E. Ben-Naim , P. L. Krapivsky

We develop a temperature dependent theory for singlet exciton hopping transport in disordered semiconductors. It draws on the transport level concept within a F\"orster transfer model and bridges the gap in describing the transition from…

Mesoscale and Nanoscale Physics · Physics 2018-08-22 Mehdi Ansari-Rad , Stavros Athanasopoulos

Single-particle transport in disordered potentials is investigated on scales below the localization length. The dynamics on those scales is concretely analyzed for the 3-dimensional Anderson model with Gaussian on-site disorder. This…

Statistical Mechanics · Physics 2010-11-05 Robin Steinigeweg , Hendrik Niemeyer , Jochen Gemmer

We show that the biomolecular exciton dynamics under the influence of slow polarization fluctuations in the solvent cannot be described by approaches which are perturbative in the system-bath coupling. For this, we compare results for the…

Soft Condensed Matter · Physics 2009-12-01 P. Nalbach , M. Thorwart

The interplay between static and dynamic disorder and collective optical response in molecular ensembles is an important characteristic of nanoplasmonic and nanophotonic molecular systems. Here we investigate the cooperative superradiant…

In recent years it has become clear that the transport of excitons and charge carriers in molecular systems can be enhanced by coherent coupling with photons, giving rise to the formation of hybrid excitations known as polaritons. Such…

Materials Science · Physics 2023-01-19 M. Balasubrahmaniyam , Arie Simkovich , Adina Golombek , Guy Ankonina , Tal Schwartz

Effective medium theory of transport in disordered systems, whose basis is the replacement of spatial disorder by temporal memory, is extended in several practical directions. Restricting attention to a 1-dimensional system with bond…

Statistical Mechanics · Physics 2009-11-13 V. M. Kenkre , Z. Kalay , P. E. Parris

We study the nature of the energy transfer process within a pair of coupled two-level systems (donor and acceptor) subject to interactions with the surrounding environment. Going beyond a standard weak-coupling approach, we derive a master…

Quantum Physics · Physics 2011-04-05 Dara P. S. McCutcheon , Ahsan Nazir